Large resistance change on magnetic tunnel junction based molecular spintronics devices

Tyagi, Pawan; Friebe, Edward

doi:10.1016/j.jmmm.2018.01.024

Title: Large resistance change on magnetic tunnel junction based molecular spintronics devices

Abstract

Here, molecular bridges covalently bonded to two ferromagnetic electrodes can transform ferromagnetic materials and produce intriguing spin transport characteristics. This paper discusses the impact of molecule induced strong coupling on the spin transport. To study molecular coupling effect the octametallic molecular cluster (OMC) was bridged between two ferromagnetic electrodes of a magnetic tunnel junction (Ta/Co/NiFe/AlOx/NiFe/Ta) along the exposed side edges. OMCs induced strong inter-ferromagnetic electrode coupling to yield drastic changes in transport properties of the magnetic tunnel junction testbed at the room temperature. These OMCs also transformed the magnetic properties of magnetic tunnel junctions. SQUID and ferromagnetic resonance studies provided insightful data to explain transport studies on the magnetic tunnel junction based molecular spintronics devices.

Authors:

^[1]; Friebe, Edward ^[2]

Univ. of the District of Columbia, Washington, D.C. (United States); Univ. of Kentucky, Lexington, KY (United States)
Univ. of the District of Columbia, Washington, D.C. (United States)

Publication Date:: Fri Jan 12 00:00:00 EST 2018

Research Org.:: Univ. of the District of Columbia, Washington, D.C. (United States)

Sponsoring Org.:: USDOE National Nuclear Security Administration (NNSA), Office of Defense Nuclear Nonproliferation

OSTI Identifier:: 1439170

Grant/Contract Number:: NA0002687

Resource Type:: Accepted Manuscript

Journal Name:: Journal of Magnetism and Magnetic Materials

Additional Journal Information:: Journal Volume: 453; Journal Issue: C; Journal ID: ISSN 0304-8853

Publisher:: Elsevier

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; Molecular spintronics; Magnetic tunnel junctions; Magnetic molecules

Citation Formats


                    Tyagi, Pawan, and Friebe, Edward. Large resistance change on magnetic tunnel junction based molecular spintronics devices.  United States: N. p., 2018. 
Web.  doi:10.1016/j.jmmm.2018.01.024.

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                    Tyagi, Pawan, & Friebe, Edward. Large resistance change on magnetic tunnel junction based molecular spintronics devices.  United States.  https://doi.org/10.1016/j.jmmm.2018.01.024

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                    Tyagi, Pawan, and Friebe, Edward. Fri .  
"Large resistance change on magnetic tunnel junction based molecular spintronics devices".  United States.  https://doi.org/10.1016/j.jmmm.2018.01.024.  https://www.osti.gov/servlets/purl/1439170.

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@article{osti_1439170,

  title        = {Large resistance change on magnetic tunnel junction based molecular spintronics devices},

  author       = {Tyagi, Pawan and Friebe, Edward},

  abstractNote = {Here, molecular bridges covalently bonded to two ferromagnetic electrodes can transform ferromagnetic materials and produce intriguing spin transport characteristics. This paper discusses the impact of molecule induced strong coupling on the spin transport. To study molecular coupling effect the octametallic molecular cluster (OMC) was bridged between two ferromagnetic electrodes of a magnetic tunnel junction (Ta/Co/NiFe/AlOx/NiFe/Ta) along the exposed side edges. OMCs induced strong inter-ferromagnetic electrode coupling to yield drastic changes in transport properties of the magnetic tunnel junction testbed at the room temperature. These OMCs also transformed the magnetic properties of magnetic tunnel junctions. SQUID and ferromagnetic resonance studies provided insightful data to explain transport studies on the magnetic tunnel junction based molecular spintronics devices.},

  doi          = {10.1016/j.jmmm.2018.01.024},

  journal      = {Journal of Magnetism and Magnetic Materials},

  number       = C,

  volume       = 453,

  place        = {United States},

  year         = {Fri Jan 12 00:00:00 EST 2018},

  month        = {Fri Jan 12 00:00:00 EST 2018}

}

Copy to clipboard

Journal Article:

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https://doi.org/10.1016/j.jmmm.2018.01.024

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Cited by: 22 works

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Figures / Tables:

Fig. 1: MTJMSD fabrication steps: (a) deposit the bottom ferromagnetic (bottom-FM) electrode on the insulating substrate, (b) creates photoresist (PR) cavity pattern for the depostion of (c) ~2nm AlOx and (d) top ferromagnetic electrode (top-FM). (e) Liftoff step produces and MTJ with the exposed sides where (f) OMC molecules aremore »

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Works referencing / citing this record:

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Figures / Tables found in this record:

Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.

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Title: Large resistance change on magnetic tunnel junction based molecular spintronics devices

Abstract

Citation Formats

Figures / Tables:

Molecular spintronics using single-molecule magnets journal, March 2008

The Kondo Effect in the Presence of Ferromagnetism journal, October 2004

Spin-Dependent Transport in Molecular Tunnel Junctions journal, September 2004

Vibration-Assisted Electron Tunneling in C 140 Transistors journal, February 2005

Multilayer edge molecular electronics devices: a review journal, January 2011

Electron Transport through Single Mn 12 Molecular Magnets journal, May 2006

Paramagnetic molecule induced strong antiferromagnetic exchange coupling on a magnetic tunnel junction based molecular spintronics device journal, July 2015

Thioester-functionalised and oxime-based hexametallic manganese( iii ) single-molecule magnets journal, January 2017

Porphyrins as molecular electronic components of functional devices journal, October 2010

DNA spintronics journal, July 2002

An S = 6 Cyanide-Bridged Octanuclear Fe III 4 Ni II 4 Complex that Exhibits Slow Relaxation of the Magnetization journal, April 2006

Molecular Electrodes at the Exposed Edge of Metal/Insulator/Metal Trilayer Structures journal, April 2007

Fabrication of tunnel junction-based molecular electronics and spintronics devices journal, September 2012

Addressing the challenges of using ferromagnetic electrodes in the magnetic tunnel junction-based molecular spintronics devices journal, November 2015

C60/NiFe combination as a promising platform for molecular spintronics journal, March 2012

Permanent Magnetism, Magnetic Anisotropy, and Hysteresis of Thiol-Capped Gold Nanoparticles journal, August 2004

1-Dodecanethiol Self-Assembled Monolayers on Cobalt journal, December 2011

Activating the molecular spinterface journal, April 2017

Tunneling path toward spintronics journal, February 2011

Ferromagnetic resonance in coupled ultrathin films journal, February 2003

Ferromagnetic resonance in a coupled two-layer system journal, November 1990

Tunneling Conductance of Asymmetrical Barriers journal, April 1970

Making electrical contacts to molecular monolayers journal, October 2001

Interlayer exchange coupling and magnetic anisotropy in prototype trilayers: Ab initio theory versus experiment journal, September 2003

Why are spin wave excitations all important in nanoscale magnetism? journal, January 2008

Giant tunnel magnetoresistance in magnetic tunnel junctions with a crystalline MgO(0 0 1) barrier journal, October 2007

Spin-Polarized Current in Spin Valves and Magnetic Tunnel Junctions journal, May 2006

FeCoCp 3 Molecular Magnets as Spin Filters journal, May 2015

Ancillary Ligand Functionalization of Cyanide-Bridged S = 6 Fe III 4 Ni II 4 Complexes for Molecule-Based Electronics journal, September 2006

Change of cobalt magnetic anisotropy and spin polarization with alkanethiolates self-assembled monolayers journal, June 2015

The Rise of Single-Ion Magnets as Spin Qubits journal, November 2016

Quantum computing in molecular magnets journal, April 2001

Molecular spintronics and quantum computing journal, January 2009

Single molecule magnets for quantum computation journal, May 2007

Molecular magnetism, quo vadis? A historical perspective from a coordination chemist viewpoint☆ journal, May 2017

Molecular spintronics devices exhibiting properties of a solar cell journal, September 2019

Molecular spintronics using single-molecule magnets
journal, March 2008

The Kondo Effect in the Presence of Ferromagnetism
journal, October 2004

Spin-Dependent Transport in Molecular Tunnel Junctions
journal, September 2004

Vibration-Assisted Electron Tunneling in C ₁₄₀ Transistors
journal, February 2005

Multilayer edge molecular electronics devices: a review
journal, January 2011

Electron Transport through Single ${Mn}_{12}$ Molecular Magnets
journal, May 2006

Paramagnetic molecule induced strong antiferromagnetic exchange coupling on a magnetic tunnel junction based molecular spintronics device
journal, July 2015

Thioester-functionalised and oxime-based hexametallic manganese( iii ) single-molecule magnets
journal, January 2017

Porphyrins as molecular electronic components of functional devices
journal, October 2010

DNA spintronics
journal, July 2002

An S = 6 Cyanide-Bridged Octanuclear Fe ^III ₄ Ni ^II ₄ Complex that Exhibits Slow Relaxation of the Magnetization
journal, April 2006

Molecular Electrodes at the Exposed Edge of Metal/Insulator/Metal Trilayer Structures
journal, April 2007

Fabrication of tunnel junction-based molecular electronics and spintronics devices
journal, September 2012

Addressing the challenges of using ferromagnetic electrodes in the magnetic tunnel junction-based molecular spintronics devices
journal, November 2015

C60/NiFe combination as a promising platform for molecular spintronics
journal, March 2012

Permanent Magnetism, Magnetic Anisotropy, and Hysteresis of Thiol-Capped Gold Nanoparticles
journal, August 2004

1-Dodecanethiol Self-Assembled Monolayers on Cobalt
journal, December 2011

Activating the molecular spinterface
journal, April 2017

Tunneling path toward spintronics
journal, February 2011

Ferromagnetic resonance in coupled ultrathin films
journal, February 2003

Ferromagnetic resonance in a coupled two-layer system
journal, November 1990

Tunneling Conductance of Asymmetrical Barriers
journal, April 1970

Making electrical contacts to molecular monolayers
journal, October 2001

Interlayer exchange coupling and magnetic anisotropy in prototype trilayers: Ab initio theory versus experiment
journal, September 2003

Why are spin wave excitations all important in nanoscale magnetism?
journal, January 2008

Giant tunnel magnetoresistance in magnetic tunnel junctions with a crystalline MgO(0 0 1) barrier
journal, October 2007

Spin-Polarized Current in Spin Valves and Magnetic Tunnel Junctions
journal, May 2006

FeCoCp ₃ Molecular Magnets as Spin Filters
journal, May 2015

Ancillary Ligand Functionalization of Cyanide-Bridged S = 6 Fe ^III ₄ Ni ^II ₄ Complexes for Molecule-Based Electronics
journal, September 2006

Change of cobalt magnetic anisotropy and spin polarization with alkanethiolates self-assembled monolayers
journal, June 2015

The Rise of Single-Ion Magnets as Spin Qubits
journal, November 2016

Quantum computing in molecular magnets
journal, April 2001

Molecular spintronics and quantum computing
journal, January 2009

Single molecule magnets for quantum computation
journal, May 2007

Molecular magnetism, quo vadis? A historical perspective from a coordination chemist viewpoint☆
journal, May 2017

Molecular spintronics devices exhibiting properties of a solar cell
journal, September 2019