Effective Detection of Mycotoxins by a Highly Luminescent Metal–Organic Framework
Abstract
In this paper, we designed and synthesized a new luminescent metal–organic framework (LMOF). LMOF-241 is highly porous and emits strong blue light with high efficiency. We demonstrate for the first time that very fast and extremely sensitive optical detection can be achieved, making use of the fluorescence quenching of an LMOF material. The compound is responsive to Aflatoxin B1 at parts per billion level, which makes it the best performing luminescence-based chemical sensor to date. We studied the electronic properties of LMOF-241 and selected mycotoxins, as well as the extent of mycotoxin–LMOF interactions, employing theoretical methods. Finally, possible electron and energy transfer mechanisms are discussed.
- Authors:
-
- Rutgers Univ., Piscataway, NJ (United States). Dept. of Chemistry and Chemical Biology
- Northern Illinois Univ., DeKalb, IL (United States). Dept. of Chemistry and Biochemistry
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1436589
- Grant/Contract Number:
- AC02-05CH11231; FG02-08ER46491
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of the American Chemical Society
- Additional Journal Information:
- Journal Volume: 137; Journal Issue: 51; Journal ID: ISSN 0002-7863
- Publisher:
- American Chemical Society (ACS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 59 BASIC BIOLOGICAL SCIENCES
Citation Formats
Hu, Zhichao, Lustig, William P., Zhang, Jingming, Zheng, Chong, Wang, Hao, Teat, Simon J., Gong, Qihan, Rudd, Nathan D., and Li, Jing. Effective Detection of Mycotoxins by a Highly Luminescent Metal–Organic Framework. United States: N. p., 2015.
Web. doi:10.1021/jacs.5b10308.
Hu, Zhichao, Lustig, William P., Zhang, Jingming, Zheng, Chong, Wang, Hao, Teat, Simon J., Gong, Qihan, Rudd, Nathan D., & Li, Jing. Effective Detection of Mycotoxins by a Highly Luminescent Metal–Organic Framework. United States. https://doi.org/10.1021/jacs.5b10308
Hu, Zhichao, Lustig, William P., Zhang, Jingming, Zheng, Chong, Wang, Hao, Teat, Simon J., Gong, Qihan, Rudd, Nathan D., and Li, Jing. Fri .
"Effective Detection of Mycotoxins by a Highly Luminescent Metal–Organic Framework". United States. https://doi.org/10.1021/jacs.5b10308. https://www.osti.gov/servlets/purl/1436589.
@article{osti_1436589,
title = {Effective Detection of Mycotoxins by a Highly Luminescent Metal–Organic Framework},
author = {Hu, Zhichao and Lustig, William P. and Zhang, Jingming and Zheng, Chong and Wang, Hao and Teat, Simon J. and Gong, Qihan and Rudd, Nathan D. and Li, Jing},
abstractNote = {In this paper, we designed and synthesized a new luminescent metal–organic framework (LMOF). LMOF-241 is highly porous and emits strong blue light with high efficiency. We demonstrate for the first time that very fast and extremely sensitive optical detection can be achieved, making use of the fluorescence quenching of an LMOF material. The compound is responsive to Aflatoxin B1 at parts per billion level, which makes it the best performing luminescence-based chemical sensor to date. We studied the electronic properties of LMOF-241 and selected mycotoxins, as well as the extent of mycotoxin–LMOF interactions, employing theoretical methods. Finally, possible electron and energy transfer mechanisms are discussed.},
doi = {10.1021/jacs.5b10308},
journal = {Journal of the American Chemical Society},
number = 51,
volume = 137,
place = {United States},
year = {Fri Dec 11 00:00:00 EST 2015},
month = {Fri Dec 11 00:00:00 EST 2015}
}
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What Electrochemical Biosensors Can Do for Forensic Science? Unique Features and Applications
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- Yáñez-Sedeño, Paloma; Agüí, Lourdes; Campuzano, Susana
- Biosensors, Vol. 9, Issue 4