DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Measurements of droplet size in shear-driven atomization using ultra-small angle x-ray scattering

Abstract

Measurements of droplet size in optically-thick, non-evaporating, shear-driven sprays have been made using ultra-small angle x-ray scattering (USAXS). The sprays are produced by orifice-type nozzles coupled to diesel injectors, with measurements conducted from 1 – 24 mm from the orifice, spanning from the optically-dense near-nozzle region to more dilute regions where optical diagnostics are feasible. The influence of nozzle diameter, liquid injection pressure, and ambient density were examined. The USAXS measurements reveal few if any nanoscale droplets, in conflict with a popular computational model of diesel spray breakup. The average droplet diameter rapidly decreases with downstream distance from the nozzle until a plateau value is reached, after which only small changes are seen in droplet diameter. This plateau droplet size is consistent with the droplets being small enough to be stable with respect to further breakup. As a result, liquid injection pressure and nozzle diameter have the biggest impact on droplet size, while ambient density has a smaller effect.

Authors:
 [1];  [1];  [2];  [2];  [1];  [1];  [3];  [1];  [1]
  1. Argonne National Lab. (ANL), Argonne, IL (United States)
  2. Univ. Politecnica de Valencia (Spain)
  3. Argonne National Lab. (ANL), Argonne, IL (United States); Michigan State Univ., East Lansing, MI (United States)
Publication Date:
Research Org.:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Org.:
National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Energy Efficiency and Renewable Energy (EERE), Vehicle Technologies Office (EE-3V)
OSTI Identifier:
1373736
Alternate Identifier(s):
OSTI ID: 1416038
Grant/Contract Number:  
AC02-06CH11357
Resource Type:
Accepted Manuscript
Journal Name:
International Journal of Multiphase Flow
Additional Journal Information:
Journal Volume: 92; Journal Issue: C; Journal ID: ISSN 0301-9322
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY; diesel spray; droplet size; x-ray scattering

Citation Formats

Kastengren, A., Ilavsky, J., Viera, Juan Pablo, Payri, Raul, Duke, D. J., Swantek, A., Tilocco, F. Zak, Sovis, N., and Powell, C. F. Measurements of droplet size in shear-driven atomization using ultra-small angle x-ray scattering. United States: N. p., 2017. Web. doi:10.1016/j.ijmultiphaseflow.2017.03.005.
Kastengren, A., Ilavsky, J., Viera, Juan Pablo, Payri, Raul, Duke, D. J., Swantek, A., Tilocco, F. Zak, Sovis, N., & Powell, C. F. Measurements of droplet size in shear-driven atomization using ultra-small angle x-ray scattering. United States. https://doi.org/10.1016/j.ijmultiphaseflow.2017.03.005
Kastengren, A., Ilavsky, J., Viera, Juan Pablo, Payri, Raul, Duke, D. J., Swantek, A., Tilocco, F. Zak, Sovis, N., and Powell, C. F. Thu . "Measurements of droplet size in shear-driven atomization using ultra-small angle x-ray scattering". United States. https://doi.org/10.1016/j.ijmultiphaseflow.2017.03.005. https://www.osti.gov/servlets/purl/1373736.
@article{osti_1373736,
title = {Measurements of droplet size in shear-driven atomization using ultra-small angle x-ray scattering},
author = {Kastengren, A. and Ilavsky, J. and Viera, Juan Pablo and Payri, Raul and Duke, D. J. and Swantek, A. and Tilocco, F. Zak and Sovis, N. and Powell, C. F.},
abstractNote = {Measurements of droplet size in optically-thick, non-evaporating, shear-driven sprays have been made using ultra-small angle x-ray scattering (USAXS). The sprays are produced by orifice-type nozzles coupled to diesel injectors, with measurements conducted from 1 – 24 mm from the orifice, spanning from the optically-dense near-nozzle region to more dilute regions where optical diagnostics are feasible. The influence of nozzle diameter, liquid injection pressure, and ambient density were examined. The USAXS measurements reveal few if any nanoscale droplets, in conflict with a popular computational model of diesel spray breakup. The average droplet diameter rapidly decreases with downstream distance from the nozzle until a plateau value is reached, after which only small changes are seen in droplet diameter. This plateau droplet size is consistent with the droplets being small enough to be stable with respect to further breakup. As a result, liquid injection pressure and nozzle diameter have the biggest impact on droplet size, while ambient density has a smaller effect.},
doi = {10.1016/j.ijmultiphaseflow.2017.03.005},
journal = {International Journal of Multiphase Flow},
number = C,
volume = 92,
place = {United States},
year = {Thu Mar 16 00:00:00 EDT 2017},
month = {Thu Mar 16 00:00:00 EDT 2017}
}

Journal Article:

Citation Metrics:
Cited by: 42 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Modeling Spray Atomization with the Kelvin-Helmholtz/Rayleigh-Taylor Hybrid Model
journal, January 1999


Droplet size and morphology characterization for dense sprays by image processing: application to the Diesel spray
journal, September 2005


Tailless X‐Ray Single‐Crystal Reflection Curves Obtained by Multiple Reflection
journal, November 1965

  • Bonse, U.; Hart, M.
  • Applied Physics Letters, Vol. 7, Issue 9
  • DOI: 10.1063/1.1754396

Acetic Acid Catalyzed Carbon Aerogels
journal, January 2003

  • Brandt, R.; Petricevic, R.; Pröbstle, H.
  • Journal of Porous Materials, Vol. 10, Issue 3, p. 171-178
  • DOI: 10.1023/A:1027486401135

Large Eddy Simulation of High Reynolds Number Nonreacting and Reacting JP-8 Sprays in a Constant Pressure Flow Vessel With a Detailed Chemistry Approach
journal, March 2016

  • Bravo, Luis; Wijeyakulasuriya, Sameera; Pomraning, Eric
  • Journal of Energy Resources Technology, Vol. 138, Issue 3
  • DOI: 10.1115/1.4032901

Microscopic imaging of the initial stage of diesel spray formation
journal, October 2015


Mechanistic Assessment of Swirl Coaxial Injection by Quantitative X-Ray Radiography
journal, July 2014

  • Eberhart, Chad J.; Lineberry, David M.; Frederick, Robert A.
  • Journal of Propulsion and Power, Vol. 30, Issue 4
  • DOI: 10.2514/1.B35007

Influence of Nozzle Sac Volume on Diesel Spray Droplet Sizes
journal, November 1992

  • Farrar-Khan, J. R.; Andrews, G. E.; Williams, P. T.
  • Proceedings of the Institution of Mechanical Engineers, Part A: Journal of Power and Energy, Vol. 206, Issue 4
  • DOI: 10.1243/PIME_PROC_1992_206_040_02

Analysis of diesel spray dynamics using a compressible Eulerian/VOF/LES model and microscopic shadowgraphy
journal, January 2017


Small-angle X-ray studies of soot inception and growth
journal, November 2001

  • Hessler, Jan P.; Seifert, Soenke; Winans, Randall E.
  • Faraday Discussions, Vol. 119, Issue 1
  • DOI: 10.1039/b102822g

Irena : tool suite for modeling and analysis of small-angle scattering
journal, February 2009


Ultra-small-angle X-ray scattering at the Advanced Photon Source
journal, April 2009

  • Ilavsky, Jan; Jemian, Pete R.; Allen, Andrew J.
  • Journal of Applied Crystallography, Vol. 42, Issue 3
  • DOI: 10.1107/S0021889809008802

Ultra-Small-Angle X-ray Scattering Instrument at the Advanced Photon Source: History, Recent Development, and Current Status
journal, October 2012

  • Ilavsky, J.; Zhang, F.; Allen, A. J.
  • Metallurgical and Materials Transactions A, Vol. 44, Issue 1
  • DOI: 10.1007/s11661-012-1431-y

Silicon photodiode detector for small-angle X-ray scattering
journal, October 1990


Structure of Flame-Made Silica Nanoparticles by Ultra-Small-Angle X-ray Scattering
journal, March 2004

  • Kammler, Hendrik K.; Beaucage, Gregory; Mueller, Roger
  • Langmuir, Vol. 20, Issue 5
  • DOI: 10.1021/la030155v

The 7BM beamline at the APS: a facility for time-resolved fluid dynamics measurements
journal, May 2012

  • Kastengren, Alan; Powell, Christopher F.; Arms, Dohn
  • Journal of Synchrotron Radiation, Vol. 19, Issue 4
  • DOI: 10.1107/S0909049512016883

X-Ray Radiography Measurements of Diesel Spray Structure at Engine-Like Ambient Density
journal, January 2009


Time-Resolved X-Ray Radiography of Sprays from Engine Combustion Network Spray a Diesel Injectors
journal, January 2014


Engine Combustion Network (Ecn): Measurements of Nozzle Geometry and Hydraulic Behavior
journal, January 2012


Droplet Sizes and Velocities in a Transient Diesel Fuel Spray
conference, February 1990

  • Koo, Ja-Ye; Martin, Jay K.
  • International Congress & Exposition, SAE Technical Paper Series
  • DOI: 10.4271/900397

Two-Dimensional Droplet size and Volume Fraction Distributions from the Near-Injector Region of High-Pressure Diesel Sprays
journal, January 2006


Just add water: reproducible singly dispersed silver nanoparticle suspensions on-demand
journal, June 2013

  • MacCuspie, Robert I.; Allen, Andrew J.; Martin, Matthew N.
  • Journal of Nanoparticle Research, Vol. 15, Issue 7
  • DOI: 10.1007/s11051-013-1760-9

Spray droplet velocity characterization for convergent nozzles with three different diameters
journal, November 2008


Comparison of Diesel Spray Combustion in Different High-Temperature, High-Pressure Facilities
journal, August 2010

  • Pickett, Lyle M.; Genzale, Caroline L.; Bruneaux, Gilles
  • SAE International Journal of Engines, Vol. 3, Issue 2
  • DOI: 10.4271/2010-01-2106

Comparison of Near-Field Structure and Growth of a Diesel Spray Using Light-Based Optical Microscopy and X-Ray Radiography
journal, April 2014

  • Pickett, Lyle M.; Manin, Julien; Kastengren, Alan
  • SAE International Journal of Engines, Vol. 7, Issue 2
  • DOI: 10.4271/2014-01-1412

Regimes of coalescence and separation in droplet collision
journal, January 1997


Particle Size Distribution Inferred from Small-Angle X-ray Scattering and Transmission Electron Microscopy
journal, January 1999

  • Rieker, Thomas; Hanprasopwattana, Aree; Datye, Abhaya
  • Langmuir, Vol. 15, Issue 2
  • DOI: 10.1021/la9810713

Views on the Structure of Transient Diesel Sprays
journal, January 2000


Parametric Characterization of High-Pressure Diesel Fuel Injection Systems
journal, April 2003

  • Wang, T. -C.; Han, J. -S.; Xie, X. -B.
  • Journal of Engineering for Gas Turbines and Power, Vol. 125, Issue 2
  • DOI: 10.1115/1.1498268

Small angle X-ray scattering measurements probe water nanodroplet evolution under highly non-equilibrium conditions
journal, January 2007

  • Wyslouzil, Barbara E.; Wilemski, Gerald; Strey, Reinhard
  • Physical Chemistry Chemical Physics, Vol. 9, Issue 39
  • DOI: 10.1039/b709363b

Glassy Carbon as an Absolute Intensity Calibration Standard for Small-Angle Scattering
journal, August 2009

  • Zhang, Fan; Ilavsky, Jan; Long, Gabrielle G.
  • Metallurgical and Materials Transactions A, Vol. 41, Issue 5
  • DOI: 10.1007/s11661-009-9950-x

Breakup characteristics of liquid drops in bag regime by a continuous and uniform air jet flow
journal, June 2011


Works referencing / citing this record:

Measurement of Sauter mean diameter in diesel sprays using a scattering–absorption measurement ratio technique
journal, December 2018

  • Martinez, Gabrielle L.; Poursadegh, Farzad; Magnotti, Gina M.
  • International Journal of Engine Research, Vol. 20, Issue 1
  • DOI: 10.1177/1468087418819912

Eulerian CFD modeling of nozzle geometry effects on ECN Sprays A and D: assessment and analysis
journal, October 2019

  • Pandal, Adrian; Garcia-Oliver, Jose M.; Pastor, Jose M.
  • International Journal of Engine Research, Vol. 21, Issue 1
  • DOI: 10.1177/1468087419882500

The effect of fuel on high velocity evaporating fuel sprays: Large-Eddy simulation of Spray A with various fuels
journal, June 2019

  • Kaario, Ossi Tapani; Vuorinen, Ville; Kahila, Heikki
  • International Journal of Engine Research, Vol. 21, Issue 1
  • DOI: 10.1177/1468087419854235

A multispectral, extinction-based diagnostic for drop sizing in optically dense diesel sprays
journal, July 2019

  • Poursadegh, Farzad; Bibik, Oleksandr; Yraguen, Boni
  • International Journal of Engine Research, Vol. 21, Issue 1
  • DOI: 10.1177/1468087419866034

An equilibrium phase spray model for high-pressure fuel injection and engine combustion simulations
journal, November 2017