Perspective: Advanced particle imaging
Abstract
This study discuss, the first ion imaging experiment demonstrating the capability of collecting an image of the photofragments from a unimolecular dissociation event and analyzing that image to obtain the three-dimensional velocity distribution of the fragments, the efficacy and breadth of application of the ion imaging technique have continued to improve and grow. With the addition of velocity mapping, ion/electron centroiding, and slice imaging techniques, the versatility and velocity resolution have been unmatched. Recent improvements in molecular beam, laser, sensor, and computer technology are allowing even more advanced particle imaging experiments, and eventually we can expect multi-mass imaging with co-variance and full coincidence capability on a single shot basis with repetition rates in the kilohertz range. This progress should further enable “complete” experiments—the holy grail of molecular dynamics—where all quantum numbers of reactants and products of a bimolecular scattering event are fully determined and even under our control.
- Authors:
-
- Sandia National Lab. (SNL-CA), Livermore, CA (United States)
- Cornell Univ., Ithaca, NY (United States)
- Radboud Univ. of Nijmegen, Nijmegen (Netherlands)
- Publication Date:
- Research Org.:
- Sandia National Lab. (SNL-CA), Livermore, CA (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1371480
- Alternate Identifier(s):
- OSTI ID: 1361897
- Report Number(s):
- SAND-2017-2410J
Journal ID: ISSN 0021-9606; JCPSA6; 651469
- Grant/Contract Number:
- AC04-94AL85000; KC0301020
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Chemical Physics
- Additional Journal Information:
- Journal Volume: 147; Journal Issue: 1; Journal ID: ISSN 0021-9606
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS
Citation Formats
Chandler, David W., Houston, Paul L., and Parker, David H. Perspective: Advanced particle imaging. United States: N. p., 2017.
Web. doi:10.1063/1.4983623.
Chandler, David W., Houston, Paul L., & Parker, David H. Perspective: Advanced particle imaging. United States. https://doi.org/10.1063/1.4983623
Chandler, David W., Houston, Paul L., and Parker, David H. Fri .
"Perspective: Advanced particle imaging". United States. https://doi.org/10.1063/1.4983623. https://www.osti.gov/servlets/purl/1371480.
@article{osti_1371480,
title = {Perspective: Advanced particle imaging},
author = {Chandler, David W. and Houston, Paul L. and Parker, David H.},
abstractNote = {This study discuss, the first ion imaging experiment demonstrating the capability of collecting an image of the photofragments from a unimolecular dissociation event and analyzing that image to obtain the three-dimensional velocity distribution of the fragments, the efficacy and breadth of application of the ion imaging technique have continued to improve and grow. With the addition of velocity mapping, ion/electron centroiding, and slice imaging techniques, the versatility and velocity resolution have been unmatched. Recent improvements in molecular beam, laser, sensor, and computer technology are allowing even more advanced particle imaging experiments, and eventually we can expect multi-mass imaging with co-variance and full coincidence capability on a single shot basis with repetition rates in the kilohertz range. This progress should further enable “complete” experiments—the holy grail of molecular dynamics—where all quantum numbers of reactants and products of a bimolecular scattering event are fully determined and even under our control.},
doi = {10.1063/1.4983623},
journal = {Journal of Chemical Physics},
number = 1,
volume = 147,
place = {United States},
year = {Fri May 26 00:00:00 EDT 2017},
month = {Fri May 26 00:00:00 EDT 2017}
}
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