Efficient hydrogen evolution by ternary molybdenum sulfoselenide particles on self-standing porous nickel diselenide foam
Abstract
With the massive consumption of fossil fuels and its detrimental impact on the environment, methods of generating clean power are urgent. Hydrogen is an ideal carrier for renewable energy; however, hydrogen generation is inefficient because of the lack of robust catalysts that are substantially cheaper than platinum. Therefore, robust and durable earth-abundant and cost-effective catalysts are desirable for hydrogen generation from water splitting via hydrogen evolution reaction. In this paper, we report an active and durable earth-abundant transition metal dichalcogenide-based hybrid catalyst that exhibits high hydrogen evolution activity approaching the state-of-the-art platinum catalysts, and superior to those of most transition metal dichalcogenides (molybdenum sulfide, cobalt diselenide and so on). Our material is fabricated by growing ternary molybdenum sulfoselenide particles on self-standing porous nickel diselenide foam. This advance provides a different pathway to design cheap, efficient and sizable hydrogen-evolving electrode by simultaneously tuning the number of catalytic edge sites, porosity, heteroatom doping and electrical conductivity.
- Authors:
-
- Univ. of Houston, Houston, TX (United States). Dept. of Physics and Texas Center for Superconductivity (TcSUH)
- California Inst. of Technology (CalTech), Pasadena, CA (United States). Materials and Process Simulation Center
- Univ. of Houston, Houston, TX (United States). Dept. of Electrical and Computer Engineering
- Publication Date:
- Research Org.:
- California Institute of Technology (CalTech), Pasadena, CA (United States); Univ. of Houston, TX (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC); Defense Threat Reduction Agency (DTRA); National Science Foundation (NSF); Welch Foundation, Houston, TX (United States)
- OSTI Identifier:
- 1435783
- Grant/Contract Number:
- SC0004993; FA 7000-13-1-0001; ECCS-1240510; E-1728
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 7; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 08 HYDROGEN; 36 MATERIALS SCIENCE; electrocatalysis; porous materials
Citation Formats
Zhou, Haiqing, Yu, Fang, Huang, Yufeng, Sun, Jingying, Zhu, Zhuan, Nielsen, Robert J., He, Ran, Bao, Jiming, Goddard III, William A., Chen, Shuo, and Ren, Zhifeng. Efficient hydrogen evolution by ternary molybdenum sulfoselenide particles on self-standing porous nickel diselenide foam. United States: N. p., 2016.
Web. doi:10.1038/ncomms12765.
Zhou, Haiqing, Yu, Fang, Huang, Yufeng, Sun, Jingying, Zhu, Zhuan, Nielsen, Robert J., He, Ran, Bao, Jiming, Goddard III, William A., Chen, Shuo, & Ren, Zhifeng. Efficient hydrogen evolution by ternary molybdenum sulfoselenide particles on self-standing porous nickel diselenide foam. United States. https://doi.org/10.1038/ncomms12765
Zhou, Haiqing, Yu, Fang, Huang, Yufeng, Sun, Jingying, Zhu, Zhuan, Nielsen, Robert J., He, Ran, Bao, Jiming, Goddard III, William A., Chen, Shuo, and Ren, Zhifeng. Fri .
"Efficient hydrogen evolution by ternary molybdenum sulfoselenide particles on self-standing porous nickel diselenide foam". United States. https://doi.org/10.1038/ncomms12765. https://www.osti.gov/servlets/purl/1435783.
@article{osti_1435783,
title = {Efficient hydrogen evolution by ternary molybdenum sulfoselenide particles on self-standing porous nickel diselenide foam},
author = {Zhou, Haiqing and Yu, Fang and Huang, Yufeng and Sun, Jingying and Zhu, Zhuan and Nielsen, Robert J. and He, Ran and Bao, Jiming and Goddard III, William A. and Chen, Shuo and Ren, Zhifeng},
abstractNote = {With the massive consumption of fossil fuels and its detrimental impact on the environment, methods of generating clean power are urgent. Hydrogen is an ideal carrier for renewable energy; however, hydrogen generation is inefficient because of the lack of robust catalysts that are substantially cheaper than platinum. Therefore, robust and durable earth-abundant and cost-effective catalysts are desirable for hydrogen generation from water splitting via hydrogen evolution reaction. In this paper, we report an active and durable earth-abundant transition metal dichalcogenide-based hybrid catalyst that exhibits high hydrogen evolution activity approaching the state-of-the-art platinum catalysts, and superior to those of most transition metal dichalcogenides (molybdenum sulfide, cobalt diselenide and so on). Our material is fabricated by growing ternary molybdenum sulfoselenide particles on self-standing porous nickel diselenide foam. This advance provides a different pathway to design cheap, efficient and sizable hydrogen-evolving electrode by simultaneously tuning the number of catalytic edge sites, porosity, heteroatom doping and electrical conductivity.},
doi = {10.1038/ncomms12765},
journal = {Nature Communications},
number = ,
volume = 7,
place = {United States},
year = {Fri Sep 16 00:00:00 EDT 2016},
month = {Fri Sep 16 00:00:00 EDT 2016}
}
Web of Science
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journal, January 2019
- Han, HyukSu; Choi, Heechae; Mhin, Sungwook
- Energy & Environmental Science, Vol. 12, Issue 8
N-Doped amorphous MoS x for the hydrogen evolution reaction
journal, January 2019
- Ding, Ruimin; Wang, Mengchao; Wang, Xianfen
- Nanoscale, Vol. 11, Issue 23
Recent advances in two-dimensional materials and their nanocomposites in sustainable energy conversion applications
journal, January 2019
- Khan, Karim; Tareen, Ayesha Khan; Aslam, Muhammad
- Nanoscale, Vol. 11, Issue 45
Neutral-pH overall water splitting catalyzed efficiently by a hollow and porous structured ternary nickel sulfoselenide electrocatalyst
journal, January 2019
- Zeng, Lingyou; Sun, Kaian; Chen, Yanju
- Journal of Materials Chemistry A, Vol. 7, Issue 28
The effect of carbon quantum dots on the electrocatalytic hydrogen evolution reaction of manganese–nickel phosphide nanosheets
journal, January 2019
- Chen, Weiwu; Qin, Zhaojun; McElhenny, Brian
- Journal of Materials Chemistry A, Vol. 7, Issue 37
Hydrogen evolution activity tuning via two-dimensional electron accumulation at buried interfaces
journal, January 2019
- Xue, Yudong; Fishman, Zachary S.; Wang, Yunting
- Journal of Materials Chemistry A, Vol. 7, Issue 36
Highly active catalyst derived from a 3D foam of Fe(PO 3 ) 2 /Ni 2 P for extremely efficient water oxidation
journal, May 2017
- Zhou, Haiqing; Yu, Fang; Sun, Jingying
- Proceedings of the National Academy of Sciences, Vol. 114, Issue 22
Synthesis of transition metal sulfide and reduced graphene oxide hybrids as efficient electrocatalysts for oxygen evolution reactions
journal, September 2018
- Hong, Yu-Rim; Mhin, Sungwook; Kwon, Jiseok
- Royal Society Open Science, Vol. 5, Issue 9
MoSe2-Ni3Se4 Hybrid Nanoelectrocatalysts and Their Enhanced Electrocatalytic Activity for Hydrogen Evolution Reaction
journal, June 2020
- Wu, Pengyuan; Sun, Gangyong; Chen, Yuanzhi
- Nanoscale Research Letters, Vol. 15, Issue 1
MoS2 Decorated Carbon Nanofibers as Efficient and Durable Electrocatalyst for Hydrogen Evolution Reaction
journal, October 2017
- Zhang, C.; Wang, Z.; Bhoyate, S.
- C, Vol. 3, Issue 4
Fabrication of Robust Hydrogen Evolution Reaction Electrocatalyst Using Ag2Se by Vacuum Evaporation
journal, October 2019
- Hussain, Sajjad; Chae, Jinwoong; Akbar, Kamran
- Nanomaterials, Vol. 9, Issue 10
Electronically Double‐Layered Metal Boride Hollow Nanoprism as an Excellent and Robust Water Oxidation Electrocatalysts
journal, February 2019
- Han, HyukSu; Hong, Yu‐Rim; Woo, Jungwook
- Advanced Energy Materials, Vol. 9, Issue 15
A structurally versatile nickel phosphite acting as a robust bifunctional electrocatalyst for overall water splitting
text, January 2018
- Menezes, Prashanth W.; Panda, Chakadola; Loos, Stefan
- Freie Universität Berlin
Helical cobalt borophosphates to master durable overall water-splitting
text, January 2019
- Menezes, Prashanth W.; Indra, Arindam; Zaharieva, Ivelina
- Freie Universität Berlin
Facile Synthesis of Molybdenum Diselenide Layers for High-Performance Hydrogen Evolution Electrocatalysts
journal, May 2018
- Vikraman, Dhanasekaran; Hussain, Sajjad; Akbar, Kamran
- ACS Omega, Vol. 3, Issue 5
Efficient hydrogen production on MoNi4 electrocatalysts with fast water dissociation kinetics
journal, May 2017
- Zhang, Jian; Wang, Tao; Liu, Pan
- Nature Communications, Vol. 8, Issue 1
High-performance bifunctional porous non-noble metal phosphide catalyst for overall water splitting
journal, June 2018
- Yu, Fang; Zhou, Haiqing; Huang, Yufeng
- Nature Communications, Vol. 9, Issue 1
Synthesis of transition metal sulfide and reduced graphene oxide hybrids as efficient electrocatalysts for oxygen evolution reactions
journal, September 2018
- Hong, Yu-Rim; Mhin, Sungwook; Kwon, Jiseok
- Royal Society Open Science, Vol. 5, Issue 9
Synthesis of Mo2C and W2C Nanoparticle Electrocatalysts for the Efficient Hydrogen Evolution Reaction in Alkali and Acid Electrolytes
journal, October 2019
- Hussain, Sajjad; Vikraman, Dhanasekaran; Feroze, Asad
- Frontiers in Chemistry, Vol. 7