Electrodynamics of the antiferromagnetic phase in URu2Si2

Hall, Jesse S.; Movassagh, M. Rahimi; Wilson, M. N.; Luke, G. M.; Kanchanavatee, N.; Huang, K.; Janoschek, M.; Maple, M. B.; Timusk, T.

doi:10.1103/PhysRevB.92.195111

Title: Electrodynamics of the antiferromagnetic phase in ${URu}_{2} {Si}_{2}$

Abstract

Here, we present data on the optical conductivity of URu_2-x(Fe,Os)_xSi₂. While the parent material URu₂Si₂ enters the enigmatic hidden order (HO) phase below 17.5 K, an antiferromagnetic (AFM) phase is induced by the substitution of Fe or Os onto the Ru sites. We find that both the HO and the AFM phases exhibit an identical gap structure that is characterized by a loss of conductivity below the gap energy with spectral weight transferred to a narrow frequency region just above the gap, the typical optical signature of a density wave. The AFM phase is marked by strong increases in both transition temperature and the energy of the gap associated with the transition. In the normal phase just above the transition the optical scattering rate varies as ω². We find that in both the HO and the AFM phases, our data are consistent with elastic resonant scattering of a Fermi liquid. This indicates that the appearance of a coherent state is a necessary condition for either ordered phase to emerge. Our measurements favor models in which the HO and the AFM phases are driven by the common physics of a nesting-induced density wave gap.

Authors:

Hall, Jesse S. ^[1]; Movassagh, M. Rahimi ^[1]; Wilson, M. N. ^[1]; Luke, G. M. ^[2]; Kanchanavatee, N. ^[3]; Huang, K. ^[3]; Janoschek, M. ^[3]; Maple, M. B. ^[3]; Timusk, T. ^[2]

McMaster Univ., Hamilton, ON (Canada)
McMaster Univ., Hamilton, ON (Canada); Canadian Inst. for Advanced Research, Toronto, ON (Canada)
Univ. of California, San Diego, CA (United States)

Publication Date:: Fri Nov 06 00:00:00 EST 2015

Research Org.:: Univ. of California, San Diego, CA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1418611

Alternate Identifier(s):: OSTI ID: 1225409

Grant/Contract Number:: FG02-04ER46105; DMR-1206553

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review. B, Condensed Matter and Materials Physics

Additional Journal Information:: Journal Volume: 92; Journal Issue: 19; Journal ID: ISSN 1098-0121

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE

Citation Formats


                    Hall, Jesse S., Movassagh, M. Rahimi, Wilson, M. N., Luke, G. M., Kanchanavatee, N., Huang, K., Janoschek, M., Maple, M. B., and Timusk, T. Electrodynamics of the antiferromagnetic phase in URu2Si2.  United States: N. p., 2015. 
Web.  doi:10.1103/PhysRevB.92.195111.

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                    Hall, Jesse S., Movassagh, M. Rahimi, Wilson, M. N., Luke, G. M., Kanchanavatee, N., Huang, K., Janoschek, M., Maple, M. B., & Timusk, T. Electrodynamics of the antiferromagnetic phase in URu2Si2.  United States.  https://doi.org/10.1103/PhysRevB.92.195111

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                    Hall, Jesse S., Movassagh, M. Rahimi, Wilson, M. N., Luke, G. M., Kanchanavatee, N., Huang, K., Janoschek, M., Maple, M. B., and Timusk, T. Fri .  
"Electrodynamics of the antiferromagnetic phase in URu2Si2".  United States.  https://doi.org/10.1103/PhysRevB.92.195111.  https://www.osti.gov/servlets/purl/1418611.

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@article{osti_1418611,

  title        = {Electrodynamics of the antiferromagnetic phase in URu2Si2},

  author       = {Hall, Jesse S. and Movassagh, M. Rahimi and Wilson, M. N. and Luke, G. M. and Kanchanavatee, N. and Huang, K. and Janoschek, M. and Maple, M. B. and Timusk, T.},

  abstractNote = {Here, we present data on the optical conductivity of URu2-x(Fe,Os)xSi2. While the parent material URu2Si2 enters the enigmatic hidden order (HO) phase below 17.5 K, an antiferromagnetic (AFM) phase is induced by the substitution of Fe or Os onto the Ru sites. We find that both the HO and the AFM phases exhibit an identical gap structure that is characterized by a loss of conductivity below the gap energy with spectral weight transferred to a narrow frequency region just above the gap, the typical optical signature of a density wave. The AFM phase is marked by strong increases in both transition temperature and the energy of the gap associated with the transition. In the normal phase just above the transition the optical scattering rate varies as ω2. We find that in both the HO and the AFM phases, our data are consistent with elastic resonant scattering of a Fermi liquid. This indicates that the appearance of a coherent state is a necessary condition for either ordered phase to emerge. Our measurements favor models in which the HO and the AFM phases are driven by the common physics of a nesting-induced density wave gap.},

  doi          = {10.1103/PhysRevB.92.195111},

  journal      = {Physical Review. B, Condensed Matter and Materials Physics},

  number       = 19,

  volume       = 92,

  place        = {United States},

  year         = {Fri Nov 06 00:00:00 EST 2015},

  month        = {Fri Nov 06 00:00:00 EST 2015}

}

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Cited by: 8 works

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Figure 1: Temperature and doping dependence of the reflectance of doped samples of URu_2−x(Fe,Os)_xSi₂. The top panels shows the absolute reflectance for a) Fe doping, b) Os doping, both in the AFM state as a function of temperature. The bottom panels show the absolute reflectance as function of doping formore »

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Works referenced in this record:

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Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.

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Similar Records

Title: Electrodynamics of the antiferromagnetic phase in URu 2 Si 2

Abstract

Citation Formats

Figures / Tables:

Effect of Pressure on Tiny Antiferromagnetic Moment in the Heavy-Electron Compound URu 2 Si 2 journal, December 1999

Hidden order in journal, April 2005

The appearance of homogeneous antiferromagnetism in URu 2 Si 2 under high pressure: a 29 Si nuclear magnetic resonance study journal, March 2003

Anisotropic electrical resistivity of the magnetic heavy-fermion superconductor URu 2 Si 2 journal, May 1986

Partially gapped Fermi surface in the heavy-electron superconductor URu 2 Si 2 journal, January 1986

Gapped itinerant spin excitations account for missing entropy in the hidden-order state of URu2Si2 journal, January 2007

Fermi-surface instability at the ‘hidden-order’ transition of URu2Si2 journal, July 2009

Imaging the Fano lattice to ‘hidden order’ transition in URu2Si2 journal, June 2010

Visualizing the formation of the Kondo lattice and the hidden order in URu2Si2 journal, May 2010

Similarity of the Fermi Surface in the Hidden Order State and in the Antiferromagnetic State of URu 2 Si 2 journal, November 2010

Arrested Kondo effect and hidden order in URu2Si2 journal, September 2009

Hybridization Wave as the “Hidden Order” in URu 2 Si 2 journal, February 2011

Hastatic order in the heavy-fermion compound URu2Si2 journal, January 2013

Phase transition arising from the underscreened Anderson lattice model: A candidate concept for explaining hidden order in URu 2 Si 2 journal, April 2012

Imprints of spin-orbit density wave in the hidden-order state of URu 2 Si 2 journal, January 2014

Effect of pressure on competing electronic correlations in the heavy-electron system URu 2 Si 2 journal, January 1987

Parasitic Small-Moment Antiferromagnetism and Nonlinear Coupling of Hidden Order and Antiferromagnetism in URu 2 Si 2 Observed by Larmor Diffraction journal, March 2010

Pressure–temperature phase diagram of the heavy-electron superconductor journal, March 2007

Neutron scattering studies on URu 2 Si 2 journal, July 2014

Temperature-pressure phase diagram of U Ru 2 Si 2 from resistivity measurements and ac calorimetry: Hidden order and Fermi-surface nesting journal, March 2008

The de Haas–van Alphen effect in URu 2 Si 2 under pressure journal, July 2003

Hidden order in URu2Si2 originates from Fermi surface gapping induced by dynamic symmetry breaking journal, February 2009

Spin and orbital hybridization at specifically nested Fermi surfaces in URu 2 Si 2 journal, December 2011

Twofold enhancement of the hidden-order/large-moment antiferromagnetic phase boundary in the URu 2 − x Fe x Si 2 system journal, December 2011

Chemical pressure tuning of URu 2 Si 2 via isoelectronic substitution of Ru with Fe journal, February 2015

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Competing Ordered Phases in URu 2 Si 2 : Hydrostatic Pressure and Rhenium Substitution journal, November 2007

Technique for measuring the reflectance of irregular, submillimeter-sized samples journal, January 1993

Observation of multiple-gap structure in hidden order state of URu 2 Si 2 from optical conductivity journal, July 2012

The evolution of the ordered states of single-crystal URu 2 Si 2 under pressure journal, February 2008

Optical spectroscopy shows that the normal state of URu2Si2 is an anomalous Fermi liquid journal, October 2012

Hybridization gap versus hidden-order gap in URu 2 Si 2 as revealed by optical spectroscopy journal, May 2012

Optical study of hybridization and hidden order in URu 2 Si 2 journal, April 2014

First-Matsubara-frequency rule in a Fermi liquid. II. Optical conductivity and comparison to experiment journal, October 2012

Evolution of the bosonic spectral density of the high-temperature superconductor Bi 2 Sr 2 Ca Cu 2 O 8 + δ journal, April 2007

Title: Electrodynamics of the antiferromagnetic phase in ${URu}_{2} {Si}_{2}$

Effect of Pressure on Tiny Antiferromagnetic Moment in the Heavy-Electron Compound ${URu}_{2} {Si}_{2}$
journal, December 1999

Hidden order in
journal, April 2005

The appearance of homogeneous antiferromagnetism in URu ₂ Si ₂ under high pressure: a ²⁹ Si nuclear magnetic resonance study
journal, March 2003

Anisotropic electrical resistivity of the magnetic heavy-fermion superconductor ${URu}_{2}$ ${Si}_{2}$
journal, May 1986

Partially gapped Fermi surface in the heavy-electron superconductor ${URu}_{2}$ ${Si}_{2}$
journal, January 1986

Gapped itinerant spin excitations account for missing entropy in the hidden-order state of URu2Si2
journal, January 2007

Fermi-surface instability at the ‘hidden-order’ transition of URu2Si2
journal, July 2009

Imaging the Fano lattice to ‘hidden order’ transition in URu2Si2
journal, June 2010

Visualizing the formation of the Kondo lattice and the hidden order in URu2Si2
journal, May 2010

Similarity of the Fermi Surface in the Hidden Order State and in the Antiferromagnetic State of ${URu}_{2} {Si}_{2}$
journal, November 2010

Arrested Kondo effect and hidden order in URu2Si2
journal, September 2009

Hybridization Wave as the “Hidden Order” in ${URu}_{2} {Si}_{2}$
journal, February 2011

Hastatic order in the heavy-fermion compound URu2Si2
journal, January 2013

Phase transition arising from the underscreened Anderson lattice model: A candidate concept for explaining hidden order in URu $_{2}$ Si $_{2}$
journal, April 2012

Imprints of spin-orbit density wave in the hidden-order state of URu $_{2}$ Si $_{2}$
journal, January 2014

Effect of pressure on competing electronic correlations in the heavy-electron system ${URu}_{2}$ ${Si}_{2}$
journal, January 1987

Parasitic Small-Moment Antiferromagnetism and Nonlinear Coupling of Hidden Order and Antiferromagnetism in ${URu}_{2} {Si}_{2}$ Observed by Larmor Diffraction
journal, March 2010

Pressure–temperature phase diagram of the heavy-electron superconductor
journal, March 2007

Neutron scattering studies on URu ₂ Si ₂
journal, July 2014

Temperature-pressure phase diagram of $U {Ru}_{2} {Si}_{2}$ from resistivity measurements and ac calorimetry: Hidden order and Fermi-surface nesting
journal, March 2008

The de Haas–van Alphen effect in URu ₂ Si ₂ under pressure
journal, July 2003

Hidden order in URu2Si2 originates from Fermi surface gapping induced by dynamic symmetry breaking
journal, February 2009

Spin and orbital hybridization at specifically nested Fermi surfaces in URu $_{2}$ Si $_{2}$
journal, December 2011

Twofold enhancement of the hidden-order/large-moment antiferromagnetic phase boundary in the URu $_{2 - x}$ Fe $_{x}$ Si $_{2}$ system
journal, December 2011

Chemical pressure tuning of ${URu}_{2} {Si}_{2}$ via isoelectronic substitution of Ru with Fe
journal, February 2015

Enhancement of the hidden order/large moment antiferromagnetic transition temperature in the URu _{2− x} Os _x Si ₂ system
journal, April 2014

Competing Ordered Phases in ${URu}_{2} {Si}_{2}$ : Hydrostatic Pressure and Rhenium Substitution
journal, November 2007

Technique for measuring the reflectance of irregular, submillimeter-sized samples
journal, January 1993

Observation of multiple-gap structure in hidden order state of URu $_{2}$ Si $_{2}$ from optical conductivity
journal, July 2012

The evolution of the ordered states of single-crystal URu ₂ Si ₂ under pressure
journal, February 2008

Optical spectroscopy shows that the normal state of URu2Si2 is an anomalous Fermi liquid
journal, October 2012

Hybridization gap versus hidden-order gap in URu $_{2}$ Si $_{2}$ as revealed by optical spectroscopy
journal, May 2012

Optical study of hybridization and hidden order in URu ₂ Si ₂
journal, April 2014

First-Matsubara-frequency rule in a Fermi liquid. II. Optical conductivity and comparison to experiment
journal, October 2012

Evolution of the bosonic spectral density of the high-temperature superconductor ${Bi}_{2} {Sr}_{2} Ca {Cu}_{2} O_{8 + δ}$
journal, April 2007