DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Attosecond time-resolved photoelectron holography

Abstract

Ultrafast strong-field physics provides insight into quantum phenomena that evolve on an attosecond time scale, the most fundamental of which is quantum tunneling. The tunneling process initiates a range of strong field phenomena such as high harmonic generation (HHG), laser-induced electron diffraction, double ionization and photoelectron holography—all evolving during a fraction of the optical cycle. Here we apply attosecond photoelectron holography as a method to resolve the temporal properties of the tunneling process. Adding a weak second harmonic (SH) field to a strong fundamental laser field enables us to reconstruct the ionization times of photoelectrons that play a role in the formation of a photoelectron hologram with attosecond precision. In conclusion, we decouple the contributions of the two arms of the hologram and resolve the subtle differences in their ionization times, separated by only a few tens of attoseconds.

Authors:
 [1];  [2];  [2];  [2]; ORCiD logo [2];  [2]; ORCiD logo [3];  [2];  [2];  [4];  [2]
  1. Univ. of Colorado, Boulder, CO (United States); Weizmann Institute of Science, Rehovot (Israel)
  2. Weizmann Institute of Science, Rehovot (Israel)
  3. SLAC National Accelerator Lab., Menlo Park, CA (United States)
  4. Max-Born-Institut, Berlin (Germany)
Publication Date:
Research Org.:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1463349
Grant/Contract Number:  
AC02-76SF00515
Resource Type:
Accepted Manuscript
Journal Name:
Nature Communications
Additional Journal Information:
Journal Volume: 9; Journal Issue: 1; Journal ID: ISSN 2041-1723
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS

Citation Formats

Porat, G., Alon, G., Rozen, S., Pedatzur, O., Kruger, M., Azoury, D., Natan, A., Orenstein, G., Bruner, B. D., Vrakking, M. J. J., and Dudovich, N. Attosecond time-resolved photoelectron holography. United States: N. p., 2018. Web. doi:10.1038/s41467-018-05185-6.
Porat, G., Alon, G., Rozen, S., Pedatzur, O., Kruger, M., Azoury, D., Natan, A., Orenstein, G., Bruner, B. D., Vrakking, M. J. J., & Dudovich, N. Attosecond time-resolved photoelectron holography. United States. https://doi.org/10.1038/s41467-018-05185-6
Porat, G., Alon, G., Rozen, S., Pedatzur, O., Kruger, M., Azoury, D., Natan, A., Orenstein, G., Bruner, B. D., Vrakking, M. J. J., and Dudovich, N. Wed . "Attosecond time-resolved photoelectron holography". United States. https://doi.org/10.1038/s41467-018-05185-6. https://www.osti.gov/servlets/purl/1463349.
@article{osti_1463349,
title = {Attosecond time-resolved photoelectron holography},
author = {Porat, G. and Alon, G. and Rozen, S. and Pedatzur, O. and Kruger, M. and Azoury, D. and Natan, A. and Orenstein, G. and Bruner, B. D. and Vrakking, M. J. J. and Dudovich, N.},
abstractNote = {Ultrafast strong-field physics provides insight into quantum phenomena that evolve on an attosecond time scale, the most fundamental of which is quantum tunneling. The tunneling process initiates a range of strong field phenomena such as high harmonic generation (HHG), laser-induced electron diffraction, double ionization and photoelectron holography—all evolving during a fraction of the optical cycle. Here we apply attosecond photoelectron holography as a method to resolve the temporal properties of the tunneling process. Adding a weak second harmonic (SH) field to a strong fundamental laser field enables us to reconstruct the ionization times of photoelectrons that play a role in the formation of a photoelectron hologram with attosecond precision. In conclusion, we decouple the contributions of the two arms of the hologram and resolve the subtle differences in their ionization times, separated by only a few tens of attoseconds.},
doi = {10.1038/s41467-018-05185-6},
journal = {Nature Communications},
number = 1,
volume = 9,
place = {United States},
year = {Wed Jul 18 00:00:00 EDT 2018},
month = {Wed Jul 18 00:00:00 EDT 2018}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 63 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Studying the universality of field induced tunnel ionization times via high-order harmonic spectroscopy
journal, October 2014

  • Soifer, H.; Bruner, B. D.; Negro, M.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 47, Issue 20
  • DOI: 10.1088/0953-4075/47/20/204029

Attosecond real-time observation of electron tunnelling in atoms
journal, April 2007

  • Uiberacker, M.; Uphues, Th.; Schultze, M.
  • Nature, Vol. 446, Issue 7136
  • DOI: 10.1038/nature05648

Reading diffraction images in strong field ionization of diatomic molecules
journal, May 2004

  • Spanner, Michael; Smirnova, Olga; Corkum, Paul B.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 37, Issue 12
  • DOI: 10.1088/0953-4075/37/12/L02

Attosecond Ionization and Tunneling Delay Time Measurements in Helium
journal, December 2008


Resolving the time when an electron exits a tunnelling barrier
journal, May 2012

  • Shafir, Dror; Soifer, Hadas; Bruner, Barry D.
  • Nature, Vol. 485, Issue 7398
  • DOI: 10.1038/nature11025

What will it take to observe processes in 'real time'?
journal, February 2014

  • Leone, Stephen R.; McCurdy, C. William; Burgdörfer, Joachim
  • Nature Photonics, Vol. 8, Issue 3
  • DOI: 10.1038/nphoton.2014.48

Attosecond science
journal, June 2007

  • Corkum, P. B.; Krausz, Ferenc
  • Nature Physics, Vol. 3, Issue 6
  • DOI: 10.1038/nphys620

Attosecond Time-Resolved Imaging of Molecular Structure by Photoelectron Holography
journal, June 2012


Strong field approximation for systems with Coulomb interaction
journal, September 2008


Theory of high-harmonic generation by low-frequency laser fields
journal, March 1994


Attosecond tunnelling interferometry
journal, August 2015

  • Pedatzur, O.; Orenstein, G.; Serbinenko, V.
  • Nature Physics, Vol. 11, Issue 10
  • DOI: 10.1038/nphys3436

Two-Color Strong-Field Photoelectron Spectroscopy and the Phase of the Phase
journal, July 2015


New frontiers in attosecond science
journal, January 2009


Imaging an aligned polyatomic molecule with laser-induced electron diffraction
journal, June 2015

  • Pullen, Michael G.; Wolter, Benjamin; Le, Anh-Thu
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms8262

Signatures of the continuum electron phase in molecular strong-field photoelectron holography
journal, July 2014

  • Meckel, M.; Staudte, A.; Patchkovskii, S.
  • Nature Physics, Vol. 10, Issue 8
  • DOI: 10.1038/nphys3010

Anatomy of strong field ionization
journal, January 2005


Subcycle interference dynamics of time-resolved photoelectron holography with midinfrared laser pulses
journal, October 2011


Velocity map imaging of ions and electrons using electrostatic lenses: Application in photoelectron and photofragment ion imaging of molecular oxygen
journal, September 1997

  • Eppink, André T. J. B.; Parker, David H.
  • Review of Scientific Instruments, Vol. 68, Issue 9
  • DOI: 10.1063/1.1148310

Laser-Induced Electron Tunneling and Diffraction
journal, June 2008


Imaging ultrafast molecular dynamics with laser-induced electron diffraction
journal, March 2012

  • Blaga, Cosmin I.; Xu, Junliang; DiChiara, Anthony D.
  • Nature, Vol. 483, Issue 7388
  • DOI: 10.1038/nature10820

Time-Resolved Holography with Photoelectrons
journal, December 2010


Studies of multiphoton production of vacuum-ultraviolet radiation in the rare gases
journal, January 1987

  • McPherson, A.; Gibson, G.; Jara, H.
  • Journal of the Optical Society of America B, Vol. 4, Issue 4
  • DOI: 10.1364/JOSAB.4.000595

Toward real-time charged-particle image reconstruction using polar onion-peeling
journal, May 2009

  • Roberts, G. M.; Nixon, J. L.; Lecointre, J.
  • Review of Scientific Instruments, Vol. 80, Issue 5
  • DOI: 10.1063/1.3126527

Attosecond physics
conference, January 2007

  • Kienberger, Reinhard; Krausz, Ferenc
  • ICALEO® 2007: 26th International Congress on Laser Materials Processing, Laser Microprocessing and Nanomanufacturing, International Congress on Applications of Lasers & Electro-Optics
  • DOI: 10.2351/1.5061046

Strong Field Approximation for Systems with Coulomb Interaction
text, January 2008


Two-Color Strong-Field Photoelectron Spectroscopy and the Phase of the Phase
text, January 2015


Imaging an aligned polyatomic molecule with laser-induced electron diffraction
text, January 2015


New frontiers in attosecond science
journal, January 2009


Atomic phenomena in bichromatic laser fields
journal, May 2001


Attosecond real-time observation of electron tunnelling in atoms
journal, April 2007

  • Uiberacker, M.; Uphues, Th.; Schultze, M.
  • Nature, Vol. 446, Issue 7136
  • DOI: 10.1038/nature05648

Imaging ultrafast molecular dynamics with laser-induced electron diffraction
journal, March 2012

  • Blaga, Cosmin I.; Xu, Junliang; DiChiara, Anthony D.
  • Nature, Vol. 483, Issue 7388
  • DOI: 10.1038/nature10820

Resolving the time when an electron exits a tunnelling barrier
journal, May 2012

  • Shafir, Dror; Soifer, Hadas; Bruner, Barry D.
  • Nature, Vol. 485, Issue 7398
  • DOI: 10.1038/nature11025

Signatures of the continuum electron phase in molecular strong-field photoelectron holography
journal, July 2014

  • Meckel, M.; Staudte, A.; Patchkovskii, S.
  • Nature Physics, Vol. 10, Issue 8
  • DOI: 10.1038/nphys3010

Attosecond tunnelling interferometry
journal, August 2015

  • Pedatzur, O.; Orenstein, G.; Serbinenko, V.
  • Nature Physics, Vol. 11, Issue 10
  • DOI: 10.1038/nphys3436

Attosecond science
journal, June 2007

  • Corkum, P. B.; Krausz, Ferenc
  • Nature Physics, Vol. 3, Issue 6
  • DOI: 10.1038/nphys620

Glory scattering in deeply inelastic molecular collisions
journal, March 2022


Toward real-time charged-particle image reconstruction using polar onion-peeling
journal, May 2009

  • Roberts, G. M.; Nixon, J. L.; Lecointre, J.
  • Review of Scientific Instruments, Vol. 80, Issue 5
  • DOI: 10.1063/1.3126527

Anatomy of strong field ionization
journal, January 2005


Strong field approximation for systems with Coulomb interaction
journal, September 2008


Studying the universality of field induced tunnel ionization times via high-order harmonic spectroscopy
journal, October 2014

  • Soifer, H.; Bruner, B. D.; Negro, M.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 47, Issue 20
  • DOI: 10.1088/0953-4075/47/20/204029

Attosecond Probe of Valence-Electron Wave Packets by Subcycle Sculpted Laser Fields
journal, May 2012


Direct Visualization of Laser-Driven Electron Multiple Scattering and Tunneling Distance in Strong-Field Ionization
journal, August 2012


Plasma perspective on strong field multiphoton ionization
journal, September 1993


Precision Measurement of Strong Field Double Ionization of Helium
journal, August 1994


Phase Dependence of Intense Field Ionization: A Study Using Two Colors
journal, September 1994

  • Schumacher, D. W.; Weihe, F.; Muller, H. G.
  • Physical Review Letters, Vol. 73, Issue 10, p. 1344-1347
  • DOI: 10.1103/physrevlett.73.1344

Laser-Induced Electron Tunneling and Diffraction
journal, June 2008


Attosecond Ionization and Tunneling Delay Time Measurements in Helium
journal, December 2008


Time-Resolved Holography with Photoelectrons
journal, December 2010


Two-Color Strong-Field Photoelectron Spectroscopy and the Phase of the Phase
text, January 2015


Works referencing / citing this record:

Spatiotemporal imaging of valence electron motion
journal, March 2019


Asymmetry of molecular frame photoelectron angular distributions in ${{\rm{H}}}_{2}^{+}$ by intense two-color attosecond pulses: coherent excitation and charge migration effects
journal, February 2020

  • Yuan, Kai-Jun; Bandrauk, André D.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 53, Issue 6
  • DOI: 10.1088/1361-6455/ab5bac

It is all about phases: ultrafast holographic photoelectron imaging
journal, January 2020

  • Figueira de Morisson Faria, C.; Maxwell, A. S.
  • Reports on Progress in Physics, Vol. 83, Issue 3
  • DOI: 10.1088/1361-6633/ab5c91

Strong-field ionization of Ar atoms with a 45 cross-linearly-polarized two-color laser field
journal, July 2019


Holographic interference in atomic photoionization from a semiclassical standpoint
journal, August 2019


Angular distribution of photoelectron momentum in above-threshold ionization by circularly polarized laser pulses
journal, January 2020


Dynamic quantum state holography
journal, January 2020


Two-color phase-of-the-phase spectroscopy with circularly polarized laser pulses
journal, November 2018


R -matrix-with-time-dependence theory for ultrafast atomic processes in arbitrary light fields
journal, November 2018


Attoclock with counter-rotating bicircular laser fields
journal, March 2019


Coherent quantum enhancement of pair production in the null domain
journal, January 2020


Determination of the Ionization Time Using Attosecond Photoelectron Interferometry
journal, December 2018


Photoelectron Holographic Interferometry to Probe the Longitudinal Momentum Offset at the Tunnel Exit
journal, May 2019


Attosecond-Scale Streaking Methods for Strong-Field Ionization by Tailored Fields
journal, January 2020


$R$-matrix with Time-dependence Theory for Ultrafast Atomic Processes in Arbitrary Light Fields
text, January 2018


Spatiotemporal imaging of valence electron motion
text, January 2019


Deep Learning for Feynman’s Path Integral in Strong-Field Time-Dependent Dynamics
journal, March 2020


Spatiotemporal imaging of valence electron motion
text, January 2019