Collapse of superconductivity in cuprates via ultrafast quenching of phase coherence
Abstract
The possibility of driving phase transitions in low-density condensates through the loss of phase coherence alone has far-reaching implications for the study of quantum phases of matter. This has inspired the development of tools to control and explore the collective properties of condensate phases via phase fluctuations. Electrically gated oxide interfaces, ultracold Fermi atoms and cuprate superconductors, which are characterized by an intrinsically small phase stiffness, are paradigmatic examples where these tools are having a dramatic impact. In this study, we use light pulses shorter than the internal thermalization time to drive and probe the phase fragility of the Bi2Sr2CaCu2O8+δ cuprate superconductor, completely melting the superconducting condensate without affecting the pairing strength. The resulting ultrafast dynamics of phase fluctuations and charge excitations are captured and disentangled by time-resolved photoemission spectroscopy. This work demonstrates the dominant role of phase coherence in the superconductor-to-normal state phase transition and offers a benchmark for non-equilibrium spectroscopic investigations of the cuprate phase diagram.
- Authors:
-
- Univ. of British Columbia, Vancouver, BC (Canada). Dept. of Physics and Astronomy and Quantum Matter Inst.
- Univ. of British Columbia, Vancouver, BC (Canada). Dept. of Physics and Astronomy and Quantum Matter Inst.; Max Planck Inst. for Solid State Research, Stuttgart (Germany); Univ. of California, Davis, CA (United States). Dept. of Physics
- Catholic Univ. of the Sacred Heart, Brescia (Italy). Dept. of Mathematics and Physics and Interdisciplinary Lab. for Advanced Materials Physics (ILAMP)
- Univ. of British Columbia, Vancouver, BC (Canada). Dept. of Physics and Astronomy and Quantum Matter Inst.; Max Planck Inst. for Chemical Physics of Solids, Dresden (Germany)
- Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.
- Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.; Stony Brook Univ., NY (United States). Dept. of Physics and Astronomy
- Publication Date:
- Research Org.:
- Energy Frontier Research Centers (EFRC) (United States). Center for Emergent Superconductivity (CES); Brookhaven National Laboratory (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Science & Engineering Division; Ministry of Education, Universities and Research (MIUR); Catholic Univ. of the Sacred Heart, Brescia (Italy); Max Planck-UBC-UTokyo Centre for Quantum Materials (CQM); Canada First Research Excellence Fund; Gordon and Betty Moore Foundation; Killam Fellowships Program; Alfred P. Sloan Foundation; Natural Sciences and Engineering Research Council of Canada (NSERC); Alexander von Humboldt Foundation; Canada Research Chairs Program; Canada Foundation for Innovation (CFI); Canadian Inst. for Advanced Research (CIFAR); Swiss National Science Foundation (SNSF)
- OSTI Identifier:
- 1440896
- Report Number(s):
- BNL-205749-2018-JAAM
Journal ID: ISSN 1476-1122
- Grant/Contract Number:
- SC0012704; AC02-98CH10886; Prot. 2015C5SEJJ001; D.1; D.2.2; D.3.1; GBMF4779; P300P2-164649
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Materials
- Additional Journal Information:
- Journal Volume: 17; Journal Issue: 5; Journal ID: ISSN 1476-1122
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Boschini, F., da Silva Neto, E. H., Razzoli, E., Zonno, M., Peli, S., Day, R. P., Michiardi, M., Schneider, M., Zwartsenberg, B., Nigge, P., Zhong, R. D., Schneeloch, J., Gu, G. D., Zhdanovich, S., Mills, A. K., Levy, G., Jones, D. J., Giannetti, C., and Damascelli, A. Collapse of superconductivity in cuprates via ultrafast quenching of phase coherence. United States: N. p., 2018.
Web. doi:10.1038/s41563-018-0045-1.
Boschini, F., da Silva Neto, E. H., Razzoli, E., Zonno, M., Peli, S., Day, R. P., Michiardi, M., Schneider, M., Zwartsenberg, B., Nigge, P., Zhong, R. D., Schneeloch, J., Gu, G. D., Zhdanovich, S., Mills, A. K., Levy, G., Jones, D. J., Giannetti, C., & Damascelli, A. Collapse of superconductivity in cuprates via ultrafast quenching of phase coherence. United States. https://doi.org/10.1038/s41563-018-0045-1
Boschini, F., da Silva Neto, E. H., Razzoli, E., Zonno, M., Peli, S., Day, R. P., Michiardi, M., Schneider, M., Zwartsenberg, B., Nigge, P., Zhong, R. D., Schneeloch, J., Gu, G. D., Zhdanovich, S., Mills, A. K., Levy, G., Jones, D. J., Giannetti, C., and Damascelli, A. Mon .
"Collapse of superconductivity in cuprates via ultrafast quenching of phase coherence". United States. https://doi.org/10.1038/s41563-018-0045-1. https://www.osti.gov/servlets/purl/1440896.
@article{osti_1440896,
title = {Collapse of superconductivity in cuprates via ultrafast quenching of phase coherence},
author = {Boschini, F. and da Silva Neto, E. H. and Razzoli, E. and Zonno, M. and Peli, S. and Day, R. P. and Michiardi, M. and Schneider, M. and Zwartsenberg, B. and Nigge, P. and Zhong, R. D. and Schneeloch, J. and Gu, G. D. and Zhdanovich, S. and Mills, A. K. and Levy, G. and Jones, D. J. and Giannetti, C. and Damascelli, A.},
abstractNote = {The possibility of driving phase transitions in low-density condensates through the loss of phase coherence alone has far-reaching implications for the study of quantum phases of matter. This has inspired the development of tools to control and explore the collective properties of condensate phases via phase fluctuations. Electrically gated oxide interfaces, ultracold Fermi atoms and cuprate superconductors, which are characterized by an intrinsically small phase stiffness, are paradigmatic examples where these tools are having a dramatic impact. In this study, we use light pulses shorter than the internal thermalization time to drive and probe the phase fragility of the Bi2Sr2CaCu2O8+δ cuprate superconductor, completely melting the superconducting condensate without affecting the pairing strength. The resulting ultrafast dynamics of phase fluctuations and charge excitations are captured and disentangled by time-resolved photoemission spectroscopy. This work demonstrates the dominant role of phase coherence in the superconductor-to-normal state phase transition and offers a benchmark for non-equilibrium spectroscopic investigations of the cuprate phase diagram.},
doi = {10.1038/s41563-018-0045-1},
journal = {Nature Materials},
number = 5,
volume = 17,
place = {United States},
year = {Mon Apr 02 00:00:00 EDT 2018},
month = {Mon Apr 02 00:00:00 EDT 2018}
}
Web of Science
Works referenced in this record:
Effect of phase fluctuations on the single-particle properties of underdoped cuprates
journal, March 1999
- Kwon, Hyok-Jon; Dorsey, Alan T.
- Physical Review B, Vol. 59, Issue 9
Mapping of the formation of the pairing gap in
journal, December 2008
- Gomes, Kenjiro K.; Pasupathy, Abhay N.; Pushp, Aakash
- Journal of Physics and Chemistry of Solids, Vol. 69, Issue 12
The rate of quasiparticle recombination probes the onset of coherence in cuprate superconductors
journal, April 2016
- Hinton, J. P.; Thewalt, E.; Alpichshev, Z.
- Scientific Reports, Vol. 6, Issue 1
Point nodes persisting far beyond Tc in Bi2212
journal, July 2015
- Kondo, Takeshi; Malaeb, W.; Ishida, Y.
- Nature Communications, Vol. 6, Issue 1
Ultrafast Electron Relaxation in Superconducting by Time-Resolved Photoelectron Spectroscopy
journal, November 2007
- Perfetti, L.; Loukakos, P. A.; Lisowski, M.
- Physical Review Letters, Vol. 99, Issue 19
Energy dissipation from a correlated system driven out of equilibrium
journal, December 2016
- Rameau, J. D.; Freutel, S.; Kemper, A. F.
- Nature Communications, Vol. 7, Issue 1
Observation of pseudogap behaviour in a strongly interacting Fermi gas
journal, July 2010
- Gaebler, J. P.; Stewart, J. T.; Drake, T. E.
- Nature Physics, Vol. 6, Issue 8
Coherent Quasiparticle Weight and Its Connection to High- Superconductivity from Angle-Resolved Photoemission
journal, November 2001
- Ding, H.; Engelbrecht, J. R.; Wang, Z.
- Physical Review Letters, Vol. 87, Issue 22
Tracking Cooper Pairs in a Cuprate Superconductor by Ultrafast Angle-Resolved Photoemission
journal, May 2012
- Smallwood, C. L.; Hinton, J. P.; Jozwiak, C.
- Science, Vol. 336, Issue 6085
Phase fluctuations, dissipation, and superfluid stiffness in d -wave superconductors
journal, April 2001
- Benfatto, L.; Caprara, S.; Castellani, C.
- Physical Review B, Vol. 63, Issue 17
Dynamics of Cooper pair formation in
journal, August 2005
- Kaindl, Robert A.; Carnahan, Marc A.; Chemla, Daniel S.
- Physical Review B, Vol. 72, Issue 6
An ARPES view on the high-T c problem: Phonons vs. spin-fluctuations
journal, October 2010
- Kordyuk, A. A.; Zabolotnyy, V. B.; Evtushinsky, D. V.
- The European Physical Journal Special Topics, Vol. 188, Issue 1
Stimulated emission of Cooper pairs in a high-temperature cuprate superconductor
journal, July 2016
- Zhang, Wentao; Miller, Tristan; Smallwood, Christopher L.
- Scientific Reports, Vol. 6, Issue 1
Vanishing of phase coherence in underdoped Bi2Sr2CaCu2O8+δ
journal, March 1999
- Corson, J.; Mallozzi, R.; Orenstein, J.
- Nature, Vol. 398, Issue 6724
Controlled Vaporization of the Superconducting Condensate in Cuprate Superconductors by Femtosecond Photoexcitation
journal, November 2008
- Kusar, P.; Kabanov, V. V.; Demsar, J.
- Physical Review Letters, Vol. 101, Issue 22
Separating pairing from quantum phase coherence dynamics above the superconducting transition by femtosecond spectroscopy
journal, July 2014
- Madan, I.; Kurosawa, T.; Toda, Y.
- Scientific Reports, Vol. 4, Issue 1
Nodal quasiparticle meltdown in ultrahigh-resolution pump–probe angle-resolved photoemission
journal, July 2011
- Graf, J.; Jozwiak, C.; Smallwood, C. L.
- Nature Physics, Vol. 7, Issue 10
Diamagnetism and Cooper pairing above in cuprates
journal, February 2010
- Li, Lu; Wang, Yayu; Komiya, Seiki
- Physical Review B, Vol. 81, Issue 5
Onset of the vortexlike Nernst signal above in and
journal, November 2001
- Wang, Yayu; Xu, Z. A.; Kakeshita, T.
- Physical Review B, Vol. 64, Issue 22
Review of the Theoretical Description of Time-Resolved Angle-Resolved Photoemission Spectroscopy in Electron-Phonon Mediated Superconductors: Review of the theoretical description of time-resolved angle-resolved photoemission spectroscopy ⋅⋅⋅
journal, July 2017
- Kemper, A. F.; Sentef, M. A.; Moritz, B.
- Annalen der Physik, Vol. 529, Issue 9
BCS-Like Bogoliubov Quasiparticles in High- Superconductors Observed by Angle-Resolved Photoemission Spectroscopy
journal, May 2003
- Matsui, H.; Sato, T.; Takahashi, T.
- Physical Review Letters, Vol. 90, Issue 21
Clocking the onset of bilayer coherence in a high- cuprate
journal, January 2017
- Baldini, Edoardo; Mann, Andreas; Mallett, Benjamin P. P.
- Physical Review B, Vol. 95, Issue 2
Electric field control of the LaAlO3/SrTiO3 interface ground state
journal, December 2008
- Caviglia, A. D.; Gariglio, S.; Reyren, N.
- Nature, Vol. 456, Issue 7222
Signatures of superconductivity and pseudogap formation in nonequilibrium nodal quasiparticles revealed by ultrafast angle-resolved photoemission
journal, December 2013
- Zhang, Wentao; Smallwood, Christopher L.; Jozwiak, Chris
- Physical Review B, Vol. 88, Issue 24
Destruction of the Fermi surface in underdoped high-Tc superconductors
journal, March 1998
- Norman, M. R.; Ding, H.; Randeria, M.
- Nature, Vol. 392, Issue 6672
Photoinduced filling of near-nodal gap in
journal, August 2017
- Zhang, Z.; Piovera, C.; Papalazarou, E.
- Physical Review B, Vol. 96, Issue 6
Emergent phenomena at oxide interfaces
journal, January 2012
- Hwang, H. Y.; Iwasa, Y.; Kawasaki, M.
- Nature Materials, Vol. 11, Issue 2
Ultrafast Dynamics of Fluctuations in High-Temperature Superconductors Far from Equilibrium
journal, February 2015
- Perfetti, L.; Sciolla, B.; Biroli, G.
- Physical Review Letters, Vol. 114, Issue 6
Coherence Factors in a High-Tc Cuprate Probed by Quasi-Particle Scattering Off Vortices
journal, February 2009
- Hanaguri, T.; Kohsaka, Y.; Ono, M.
- Science, Vol. 323, Issue 5916
Phenomenology of the low-energy spectral function in high- superconductors
journal, May 1998
- Norman, M. R.; Randeria, M.; Ding, H.
- Physical Review B, Vol. 57, Issue 18
Ultrafast optical spectroscopy of strongly correlated materials and high-temperature superconductors: a non-equilibrium approach
journal, March 2016
- Giannetti, Claudio; Capone, Massimo; Fausti, Daniele
- Advances in Physics, Vol. 65, Issue 2
Angle-resolved photoemission spectroscopy study of the superconducting gap anisotropy in
journal, October 1996
- Ding, H.; Norman, M. R.; Campuzano, J. C.
- Physical Review B, Vol. 54, Issue 14
Energy gaps in high-transition-temperature cuprate superconductors
journal, June 2014
- Hashimoto, Makoto; Vishik, Inna M.; He, Rui-Hua
- Nature Physics, Vol. 10, Issue 7
Signature of Superfluid Density in the Single-Particle Excitation Spectrum of Bi2Sr2CaCu2O8+delta
journal, July 2000
- Feng, D. L.
- Science, Vol. 289, Issue 5477
The origin and non-quasiparticle nature of Fermi arcs in Bi2Sr2CaCu2O8+δ
journal, July 2012
- Reber, T. J.; Plumb, N. C.; Sun, Z.
- Nature Physics, Vol. 8, Issue 8
Discontinuity of the ultrafast electronic response of underdoped superconducting strongly excited by ultrashort light pulses
journal, June 2009
- Giannetti, Claudio; Coslovich, Giacomo; Cilento, Federico
- Physical Review B, Vol. 79, Issue 22
Quasi-particles ultrafastly releasing kink bosons to form Fermi arcs in a cuprate superconductor
journal, January 2016
- Ishida, Y.; Saitoh, T.; Mochiku, T.
- Scientific Reports, Vol. 6, Issue 1
Snapshots of the retarded interaction of charge carriers with ultrafast fluctuations in cuprates
journal, March 2015
- Dal Conte, S.; Vidmar, L.; Golež, D.
- Nature Physics, Vol. 11, Issue 5
Nonequilibrium superconductivity and quasiparticle dynamics in
journal, March 2001
- Averitt, R. D.; Rodriguez, G.; Lobad, A. I.
- Physical Review B, Vol. 63, Issue 14
Gapless pairing and the Fermi arc in the cuprates
journal, November 2007
- Chubukov, A. V.; Norman, M. R.; Millis, A. J.
- Physical Review B, Vol. 76, Issue 18
Phase fluctuations and spectral properties of underdoped cuprates
journal, December 1998
- Franz, M.; Millis, A. J.
- Physical Review B, Vol. 58, Issue 21
Time- and momentum-resolved gap dynamics in
journal, March 2014
- Smallwood, Christopher L.; Zhang, Wentao; Miller, Tristan L.
- Physical Review B, Vol. 89, Issue 11
Importance of phase fluctuations in superconductors with small superfluid density
journal, March 1995
- Emery, V. J.; Kivelson, S. A.
- Nature, Vol. 374, Issue 6521
Angle-resolved photoemission studies of the cuprate superconductors
journal, April 2003
- Damascelli, Andrea; Hussain, Zahid; Shen, Zhi-Xun
- Reviews of Modern Physics, Vol. 75, Issue 2
Emergence of preformed Cooper pairs from the doped Mott insulating state in Bi2Sr2CaCu2O8+δ
journal, November 2008
- Yang, H. -B.; Rameau, J. D.; Johnson, P. D.
- Nature, Vol. 456, Issue 7218
Material and Doping Dependence of the Nodal and Antinodal Dispersion Renormalizations in Single- and Multilayer Cuprates
journal, January 2010
- Johnston, S.; Lee, W. S.; Chen, Y.
- Advances in Condensed Matter Physics, Vol. 2010
An ARPES view on the high-Tc problem: phonons vs spin-fluctuations
text, January 2010
- Kordyuk, A. A.; Zabolotnyy, V. B.; Evtushinsky, D. V.
- arXiv
Tracking Cooper Pairs in a Cuprate Superconductor by Ultrafast Angle-Resolved Photoemission
text, January 2012
- Smallwood, Christopher L.; Hinton, James P.; Jozwiak, Christopher
- arXiv
Ultrafast dynamics of fluctuations in high-temperature superconductors far from equilibrium
text, January 2014
- Perfetti, L.; Sciolla, B.; Biroli, G.
- arXiv
Snapshots of the retarded interaction of charge carriers with ultrafast fluctuations in cuprates
text, January 2015
- Conte, S. Dal; Vidmar, L.; Golež, D.
- arXiv
Quasi-particles ultrafastly releasing kink bosons to form Fermi arcs in a cuprate superconductor
text, January 2015
- Ishida, Y.; Saitoh, T.; Mochiku, T.
- arXiv
Coherent quasiparticle weight and its connection to high-T_c superconductivity from angle-resolved photoemission
text, January 2000
- Ding, H.; Engelbrecht, J. R.; Wang, Z.
- arXiv
Signature of Superfluid Density in the Single-Particle Excitation Spectrum of Bi2Sr2CaCu2O8+delta
text, January 2000
- Feng, D. L.; Lu, D. H.; Shen, K. M.
- arXiv
BCS-like Bogoliubov Quasiparticles in High-Tc Superconductors Observed by Angle-Resolved Photoemission Spectroscopy
text, January 2003
- Matsui, H.; Sato, T.; Takahashi, T.
- arXiv
Destruction of the Fermi Surface in Underdoped High Tc Superconductors
text, January 1997
- Norman, M. R.; Ding, H.; Randeria, M.
- arXiv
Phase Fluctuations and Spectral Properties of Underdoped Cuprates
text, January 1998
- Franz, M.; Millis, A. J.
- arXiv
Energy dissipation from a correlated system driven out of equilibrium
journal, December 2016
- Rameau, J. D.; Freutel, S.; Kemper, A. F.
- Nature Communications, Vol. 7, Issue 1
Snapshots of the retarded interaction of charge carriers with ultrafast fluctuations in cuprates
journal, March 2015
- Dal Conte, S.; Vidmar, L.; Golež, D.
- Nature Physics, Vol. 11, Issue 5
Material and Doping Dependence of the Nodal and Antinodal Dispersion Renormalizations in Single- and Multilayer Cuprates
journal, January 2010
- Johnston, S.; Lee, W. S.; Chen, Y.
- Advances in Condensed Matter Physics, Vol. 2010
Gapless superconductivity and the Fermi arc in the cuprates
text, January 2007
- Chubukov, A. V.; Norman, M. R.; Millis, A. J.
- arXiv
Electric Field Control of the LaAlO$_{3}$/SrTiO$_{3}$ Interface Ground State
text, January 2008
- Caviglia, A. D.; Gariglio, S.; Reyren, N.
- arXiv
Works referencing / citing this record:
Emergence of pseudogap from short-range spin-correlations in electron-doped cuprates
journal, January 2020
- Boschini, Fabio; Zonno, Marta; Razzoli, Elia
- npj Quantum Materials, Vol. 5, Issue 1
Angle-resolved photoemission spectroscopy and its application to topological materials
journal, August 2019
- Lv, Baiqing; Qian, Tian; Ding, Hong
- Nature Reviews Physics, Vol. 1, Issue 10
A tunable time-resolved spontaneous Raman spectroscopy setup for probing ultrafast collective excitation and quasiparticle dynamics in quantum materials
journal, July 2018
- Versteeg, R. B.; Zhu, J.; Padmanabhan, P.
- Structural Dynamics, Vol. 5, Issue 4
Cavity-enhanced high harmonic generation for extreme ultraviolet time- and angle-resolved photoemission spectroscopy
journal, August 2019
- Mills, A. K.; Zhdanovich, S.; Na, M. X.
- Review of Scientific Instruments, Vol. 90, Issue 8
Superfluid stiffness in cuprates: Effect of Mott transition and phase competition
journal, September 2019
- Simard, O.; Hébert, C. -D.; Foley, A.
- Physical Review B, Vol. 100, Issue 9
Excitonic and lattice contributions to the charge density wave in revealed by a phonon bottleneck
journal, September 2019
- Hedayat, H.; Sayers, C. J.; Bugini, D.
- Physical Review Research, Vol. 1, Issue 2
Ultrafast electron calorimetry uncovers a new long-lived metastable state in 1 T -TaSe 2 mediated by mode-selective electron-phonon coupling
journal, March 2019
- Shi, Xun; You, Wenjing; Zhang, Yingchao
- Science Advances, Vol. 5, Issue 3
Direct determination of mode-projected electron-phonon coupling in the time domain
journal, December 2019
- Na, M. X.; Mills, A. K.; Boschini, F.
- Science, Vol. 366, Issue 6470
Emergence of pseudogap from short-range spin-correlations in electron doped cuprates
text, January 2018
- Boschini, F.; Zonno, M.; Razzoli, E.
- arXiv
Ultrafast electron calorimetry uncovers a new long-lived metastable state in 1T-TaSe$_2$ mediated by mode-selective electron-phonon coupling
text, January 2019
- Shi, Xun; You, Wenjing; Zhang, Yingchao
- arXiv
Direct determination of mode-projected electron-phonon coupling in the time-domain
text, January 2019
- Na, MengXing; Mills, Arthur K.; Boschini, Fabio
- arXiv
Angle-resolved photoemission spectroscopy and its application to topological materials
text, January 2021
- Lv, Baiqing; Qian, Tian; Ding, Hong
- arXiv
Ultrafast electron calorimetry uncovers a new long-lived metastable state in 1T-TaSe$_2$ mediated by mode-selective electron-phonon coupling
text, January 2019
- Shi, Xun; You, Wenjing; Zhang, Yingchao
- arXiv