Tailored interfaces of unencapsulated perovskite solar cells for >1,000 hour operational stability
Abstract
Long-term device stability is the most pressing issue that impedes perovskite solar cell commercialization, given the achieved 22.7% efficiency. The perovskite absorber material itself has been heavily scrutinized for being prone to degradation by water, oxygen and ultraviolet light. To date, most reports characterize device stability in the absence of these extrinsic factors. Here we show that, even under the combined stresses of light (including ultraviolet light), oxygen and moisture, perovskite solar cells can retain 94% of peak efficiency despite 1,000 hours of continuous unencapsulated operation in ambient air conditions (relative humidity of 10-20%). Each interface and contact layer throughout the device stack plays an important role in the overall stability which, when appropriately modified, yields devices in which both the initial rapid decay (often termed burn-in) and the gradual slower decay are suppressed. This extensively modified device architecture and the understanding developed will lead towards durable long-term device performance.
- Authors:
-
[1];
[1];
[2];
[1];
[1];
[3];
[1];
[1]
- National Renewable Energy Lab. (NREL), Golden, CO (United States)
- Colorado School of Mines, Golden, CO (United States)
- National Renewable Energy Lab. (NREL), Golden, CO (United States); Colorado School of Mines, Golden, CO (United States)
- Publication Date:
- Research Org.:
- National Renewable Energy Laboratory (NREL), Golden, CO (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office
- OSTI Identifier:
- 1419410
- Report Number(s):
- NREL/JA-5900-68531
Journal ID: ISSN 2058-7546
- Grant/Contract Number:
- AC36-08GO28308
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Energy
- Additional Journal Information:
- Journal Volume: 3; Journal Issue: 1; Journal ID: ISSN 2058-7546
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; 36 MATERIALS SCIENCE; perovskite solar cells; efficiency; stability
Citation Formats
Christians, Jeffrey A., Schulz, Philip, Tinkham, Jonathan S., Schloemer, Tracy H., Harvey, Steven P., Tremolet de Villers, Bertrand J., Sellinger, Alan, Berry, Joseph J., and Luther, Joseph M. Tailored interfaces of unencapsulated perovskite solar cells for >1,000 hour operational stability. United States: N. p., 2017.
Web. doi:10.1038/s41560-017-0067-y.
Christians, Jeffrey A., Schulz, Philip, Tinkham, Jonathan S., Schloemer, Tracy H., Harvey, Steven P., Tremolet de Villers, Bertrand J., Sellinger, Alan, Berry, Joseph J., & Luther, Joseph M. Tailored interfaces of unencapsulated perovskite solar cells for >1,000 hour operational stability. United States. https://doi.org/10.1038/s41560-017-0067-y
Christians, Jeffrey A., Schulz, Philip, Tinkham, Jonathan S., Schloemer, Tracy H., Harvey, Steven P., Tremolet de Villers, Bertrand J., Sellinger, Alan, Berry, Joseph J., and Luther, Joseph M. Tue .
"Tailored interfaces of unencapsulated perovskite solar cells for >1,000 hour operational stability". United States. https://doi.org/10.1038/s41560-017-0067-y. https://www.osti.gov/servlets/purl/1419410.
@article{osti_1419410,
title = {Tailored interfaces of unencapsulated perovskite solar cells for >1,000 hour operational stability},
author = {Christians, Jeffrey A. and Schulz, Philip and Tinkham, Jonathan S. and Schloemer, Tracy H. and Harvey, Steven P. and Tremolet de Villers, Bertrand J. and Sellinger, Alan and Berry, Joseph J. and Luther, Joseph M.},
abstractNote = {Long-term device stability is the most pressing issue that impedes perovskite solar cell commercialization, given the achieved 22.7% efficiency. The perovskite absorber material itself has been heavily scrutinized for being prone to degradation by water, oxygen and ultraviolet light. To date, most reports characterize device stability in the absence of these extrinsic factors. Here we show that, even under the combined stresses of light (including ultraviolet light), oxygen and moisture, perovskite solar cells can retain 94% of peak efficiency despite 1,000 hours of continuous unencapsulated operation in ambient air conditions (relative humidity of 10-20%). Each interface and contact layer throughout the device stack plays an important role in the overall stability which, when appropriately modified, yields devices in which both the initial rapid decay (often termed burn-in) and the gradual slower decay are suppressed. This extensively modified device architecture and the understanding developed will lead towards durable long-term device performance.},
doi = {10.1038/s41560-017-0067-y},
journal = {Nature Energy},
number = 1,
volume = 3,
place = {United States},
year = {Tue Nov 28 00:00:00 EST 2017},
month = {Tue Nov 28 00:00:00 EST 2017}
}
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