Anisotropic angular magnetoresistance and Fermi surface topology of the candidate novel topological metal Pd3Pb

Ghimire, N. J.; Khan, Mojammel A.; Botana, A. S.; Jiang, J. S.; Mitchell, J. F.

doi:10.1103/PhysRevMaterials.2.081201

Title: Anisotropic angular magnetoresistance and Fermi surface topology of the candidate novel topological metal ${Pd}_{3} Pb$

Abstract

In this paper, the recent realization of topological electronic states such as Dirac and Weyl fermions in real materials and their potential for future energy and electronics applications has motivated interest in the study of new forms of topological behavior embodied through new materials. Pd₃Pb is one such candidate predicted recently to host unique topological features, including a dispersionless band near the Fermi level and triple nodal points hosting Dirac fermions and open Fermi arcs. Here, we report the crystal growth and electric transport properties of Pd₃Pb. Our low field magnetoresistance measurements indicate an anisotropic Fermi surface. We found that Pd₃Pb manifests a large transverse magnetoresistance, which reaches 650% at 1.8 K and 14 T, and pronounced Shubnikov-de Haas (SdH) oscillations. Preliminary analysis of the field dependence of the SdH oscillations points to the likelihood of nontrivial Berry phase in Pd₃Pb. Further studies in high field limit are desirable to extend the realization of the topological properties of the predicted novel fermions in this material.

Authors:

Ghimire, N. J. ^[1]; Khan, Mojammel A. ^[1]; Botana, A. S. ^[1]; Jiang, J. S. ^[1]; Mitchell, J. F. ^[1]

Argonne National Lab. (ANL), Argonne, IL (United States)

Publication Date:: Mon Aug 20 00:00:00 EDT 2018

Research Org.:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE Office of Science (SC)

OSTI Identifier:: 1471586

Alternate Identifier(s):: OSTI ID: 1465229

Grant/Contract Number:: AC02-06CH11357

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review Materials

Additional Journal Information:: Journal Volume: 2; Journal Issue: 8; Journal ID: ISSN 2475-9953

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; Toplogical material; Quantum oscillations; Magnetoresistance

Citation Formats


                    Ghimire, N. J., Khan, Mojammel A., Botana, A. S., Jiang, J. S., and Mitchell, J. F. Anisotropic angular magnetoresistance and Fermi surface topology of the candidate novel topological metal Pd3Pb.  United States: N. p., 2018. 
Web.  doi:10.1103/PhysRevMaterials.2.081201.

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                    Ghimire, N. J., Khan, Mojammel A., Botana, A. S., Jiang, J. S., & Mitchell, J. F. Anisotropic angular magnetoresistance and Fermi surface topology of the candidate novel topological metal Pd3Pb.  United States.  https://doi.org/10.1103/PhysRevMaterials.2.081201

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                    Ghimire, N. J., Khan, Mojammel A., Botana, A. S., Jiang, J. S., and Mitchell, J. F. Mon .  
"Anisotropic angular magnetoresistance and Fermi surface topology of the candidate novel topological metal Pd3Pb".  United States.  https://doi.org/10.1103/PhysRevMaterials.2.081201.  https://www.osti.gov/servlets/purl/1471586.

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@article{osti_1471586,

  title        = {Anisotropic angular magnetoresistance and Fermi surface topology of the candidate novel topological metal Pd3Pb},

  author       = {Ghimire, N. J. and Khan, Mojammel A. and Botana, A. S. and Jiang, J. S. and Mitchell, J. F.},

  abstractNote = {In this paper, the recent realization of topological electronic states such as Dirac and Weyl fermions in real materials and their potential for future energy and electronics applications has motivated interest in the study of new forms of topological behavior embodied through new materials. Pd3Pb is one such candidate predicted recently to host unique topological features, including a dispersionless band near the Fermi level and triple nodal points hosting Dirac fermions and open Fermi arcs. Here, we report the crystal growth and electric transport properties of Pd3Pb. Our low field magnetoresistance measurements indicate an anisotropic Fermi surface. We found that Pd3Pb manifests a large transverse magnetoresistance, which reaches 650% at 1.8 K and 14 T, and pronounced Shubnikov-de Haas (SdH) oscillations. Preliminary analysis of the field dependence of the SdH oscillations points to the likelihood of nontrivial Berry phase in Pd3Pb. Further studies in high field limit are desirable to extend the realization of the topological properties of the predicted novel fermions in this material.},

  doi          = {10.1103/PhysRevMaterials.2.081201},

  journal      = {Physical Review Materials},

  number       = 8,

  volume       = 2,

  place        = {United States},

  year         = {Mon Aug 20 00:00:00 EDT 2018},

  month        = {Mon Aug 20 00:00:00 EDT 2018}

}

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Title: Anisotropic angular magnetoresistance and Fermi surface topology of the candidate novel topological metal Pd 3 Pb

Abstract

Citation Formats

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Title: Anisotropic angular magnetoresistance and Fermi surface topology of the candidate novel topological metal ${Pd}_{3} Pb$

Generalized Gradient Approximation Made Simple
journal, October 1996

Weyl and Dirac semimetals in three-dimensional solids
journal, January 2018

Extremely large magnetoresistance and Kohler's rule in ${PdSn}_{4}$ : A complete study of thermodynamic, transport, and band-structure properties
journal, October 2017

Observation of the Chiral-Anomaly-Induced Negative Magnetoresistance in 3D Weyl Semimetal TaAs
journal, August 2015

Angle Dependence of the Orbital Magnetoresistance in Bismuth
journal, June 2015

Skyrmion Lattice in a Chiral Magnet
journal, February 2009

Magnetic Oscillations in Metals
book, October 2011

Introduction to topological superconductivity and Majorana fermions
journal, November 2012

Rietveld refinement guidelines
journal, February 1999

Recent advances in magnetic structure determination by neutron powder diffraction
journal, October 1993

Magnetotransport of single crystalline NbAs
journal, March 2015

Coexistence of triple nodal points, nodal links, and unusual flat bands in intermetallic $A Pd_{3}$ ( $A = Pb$ , Sn)
journal, July 2018

Discovery of a Weyl fermion semimetal and topological Fermi arcs
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