Ultrahigh thermoelectric power factor in flexible hybrid inorganic-organic superlattice
Abstract
Hybrid inorganic–organic superlattice with an electron-transmitting but phonon-blocking structure has emerged as a promising flexible thin film thermoelectric material. However, the substantial challenge in optimizing carrier concentration without disrupting the superlattice structure prevents further improvement of the thermoelectric performance. Here we demonstrate a strategy for carrier optimization in a hybrid inorganic–organic superlattice of TiS2[tetrabutylammonium] x [hexylammonium] y, where the organic layers are composed of a random mixture of tetrabutylammonium and hexylammonium molecules. By vacuum heating the hybrid materials at an intermediate temperature, the hexylammonium molecules with a lower boiling point are selectively de-intercalated, which reduces the electron density due to the requirement of electroneutrality. The tetrabutylammonium molecules with a higher boiling point remain to support and stabilize the superlattice structure. Furthermore, the carrier concentration can thus be effectively reduced, resulting in a remarkably high power factor of 904 µW m–1 K–2 at 300 K for flexible thermoelectrics, approaching the values achieved in conventional inorganic semiconductors.
- Authors:
-
- Tsinghua Univ., Beijing (China)
- Toyota Physical and Chemical Research Institute, Nagakute (Japan)
- Nagoya Univ., Nagoya (Japan)
- Univ. of Colorado, Boulder, CO (United States); National Renewable Energy Lab. (NREL), Golden, CO (United States)
- Publication Date:
- Research Org.:
- National Renewable Energy Laboratory (NREL), Golden, CO (United States)
- Sponsoring Org.:
- National Science Foundation (NSF); USDOE
- OSTI Identifier:
- 1406989
- Report Number(s):
- NREL/JA-5500-70434
Journal ID: ISSN 2041-1723
- Grant/Contract Number:
- AC36-08GO28308
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 8; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; 77 NANOSCIENCE AND NANOTECHNOLOGY; organic-inorganic nanostructures; thermoelectrics; two-dimensional materials
Citation Formats
Wan, Chunlei, Tian, Ruoming, Kondou, Mami, Yang, Ronggui, Zong, Pengan, and Koumoto, Kunihito. Ultrahigh thermoelectric power factor in flexible hybrid inorganic-organic superlattice. United States: N. p., 2017.
Web. doi:10.1038/s41467-017-01149-4.
Wan, Chunlei, Tian, Ruoming, Kondou, Mami, Yang, Ronggui, Zong, Pengan, & Koumoto, Kunihito. Ultrahigh thermoelectric power factor in flexible hybrid inorganic-organic superlattice. United States. https://doi.org/10.1038/s41467-017-01149-4
Wan, Chunlei, Tian, Ruoming, Kondou, Mami, Yang, Ronggui, Zong, Pengan, and Koumoto, Kunihito. Wed .
"Ultrahigh thermoelectric power factor in flexible hybrid inorganic-organic superlattice". United States. https://doi.org/10.1038/s41467-017-01149-4. https://www.osti.gov/servlets/purl/1406989.
@article{osti_1406989,
title = {Ultrahigh thermoelectric power factor in flexible hybrid inorganic-organic superlattice},
author = {Wan, Chunlei and Tian, Ruoming and Kondou, Mami and Yang, Ronggui and Zong, Pengan and Koumoto, Kunihito},
abstractNote = {Hybrid inorganic–organic superlattice with an electron-transmitting but phonon-blocking structure has emerged as a promising flexible thin film thermoelectric material. However, the substantial challenge in optimizing carrier concentration without disrupting the superlattice structure prevents further improvement of the thermoelectric performance. Here we demonstrate a strategy for carrier optimization in a hybrid inorganic–organic superlattice of TiS2[tetrabutylammonium] x [hexylammonium] y, where the organic layers are composed of a random mixture of tetrabutylammonium and hexylammonium molecules. By vacuum heating the hybrid materials at an intermediate temperature, the hexylammonium molecules with a lower boiling point are selectively de-intercalated, which reduces the electron density due to the requirement of electroneutrality. The tetrabutylammonium molecules with a higher boiling point remain to support and stabilize the superlattice structure. Furthermore, the carrier concentration can thus be effectively reduced, resulting in a remarkably high power factor of 904 µW m–1 K–2 at 300 K for flexible thermoelectrics, approaching the values achieved in conventional inorganic semiconductors.},
doi = {10.1038/s41467-017-01149-4},
journal = {Nature Communications},
number = 1,
volume = 8,
place = {United States},
year = {Wed Oct 18 00:00:00 EDT 2017},
month = {Wed Oct 18 00:00:00 EDT 2017}
}
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