MIX: a mosaic Asian anthropogenic emission inventory under the international collaboration framework of the MICS-Asia and HTAP
Abstract
Here, the MIX inventory is developed for the years 2008 and 2010 to support the Model Inter-Comparison Study for Asia (MICS-Asia) and the Task Force on Hemispheric Transport of Air Pollution (TF HTAP) by a mosaic of up-to-date regional emission inventories. Emissions are estimated for all major anthropogenic sources in 29 countries and regions in Asia. We conducted detailed comparisons of different regional emission inventories and incorporated the best available ones for each region into the mosaic inventory at a uniform spatial and temporal resolution. Emissions are aggregated to five anthropogenic sectors: power, industry, residential, transportation, and agriculture. We estimate the total Asian emissions of 10 species in 2010 as follows: 51.3 Tg SO2, 52.1 Tg NOx, 336.6 Tg CO, 67.0 Tg NMVOC (non-methane volatile organic compounds), 28.8 Tg NH3, 31.7 Tg PM10, 22.7 Tg PM2.5, 3.5 Tg BC, 8.3 Tg OC, and 17.3 Pg CO2. Emissions from China and India dominate the emissions of Asia for most of the species. We also estimated Asian emissions in 2006 using the same methodology of MIX. The relative change rates of Asian emissions for the period of 2006–2010 are estimated as follows: –8.1 % for SO2, +19.2 % for NOx, +3.9 % for CO,more »
- Authors:
-
- Tsinghua Univ., Beijing (China)
- Tsinghua Univ., Beijing (China); Collaborative Innovation Center for Regional Environmental Quality, Beijing (China)
- Asia Center for Air Pollution Research, Niigata (Japan)
- Konkuk Univ., Seoul (Korea)
- Tsinghua Univ., Beijing (China); State Environmental Protection Key Lab. of Sources and Control of Air Pollution Complex, Beijing (China); Collaborative Innovation Center for Regional Environmental Quality, Beijing (China)
- Argonne National Lab. (ANL), Argonne, IL (United States)
- National Institute for Environmental Studies, Ibaraki (Japan)
- Peking Univ., Beijing (China)
- Univ. of Iowa, Iowa City, IA (United States)
- Max Planck Institute for Chemistry, Mainz (Germany)
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- National Basic Research Program of China; National Science Foundation of China; USDOE
- OSTI Identifier:
- 1416372
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Atmospheric Chemistry and Physics (Online)
- Additional Journal Information:
- Journal Name: Atmospheric Chemistry and Physics (Online); Journal Volume: 17; Journal Issue: 2; Journal ID: ISSN 1680-7324
- Publisher:
- European Geosciences Union
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 54 ENVIRONMENTAL SCIENCES
Citation Formats
Li, Meng, Zhang, Qiang, Kurokawa, Jun-ichi, Woo, Jung -Hun, He, Kebin, Lu, Zifeng, Ohara, Toshimasa, Song, Yu, Streets, David G., Carmichael, Gregory R., Cheng, Yafang, Hong, Chaopeng, Huo, Hong, Jiang, Xujia, Kang, Sicong, Liu, Fei, Su, Hang, and Zheng, Bo. MIX: a mosaic Asian anthropogenic emission inventory under the international collaboration framework of the MICS-Asia and HTAP. United States: N. p., 2017.
Web. doi:10.5194/acp-17-935-2017.
Li, Meng, Zhang, Qiang, Kurokawa, Jun-ichi, Woo, Jung -Hun, He, Kebin, Lu, Zifeng, Ohara, Toshimasa, Song, Yu, Streets, David G., Carmichael, Gregory R., Cheng, Yafang, Hong, Chaopeng, Huo, Hong, Jiang, Xujia, Kang, Sicong, Liu, Fei, Su, Hang, & Zheng, Bo. MIX: a mosaic Asian anthropogenic emission inventory under the international collaboration framework of the MICS-Asia and HTAP. United States. https://doi.org/10.5194/acp-17-935-2017
Li, Meng, Zhang, Qiang, Kurokawa, Jun-ichi, Woo, Jung -Hun, He, Kebin, Lu, Zifeng, Ohara, Toshimasa, Song, Yu, Streets, David G., Carmichael, Gregory R., Cheng, Yafang, Hong, Chaopeng, Huo, Hong, Jiang, Xujia, Kang, Sicong, Liu, Fei, Su, Hang, and Zheng, Bo. Fri .
"MIX: a mosaic Asian anthropogenic emission inventory under the international collaboration framework of the MICS-Asia and HTAP". United States. https://doi.org/10.5194/acp-17-935-2017. https://www.osti.gov/servlets/purl/1416372.
@article{osti_1416372,
title = {MIX: a mosaic Asian anthropogenic emission inventory under the international collaboration framework of the MICS-Asia and HTAP},
author = {Li, Meng and Zhang, Qiang and Kurokawa, Jun-ichi and Woo, Jung -Hun and He, Kebin and Lu, Zifeng and Ohara, Toshimasa and Song, Yu and Streets, David G. and Carmichael, Gregory R. and Cheng, Yafang and Hong, Chaopeng and Huo, Hong and Jiang, Xujia and Kang, Sicong and Liu, Fei and Su, Hang and Zheng, Bo},
abstractNote = {Here, the MIX inventory is developed for the years 2008 and 2010 to support the Model Inter-Comparison Study for Asia (MICS-Asia) and the Task Force on Hemispheric Transport of Air Pollution (TF HTAP) by a mosaic of up-to-date regional emission inventories. Emissions are estimated for all major anthropogenic sources in 29 countries and regions in Asia. We conducted detailed comparisons of different regional emission inventories and incorporated the best available ones for each region into the mosaic inventory at a uniform spatial and temporal resolution. Emissions are aggregated to five anthropogenic sectors: power, industry, residential, transportation, and agriculture. We estimate the total Asian emissions of 10 species in 2010 as follows: 51.3 Tg SO2, 52.1 Tg NOx, 336.6 Tg CO, 67.0 Tg NMVOC (non-methane volatile organic compounds), 28.8 Tg NH3, 31.7 Tg PM10, 22.7 Tg PM2.5, 3.5 Tg BC, 8.3 Tg OC, and 17.3 Pg CO2. Emissions from China and India dominate the emissions of Asia for most of the species. We also estimated Asian emissions in 2006 using the same methodology of MIX. The relative change rates of Asian emissions for the period of 2006–2010 are estimated as follows: –8.1 % for SO2, +19.2 % for NOx, +3.9 % for CO, +15.5 % for NMVOC, +1.7 % for NH3, –3.4 % for PM10, –1.6 % for PM2.5, +5.5 % for BC, +1.8 % for OC, and +19.9 % for CO2. Model-ready speciated NMVOC emissions for SAPRC-99 and CB05 mechanisms were developed following a profile-assignment approach.},
doi = {10.5194/acp-17-935-2017},
journal = {Atmospheric Chemistry and Physics (Online)},
number = 2,
volume = 17,
place = {United States},
year = {Fri Jan 20 00:00:00 EST 2017},
month = {Fri Jan 20 00:00:00 EST 2017}
}
Web of Science
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- Remote Sensing, Vol. 11, Issue 16
Surface ozone and its precursors at Summit, Greenland: comparison between observations and model simulations
journal, January 2017
- Huang, Yaoxian; Wu, Shiliang; Kramer, Louisa J.
- Atmospheric Chemistry and Physics, Vol. 17, Issue 23
Acetone–CO enhancement ratios in the upper troposphere based on 7 years of CARIBIC data: new insights and estimates of regional acetone fluxes
journal, January 2017
- Fischbeck, Garlich; Bönisch, Harald; Neumaier, Marco
- Atmospheric Chemistry and Physics, Vol. 17, Issue 3
Comparison of emissions inventories of anthropogenic air pollutants and greenhouse gases in China
journal, January 2017
- Saikawa, Eri; Kim, Hankyul; Zhong, Min
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Contributions of residential coal combustion to the air quality in Beijing–Tianjin–Hebei (BTH), China: a case study
journal, January 2018
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- Atmospheric Chemistry and Physics, Vol. 18, Issue 14
Foreign and domestic contributions to springtime ozone over China
journal, January 2018
- Ni, Ruijing; Lin, Jintai; Yan, Yingying
- Atmospheric Chemistry and Physics, Vol. 18, Issue 15
Trends in China's anthropogenic emissions since 2010 as the consequence of clean air actions
journal, January 2018
- Zheng, Bo; Tong, Dan; Li, Meng
- Atmospheric Chemistry and Physics, Vol. 18, Issue 19
Modeling the impact of chlorine emissions from coal combustion and prescribed waste incineration on tropospheric ozone formation in China
journal, January 2018
- Liu, Yiming; Fan, Qi; Chen, Xiaoyang
- Atmospheric Chemistry and Physics, Vol. 18, Issue 4
Dome effect of black carbon and its key influencing factors: a one-dimensional modelling study
journal, January 2018
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- Atmospheric Chemistry and Physics, Vol. 18, Issue 4
Comparison and evaluation of anthropogenic emissions of SO2 and NOx over China
journal, January 2018
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- Atmospheric Chemistry and Physics, Vol. 18, Issue 5
Evaluation of modeling NO2 concentrations driven by satellite-derived and bottom-up emission inventories using in situ measurements over China
journal, January 2018
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Assessment of inter-city transport of particulate matter in the Beijing–Tianjin–Hebei region
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Air quality and climate change, Topic 3 of the Model Inter-Comparison Study for Asia Phase III (MICS-Asia III) – Part 1: Overview and model evaluation
journal, January 2018
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Impacts of biogenic and anthropogenic emissions on summertime ozone formation in the Guanzhong Basin, China
journal, January 2018
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- Atmospheric Chemistry and Physics, Vol. 18, Issue 10
Source influence on emission pathways and ambient PM 2.5 pollution over India (2015–2050)
journal, January 2018
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Assessing the formation and evolution mechanisms of severe haze pollution in the Beijing–Tianjin–Hebei region using process analysis
journal, January 2019
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Exploring the impacts of anthropogenic emission sectors on PM2.5 and human health in South and East Asia
journal, January 2019
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Model evaluation and intercomparison of surface-level ozone and relevant species in East Asia in the context of MICS-Asia Phase III – Part 1: Overview
journal, January 2019
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Possible heterogeneous chemistry of hydroxymethanesulfonate (HMS) in northern China winter haze
journal, January 2019
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Wintertime secondary organic aerosol formation in Beijing–Tianjin–Hebei (BTH): contributions of HONO sources and heterogeneous reactions
journal, January 2019
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The potential role of methanesulfonic acid (MSA) in aerosol formation and growth and the associated radiative forcings
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Comparison of surface ozone simulation among selected regional models in MICS-Asia III – effects of chemistry and vertical transport for the causes of difference
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Heterogeneous sulfate aerosol formation mechanisms during wintertime Chinese haze events: air quality model assessment using observations of sulfate oxygen isotopes in Beijing
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High-time-resolution source apportionment of PM2.5 in Beijing with multiple models
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Contrasting physical properties of black carbon in urban Beijing between winter and summer
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Secondary organic aerosol enhanced by increasing atmospheric oxidizing capacity in Beijing–Tianjin–Hebei (BTH), China
journal, January 2019
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Exploring 2016–2017 surface ozone pollution over China: source contributions and meteorological influences
journal, January 2019
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Modeling the aging process of black carbon during atmospheric transport using a new approach: a case study in Beijing
journal, January 2019
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Air quality and climate change, Topic 3 of the Model Inter-Comparison Study for Asia Phase III (MICS-Asia III) – Part 2: aerosol radiative effects and aerosol feedbacks
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Effect of changing NOx lifetime on the seasonality and long-term trends of satellite-observed tropospheric NO2 columns over China
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Regional variability in black carbon and carbon monoxide ratio from long-term observations over East Asia: assessment of representativeness for black carbon (BC) and carbon monoxide (CO) emission inventories
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Nepal Ambient Monitoring and Source Testing Experiment (NAMaSTE): Emissions of particulate matter and sulfur dioxide from vehicles and brick kilns and their impacts on air quality in the Kathmandu Valley, Nepal
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Space-based NO x emission estimates over remote regions improved in DECSO
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Updated SO2 emission estimates over China using OMI/Aura observations
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Ensemble forecasts of air quality in eastern China – Part 1: Model description and implementation of the MarcoPolo–Panda prediction system, version 1
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Impact of Climate Change on Siberian High and Wintertime Air Pollution in China in Past Two Decades
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Enhancement of PM 2.5 Concentrations by Aerosol-Meteorology Interactions Over China
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Toward Synchronous Evaluation of Source Apportionments for Atmospheric Concentration and Deposition of Sulfate Aerosol Over East Asia
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The direct effects of black carbon aerosols from different source sectors in East Asia in summer
journal, June 2019
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Contribution of Hydroxymethane Sulfonate to Ambient Particulate Matter: A Potential Explanation for High Particulate Sulfur During Severe Winter Haze in Beijing
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The Impact of the Direct Effect of Aerosols on Meteorology and Air Quality Using Aerosol Optical Depth Assimilation During the KORUS‐AQ Campaign
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Changes in PM 2.5 sensitivity to NO x and NH 3 emissions due to a large decrease in SO 2 emissions from 2013 to 2018
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Rapid decline in carbon monoxide emissions and export from East Asia between years 2005 and 2016
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Anthropogenic emission inventories in China: a review
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The Effects of the Trans-Regional Transport of PM2.5 on a Heavy Haze Event in the Pearl River Delta in January 2015
journal, May 2019
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Dust Heterogeneous Reactions during Long-Range Transport of a Severe Dust Storm in May 2017 over East Asia
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Do Compactness and Poly-Centricity Mitigate PM10 Emissions? Evidence from Yangtze River Delta Area
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A new global anthropogenic SO 2 emission inventory for the last decade: a mosaic of satellite-derived and bottom-up emissions
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Variability of depolarization of aerosol particles in the megacity of Beijing: implications for the interaction between anthropogenic pollutants and mineral dust particles
journal, January 2018
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- Atmospheric Chemistry and Physics, Vol. 18, Issue 24
Lower tropospheric ozone over India and its linkage to the South Asian monsoon
journal, January 2018
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Multi-model study of HTAP II on sulfur and nitrogen deposition
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Rapid transition in winter aerosol composition in Beijing from 2014 to 2017: response to clean air actions
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Significant reduction of PM2.5 in eastern China due to regional-scale emission control: evidence from SORPES in 2011–2018
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Estimating global surface ammonia concentrations inferred from satellite retrievals
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Substantial ozone enhancement over the North China Plain from increased biogenic emissions due to heat waves and land cover in summer 2017
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Estimating ground-level CO concentrations across China based on the national monitoring network and MOPITT: potentially overlooked CO hotspots in the Tibetan Plateau
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Impacts of meteorology and emissions on summertime surface ozone increases over central eastern China between 2003 and 2015
journal, January 2019
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Arctic marine secondary organic aerosol contributes significantly to summertime particle size distributions in the Canadian Arctic Archipelago
journal, January 2019
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Causes of a continuous summertime O3 pollution event in Jinan, a central city in the North China Plain
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Characteristics of ozone and particles in the near-surface atmosphere in the urban area of the Yangtze River Delta, China
journal, January 2019
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Satellite data reveal a common combustion emission pathway for major cities in China
journal, January 2019
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Assessment of dicarbonyl contributions to secondary organic aerosols over China using RAMS-CMAQ
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Simultaneous shipborne measurements of CO2, CH4 and CO and their application to improving greenhouse-gas flux estimates in Australia
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Nepal Ambient Monitoring and Source Testing Experiment (NAMaSTE): emissions of particulate matter and sulfur dioxide from vehicles and brick kilns and their impacts on air quality in the Kathmandu Valley, Nepal
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Evaluation of the effect of regional joint-control measures on changing photochemical transformation: a comprehensive study of the optimization scenario analysis
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Observations of aerosol optical properties at a coastal site in Hong Kong, South China
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Which processes drive observed variations of HCHO columns over India?
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Contrasting physical properties of black carbon in urban Beijing between winter and summer
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MICS-Asia III: Multi-model comparison and evaluation of aerosol over East Asia
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Characterization of organic aerosols from a Chinese Mega-City during winter:
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Updated SO2 emission estimates over China using OMI/Aura observations
journal, September 2017
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Development of the Real-time On-road Emission (ROE v1.0) model for street-scale air quality modeling based on dynamic traffic big data
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Acetone–CO enhancement ratios in the upper troposphere based on 7 years of CARIBIC data: new insights and estimates of regional acetone fluxes
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A possible pathway for rapid growth of sulfate during haze days in China
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Impact of intercontinental pollution transport on North American ozone air pollution: an HTAP phase 2 multi-model study
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Speciated online PM1 from South Asian combustion sources – Part 1: Fuel-based emission factors and size distributions
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MICS-Asia III: multi-model comparison and evaluation of aerosol over East Asia
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Historical (1750–2014) anthropogenic emissions of reactive gases and aerosols from the Community Emissions Data System (CEDS)
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Constraining Emissions of Volatile Organic Compounds Over the Indian Subcontinent Using Space‐Based Formaldehyde Measurements
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Mitigation of severe urban haze pollution by a precision air pollution control approach
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Intercomparison of NOx emission inventories over East Asia
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Enhanced trans-Himalaya pollution transport to the Tibetan Plateau by cut-off low systems
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Modeling study of impacts on surface ozone of regional transport and emissions reductions over North China Plain in summer 2015
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Impacts of shipping emissions on PM2.5 pollution in China
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Characterization of organic aerosols from a Chinese megacity during winter: predominance of fossil fuel combustion
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Acetone-CO enhancement ratios in the upper troposphere based on 7 years of CARIBIC data: New insights and estimates of regional acetone fluxes
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Nitrate transboundary heavy pollution over East Asia in winter
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Lower tropospheric ozone over India and its linkage to the South Asian monsoon
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Dome effect of black carbon and its key influencing factors: A one-dimensional modelling study
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Widespread and persistent ozone pollution in eastern China during the non-winter season of 2015: observations and source attributions
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Amplification of light absorption of black carbon associated with air pollution
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Unraveling the role of silicon in atmospheric aerosol secondary formation: A new conservative tracer for aerosol chemistry
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Maritime NO x Emissions Over Chinese Seas Derived From Satellite Observations
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Air quality improvements and health benefits from China’s clean air action since 2013
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Correlations between PM2.5 and Ozone over China and Associated Underlying Reasons
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TCCON Philippines: First Measurement Results, Satellite Data and Model Comparisons in Southeast Asia
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Nitrate transboundary heavy pollution over East Asia in winter
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Emission or atmospheric processes? An attempt to attribute the source of large bias of aerosols in eastern China simulated by global climate models
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Effects of meteorology and emissions on urban air quality: a quantitative statistical approach to long-term records (1999–2016) in Seoul, South Korea
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A 15-year record (2001–2015) of the ratio of nitrate to non-sea-salt sulfate in precipitation over East Asia
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Which processes drive observed variations of HCHO columns over India?
journal, January 2018
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Unraveling the role of silicon in atmospheric aerosol secondary formation: a new conservative tracer for aerosol chemistry
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Dominant role of emission reduction in PM 2.5 air quality improvement in Beijing during 2013–2017: a model-based decomposition analysis
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Effectiveness of short-term air quality emission controls: a high-resolution model study of Beijing during the Asia-Pacific Economic Cooperation (APEC) summit period
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Heterogeneous sulfate aerosol formation mechanisms during wintertime Chinese haze events: Air quality model assessment using observations of sulfate oxygen isotopes in Beijing
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Rapid transition in winter aerosol composition in Beijing from 2014 to 2017: response to clean air actions
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Impacts of air pollutants from rural Chinese households under the rapid residential energy transition
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Predicted impact of thermal power generation emission control measures in the Beijing-Tianjin-Hebei region on air pollution over Beijing, China
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Mitigation of severe urban haze pollution by a precision air pollution control approach
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Impact of intercontinental pollution transport on North American ozone air pollution: an HTAP phase 2 multi-model study
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