Aminopolymer functionalization of boron nitride nanosheets for highly efficient capture of carbon dioxide

Huang, Kuan; Liang, Liangbo; Chai, Songhai; Tumuluri, Uma; Li, Meijun; Wu, Zili; Sumpter, Bobby G.; Dai, Sheng

doi:10.1039/C7TA00644F

Title: Aminopolymer functionalization of boron nitride nanosheets for highly efficient capture of carbon dioxide

Abstract

Here, BN nanosheets were functionalized with polyethyleneimine (PEI) which is rich in amine density, through simple impregnation to improve their performance for CO₂ capture.

Authors:

^[1];

^[2]; Chai, Songhai ^[3]; Tumuluri, Uma ^[2]; Li, Meijun ^[3]; Wu, Zili ^[2];

^[2];

^[4]

Nanchang Univ., Nanchang (People's Republic of China); Univ. of Tennessee, Knoxville, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Univ. of Tennessee, Knoxville, TN (United States)
Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Publication Date:: Thu Feb 23 00:00:00 EST 2017

Research Org.:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1376449

Grant/Contract Number:: AC05-00OR22725

Resource Type:: Accepted Manuscript

Journal Name:: Journal of Materials Chemistry. A

Additional Journal Information:: Journal Volume: 5; Journal Issue: 31; Journal ID: ISSN 2050-7488

Publisher:: Royal Society of Chemistry

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE

Citation Formats


                    Huang, Kuan, Liang, Liangbo, Chai, Songhai, Tumuluri, Uma, Li, Meijun, Wu, Zili, Sumpter, Bobby G., and Dai, Sheng. Aminopolymer functionalization of boron nitride nanosheets for highly efficient capture of carbon dioxide.  United States: N. p., 2017. 
Web.  doi:10.1039/C7TA00644F.

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                    Huang, Kuan, Liang, Liangbo, Chai, Songhai, Tumuluri, Uma, Li, Meijun, Wu, Zili, Sumpter, Bobby G., & Dai, Sheng. Aminopolymer functionalization of boron nitride nanosheets for highly efficient capture of carbon dioxide.  United States.  https://doi.org/10.1039/C7TA00644F

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                    Huang, Kuan, Liang, Liangbo, Chai, Songhai, Tumuluri, Uma, Li, Meijun, Wu, Zili, Sumpter, Bobby G., and Dai, Sheng. Thu .  
"Aminopolymer functionalization of boron nitride nanosheets for highly efficient capture of carbon dioxide".  United States.  https://doi.org/10.1039/C7TA00644F.  https://www.osti.gov/servlets/purl/1376449.

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@article{osti_1376449,

  title        = {Aminopolymer functionalization of boron nitride nanosheets for highly efficient capture of carbon dioxide},

  author       = {Huang, Kuan and Liang, Liangbo and Chai, Songhai and Tumuluri, Uma and Li, Meijun and Wu, Zili and Sumpter, Bobby G. and Dai, Sheng},

  abstractNote = {Here, BN nanosheets were functionalized with polyethyleneimine (PEI) which is rich in amine density, through simple impregnation to improve their performance for CO2 capture.},

  doi          = {10.1039/C7TA00644F},

  journal      = {Journal of Materials Chemistry. A},

  number       = 31,

  volume       = 5,

  place        = {United States},

  year         = {Thu Feb 23 00:00:00 EST 2017},

  month        = {Thu Feb 23 00:00:00 EST 2017}

}

Copy to clipboard

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Works referencing / citing this record:

Improved capture of carbon dioxide and methane via adding micropores within porous boron nitride fibers
journal, April 2019

Wang, DeKun; Xue, Yanming; Wang, Chenyang
Journal of Materials Science, Vol. 54, Issue 14
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Irreversible water mediated transformation of BCN from a 3D highly porous form to its nonporous hydrolyzed counterpart
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Daneshnia, Shirin; Adeli, Mohsen; Yari, Abdolah
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Title: Aminopolymer functionalization of boron nitride nanosheets for highly efficient capture of carbon dioxide

Abstract

Citation Formats

Generalized Gradient Approximation Made Simple journal, October 1996

Graphene Analogues of BN: Novel Synthesis and Properties journal, February 2010

Adsorptive removal of carbon dioxide using polyethyleneimine-loaded mesoporous silica materials journal, August 2008

Mesoporous Alumina-Supported Amines as Potential Steam-Stable Adsorbents for Capturing CO 2 from Simulated Flue Gas and Ambient Air journal, November 2011

Amine-functionalized boron nitride nanotubes journal, June 2007

Graphene-Based Porous Silica Sheets Impregnated with Polyethyleneimine for Superior CO 2 Capture journal, February 2013

Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set journal, July 1996

Ambient Carbon Dioxide Capture by Boron-Rich Boron Nitride Nanotube journal, February 2011

FTIR Study of CO2 Adsorption on Amine-Grafted SBA-15: Elucidation of Adsorbed Species journal, May 2011

Selective oxidative dehydrogenation of propane to propene using boron nitride catalysts journal, December 2016

Solubilization of boron nitride nanotubes journal, January 2005

Adsorbent Materials for Carbon Dioxide Capture from Large Anthropogenic Point Sources journal, September 2009

Few-layered graphene-like boron nitride induced a remarkable adsorption capacity for dibenzothiophene in fuels journal, January 2015

Optical properties of hexagonal boron nitride journal, June 1976

Competitive adsorption of CO2/CH4 in porous boron nitride nanomaterials journal, December 2015

Erratum: Acceleration of global warming due to carbon-cycle feedbacks in a coupled climate model journal, December 2000

Infrared Study of CO 2 Sorption over “Molecular Basket” Sorbent Consisting of Polyethylenimine-Modified Mesoporous Molecular Sieve journal, April 2009

CO 2 -Induced Degradation of Amine-Containing Adsorbents: Reaction Products and Pathways journal, August 2012

Boron Nitride Nanotubes and Nanosheets journal, May 2010

Molecular Selectivity of Graphene-Enhanced Raman Scattering journal, April 2015

CO 2 adsorption on single-walled boron nitride nanotubes containing vacancy defects journal, January 2015

Van der Waals Density Functional for General Geometries journal, June 2004

Polyethyleneimine–nano silica composites: a low-cost and promising adsorbent for CO 2 capture journal, January 2015

Facilely synthesized meso-macroporous polymer as support of poly(ethyleneimine) for highly efficient and selective capture of CO2 journal, April 2017

Porous boron nitride nanosheets for effective water cleaning journal, April 2013

Adsorption characteristics of carbon dioxide on organically functionalized SBA-15 journal, September 2005

Magnetic Boron Nitride Nanoribbons with Tunable Electronic Properties journal, August 2008

A template-free solvent-mediated synthesis of high surface area boron nitride nanosheets for aerobic oxidative desulfurization journal, January 2016

Polyethyleneimine Incorporated Metal-Organic Frameworks Adsorbent for Highly Selective CO2 Capture journal, May 2013

Carbon dioxide adsorption on doped boron nitride nanotubes journal, January 2014

Covalent Organic Frameworks for CO 2 Capture journal, February 2016

Dramatic Enhancement of CO 2 Uptake by Poly(ethyleneimine) Using Zirconosilicate Supports journal, June 2012

Amine Scrubbing for CO2 Capture journal, September 2009

Enhanced selective CO 2 adsorption on polyamine/MIL-101(Cr) composites journal, January 2014

A density functional theory analysis for the adsorption of the amine group on graphene and boron nitride nanosheets journal, August 2012

Progress in adsorption-based CO 2 capture by metal–organic frameworks journal, January 2012

Nitrogen-containing porous carbons: synthesis and application journal, January 2013

Direct Capture of CO2 from Ambient Air journal, August 2016

Atmospheric chemistry and environmental impact of the use of amines in carbon capture and storage (CCS) journal, January 2012

Charge-Controlled Switchable CO 2 Capture on Boron Nitride Nanomaterials journal, May 2013

Chemical Functionalization of Boron−Nitride Nanotubes with NH3 and Amino Functional Groups journal, August 2006

Amide Functionalized Microporous Organic Polymer (Am-MOP) for Selective CO 2 Sorption and Catalysis journal, March 2014

Improved capture of carbon dioxide and methane via adding micropores within porous boron nitride fibers journal, April 2019

Irreversible water mediated transformation of BCN from a 3D highly porous form to its nonporous hydrolyzed counterpart journal, January 2018

One-step template-free synthesis of 3D functionalized flower-like boron nitride nanosheets for NH 3 and CO 2 adsorption journal, January 2018

Boron nitride: a promising material for proton exchange membranes for energy applications journal, January 2019

Low temperature functionalization of two-dimensional boron nitride for electrochemical sensing journal, July 2019

Generalized Gradient Approximation Made Simple
journal, October 1996

Graphene Analogues of BN: Novel Synthesis and Properties
journal, February 2010

Adsorptive removal of carbon dioxide using polyethyleneimine-loaded mesoporous silica materials
journal, August 2008

Mesoporous Alumina-Supported Amines as Potential Steam-Stable Adsorbents for Capturing CO ₂ from Simulated Flue Gas and Ambient Air
journal, November 2011

Amine-functionalized boron nitride nanotubes
journal, June 2007

Graphene-Based Porous Silica Sheets Impregnated with Polyethyleneimine for Superior CO ₂ Capture
journal, February 2013

Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set
journal, July 1996

Ambient Carbon Dioxide Capture by Boron-Rich Boron Nitride Nanotube
journal, February 2011

FTIR Study of CO₂ Adsorption on Amine-Grafted SBA-15: Elucidation of Adsorbed Species
journal, May 2011

Selective oxidative dehydrogenation of propane to propene using boron nitride catalysts
journal, December 2016

Solubilization of boron nitride nanotubes
journal, January 2005

Adsorbent Materials for Carbon Dioxide Capture from Large Anthropogenic Point Sources
journal, September 2009

Few-layered graphene-like boron nitride induced a remarkable adsorption capacity for dibenzothiophene in fuels
journal, January 2015

Optical properties of hexagonal boron nitride
journal, June 1976

Competitive adsorption of CO2/CH4 in porous boron nitride nanomaterials
journal, December 2015

Erratum: Acceleration of global warming due to carbon-cycle feedbacks in a coupled climate model
journal, December 2000

Infrared Study of CO ₂ Sorption over “Molecular Basket” Sorbent Consisting of Polyethylenimine-Modified Mesoporous Molecular Sieve
journal, April 2009

CO ₂ -Induced Degradation of Amine-Containing Adsorbents: Reaction Products and Pathways
journal, August 2012

Boron Nitride Nanotubes and Nanosheets
journal, May 2010

Molecular Selectivity of Graphene-Enhanced Raman Scattering
journal, April 2015

CO ₂ adsorption on single-walled boron nitride nanotubes containing vacancy defects
journal, January 2015

Van der Waals Density Functional for General Geometries
journal, June 2004

Polyethyleneimine–nano silica composites: a low-cost and promising adsorbent for CO ₂ capture
journal, January 2015

Facilely synthesized meso-macroporous polymer as support of poly(ethyleneimine) for highly efficient and selective capture of CO2
journal, April 2017

Porous boron nitride nanosheets for effective water cleaning
journal, April 2013

Adsorption characteristics of carbon dioxide on organically functionalized SBA-15
journal, September 2005

Magnetic Boron Nitride Nanoribbons with Tunable Electronic Properties
journal, August 2008

A template-free solvent-mediated synthesis of high surface area boron nitride nanosheets for aerobic oxidative desulfurization
journal, January 2016

Polyethyleneimine Incorporated Metal-Organic Frameworks Adsorbent for Highly Selective CO2 Capture
journal, May 2013

Carbon dioxide adsorption on doped boron nitride nanotubes
journal, January 2014

Covalent Organic Frameworks for CO ₂ Capture
journal, February 2016

Dramatic Enhancement of CO ₂ Uptake by Poly(ethyleneimine) Using Zirconosilicate Supports
journal, June 2012

Amine Scrubbing for CO2 Capture
journal, September 2009

Enhanced selective CO ₂ adsorption on polyamine/MIL-101(Cr) composites
journal, January 2014

A density functional theory analysis for the adsorption of the amine group on graphene and boron nitride nanosheets
journal, August 2012

Progress in adsorption-based CO ₂ capture by metal–organic frameworks
journal, January 2012

Nitrogen-containing porous carbons: synthesis and application
journal, January 2013

Direct Capture of CO₂ from Ambient Air
journal, August 2016

Atmospheric chemistry and environmental impact of the use of amines in carbon capture and storage (CCS)
journal, January 2012

Charge-Controlled Switchable CO ₂ Capture on Boron Nitride Nanomaterials
journal, May 2013

Chemical Functionalization of Boron−Nitride Nanotubes with NH₃ and Amino Functional Groups
journal, August 2006

Amide Functionalized Microporous Organic Polymer (Am-MOP) for Selective CO ₂ Sorption and Catalysis
journal, March 2014

Improved capture of carbon dioxide and methane via adding micropores within porous boron nitride fibers
journal, April 2019

Irreversible water mediated transformation of BCN from a 3D highly porous form to its nonporous hydrolyzed counterpart
journal, January 2018

One-step template-free synthesis of 3D functionalized flower-like boron nitride nanosheets for NH ₃ and CO ₂ adsorption
journal, January 2018

Boron nitride: a promising material for proton exchange membranes for energy applications
journal, January 2019

Low temperature functionalization of two-dimensional boron nitride for electrochemical sensing
journal, July 2019