DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Motion of W and He atoms during formation of W fuzz

Abstract

Measurements are conducted to identify the motion of tungsten and helium atoms during the formation of tungsten fuzz. In a first series of experiments the mobility of helium within the growing fuzz was measured by adding 3He to the different stages of plasma exposure under conditions that promoted tungsten fuzz growth. Ion beam analysis was used to quantify the amount of 3He remaining in the samples following the plasma exposure. The results indicate that the retention of helium in bubbles within tungsten is a dynamic process with direct implantation rather than diffusion into the bubbles, best describing the motion of the helium atoms. In the second experiment, an isotopically enriched layer of tungsten (~92.99% 182W) is deposited on the surface of a bulk tungsten sample with the natural abundance of the isotopes. This sample is then exposed to helium plasma at the conditions necessary to support the formation of tungsten 'fuzz'. Depth profiles of the concentration of each of the tungsten isotopes are obtained using secondary ion mass spectrometry (SIMS) before and after the plasma exposure. The depth profiles clearly show mixing of tungsten atoms from the bulk sample toward the surface of the fuzz. Lastly, this supports a physicalmore » picture of the dynamic behavior of helium bubbles which, also, causes an enhanced mixing of tungsten atoms.« less

Authors:
 [1];  [1];  [1];  [2];  [3]
  1. Univ. of California, San Diego, CA (United States). Center for Energy Research
  2. Max-Planck Inst. fur Plasmaphysik, Garching, (Germany)
  3. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Physics Division
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Nuclear Physics (NP); USDOE Office of Science (SC), Fusion Energy Sciences (FES); European Union (EU)
OSTI Identifier:
1435242
Grant/Contract Number:  
AC05-00OR22725; FG02-07ER54912; SC0018302
Resource Type:
Accepted Manuscript
Journal Name:
Nuclear Fusion
Additional Journal Information:
Journal Volume: 58; Journal Issue: 6; Journal ID: ISSN 0029-5515
Publisher:
IOP Science
Country of Publication:
United States
Language:
English
Subject:
70 PLASMA PHYSICS AND FUSION TECHNOLOGY; plasma-material interaction; tungsten fuzz; helium nano-bubbles

Citation Formats

Doerner, R. P., Nishijima, D., Krasheninnikov, S. I., Schwarz-Selinger, T., and Zach, M. Motion of W and He atoms during formation of W fuzz. United States: N. p., 2018. Web. doi:10.1088/1741-4326/aab96a.
Doerner, R. P., Nishijima, D., Krasheninnikov, S. I., Schwarz-Selinger, T., & Zach, M. Motion of W and He atoms during formation of W fuzz. United States. https://doi.org/10.1088/1741-4326/aab96a
Doerner, R. P., Nishijima, D., Krasheninnikov, S. I., Schwarz-Selinger, T., and Zach, M. Wed . "Motion of W and He atoms during formation of W fuzz". United States. https://doi.org/10.1088/1741-4326/aab96a. https://www.osti.gov/servlets/purl/1435242.
@article{osti_1435242,
title = {Motion of W and He atoms during formation of W fuzz},
author = {Doerner, R. P. and Nishijima, D. and Krasheninnikov, S. I. and Schwarz-Selinger, T. and Zach, M.},
abstractNote = {Measurements are conducted to identify the motion of tungsten and helium atoms during the formation of tungsten fuzz. In a first series of experiments the mobility of helium within the growing fuzz was measured by adding 3He to the different stages of plasma exposure under conditions that promoted tungsten fuzz growth. Ion beam analysis was used to quantify the amount of 3He remaining in the samples following the plasma exposure. The results indicate that the retention of helium in bubbles within tungsten is a dynamic process with direct implantation rather than diffusion into the bubbles, best describing the motion of the helium atoms. In the second experiment, an isotopically enriched layer of tungsten (~92.99% 182W) is deposited on the surface of a bulk tungsten sample with the natural abundance of the isotopes. This sample is then exposed to helium plasma at the conditions necessary to support the formation of tungsten 'fuzz'. Depth profiles of the concentration of each of the tungsten isotopes are obtained using secondary ion mass spectrometry (SIMS) before and after the plasma exposure. The depth profiles clearly show mixing of tungsten atoms from the bulk sample toward the surface of the fuzz. Lastly, this supports a physical picture of the dynamic behavior of helium bubbles which, also, causes an enhanced mixing of tungsten atoms.},
doi = {10.1088/1741-4326/aab96a},
journal = {Nuclear Fusion},
number = 6,
volume = 58,
place = {United States},
year = {Wed Apr 11 00:00:00 EDT 2018},
month = {Wed Apr 11 00:00:00 EDT 2018}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 29 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Fuzzy nanostructure growth on Ta/Fe by He plasma irradiation
journal, July 2016

  • Kajita, Shin; Ishida, Tomoya; Ohno, Noriyasu
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep30380

A full tungsten divertor for ITER: Physics issues and design status
journal, July 2013


The influence of plasma-surface interaction on the performance of tungsten at the ITER divertor vertical targets
journal, March 2018

  • De Temmerman, G.; Hirai, T.; Pitts, R. A.
  • Plasma Physics and Controlled Fusion, Vol. 60, Issue 4
  • DOI: 10.1088/1361-6587/aaaf62

Helium induced nanoscopic morphology on tungsten under fusion relevant plasma conditions
journal, January 2008


TEM observation of the growth process of helium nanobubbles on tungsten: Nanostructure formation mechanism
journal, November 2011


Erosion and redeposition experiments in the pisces facility
journal, February 1987


RESOLNRA: A new program for optimizing the achievable depth resolution of ion beam analysis methods
journal, April 2008

  • Mayer, M.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 266, Issue 8
  • DOI: 10.1016/j.nimb.2007.11.071

Sputtering properties of tungsten ‘fuzzy’ surfaces
journal, August 2011


Quantitatively measuring the influence of helium in plasma-exposed tungsten
journal, August 2017


The influence of helium on the bulk properties of fusion reactor structural materials
journal, August 1984


Observation of a helium ion energy threshold for retention in tungsten exposed to hydrogen/helium mixture plasma
journal, August 2016


Challenges and opportunities of modeling plasma–surface interactions in tungsten using high-performance computing
journal, August 2015


Experimental mechanistic investigation of the nanostructuring of tungsten with low energy helium plasmas
journal, December 2016


Self-diffusion in tungsten
journal, February 1978


Works referencing / citing this record:

Plasma-Material-Interaction Research Using PISCES Linear Plasma Devices
journal, October 2019


The evolution of He nanobubbles in tungsten under fusion-relevant He ion irradiation conditions
journal, June 2019