Vertically Oriented and Interpenetrating CuSe Nanosheet Films with Open Channels for Flexible All-Solid-State Supercapacitors
Abstract
As a p-type multifunctional semiconductor, CuSe nanostructures show great promise in optoelectronic, sensing, and photocatalytic fields. Although great progress has been achieved, controllable synthesis of CuSe nanosheets (NSs) with a desirable spacial orientation and open frameworks remains a challenge, and their use in supercapacitors (SCs) has not been explored. Herein, a highly vertically oriented and interpenetrating CuSe NS film with open channels is deposited on an Au-coated polyethylene terephthalate substrate. Such CuSe NS films exhibit high specific capacitance (209 F g–1) and can be used as a carbon black- and binder-free electrode to construct flexible, symmetric all-solid-state SCs, using polyvinyl alcohol–LiCl gel as the solid electrolyte. A device fabricated with such CuSe NS films exhibits high volumetric specific capacitance (30.17 mF cm–3), good cycling stability, excellent flexibility, and desirable mechanical stability. The excellent performance of such devices results from the vertically oriented and interpenetrating configuration of CuSe NS building blocks, which can increase the available surface and facilitate the diffusion of electrolyte ions. Moreover, as a prototype for application, three such solid devices in series can be used to light up a red light-emitting diode.
- Authors:
-
- Hohai Univ., Nanjing (China)
- Nanjing Normal Univ. (China)
- Nanjing Normal Univ. (China); Nanjing Univ. (China)
- Nanjing Univ. (China)
- Ames Lab., Ames, IA (United States)
- Publication Date:
- Research Org.:
- Ames Laboratory (AMES), Ames, IA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1368042
- Report Number(s):
- IS-J-9285
Journal ID: ISSN 2470-1343
- Grant/Contract Number:
- 2015B22313; 2016B46014; 21271105; 21541007; 21671106; 61176087; DE-AC02-07CH11358
- Resource Type:
- Accepted Manuscript
- Journal Name:
- ACS Omega
- Additional Journal Information:
- Journal Volume: 2; Journal Issue: 3; Journal ID: ISSN 2470-1343
- Publisher:
- American Chemical Society (ACS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Li, Lingzhi, Gong, Jiangfeng, Liu, Chunyan, Tian, Yazhou, Han, Min, Wang, Qianjin, Hong, Xihao, Ding, Qingping, Zhu, Weihua, and Bao, Jianchun. Vertically Oriented and Interpenetrating CuSe Nanosheet Films with Open Channels for Flexible All-Solid-State Supercapacitors. United States: N. p., 2017.
Web. doi:10.1021/acsomega.6b00535.
Li, Lingzhi, Gong, Jiangfeng, Liu, Chunyan, Tian, Yazhou, Han, Min, Wang, Qianjin, Hong, Xihao, Ding, Qingping, Zhu, Weihua, & Bao, Jianchun. Vertically Oriented and Interpenetrating CuSe Nanosheet Films with Open Channels for Flexible All-Solid-State Supercapacitors. United States. https://doi.org/10.1021/acsomega.6b00535
Li, Lingzhi, Gong, Jiangfeng, Liu, Chunyan, Tian, Yazhou, Han, Min, Wang, Qianjin, Hong, Xihao, Ding, Qingping, Zhu, Weihua, and Bao, Jianchun. Wed .
"Vertically Oriented and Interpenetrating CuSe Nanosheet Films with Open Channels for Flexible All-Solid-State Supercapacitors". United States. https://doi.org/10.1021/acsomega.6b00535. https://www.osti.gov/servlets/purl/1368042.
@article{osti_1368042,
title = {Vertically Oriented and Interpenetrating CuSe Nanosheet Films with Open Channels for Flexible All-Solid-State Supercapacitors},
author = {Li, Lingzhi and Gong, Jiangfeng and Liu, Chunyan and Tian, Yazhou and Han, Min and Wang, Qianjin and Hong, Xihao and Ding, Qingping and Zhu, Weihua and Bao, Jianchun},
abstractNote = {As a p-type multifunctional semiconductor, CuSe nanostructures show great promise in optoelectronic, sensing, and photocatalytic fields. Although great progress has been achieved, controllable synthesis of CuSe nanosheets (NSs) with a desirable spacial orientation and open frameworks remains a challenge, and their use in supercapacitors (SCs) has not been explored. Herein, a highly vertically oriented and interpenetrating CuSe NS film with open channels is deposited on an Au-coated polyethylene terephthalate substrate. Such CuSe NS films exhibit high specific capacitance (209 F g–1) and can be used as a carbon black- and binder-free electrode to construct flexible, symmetric all-solid-state SCs, using polyvinyl alcohol–LiCl gel as the solid electrolyte. A device fabricated with such CuSe NS films exhibits high volumetric specific capacitance (30.17 mF cm–3), good cycling stability, excellent flexibility, and desirable mechanical stability. The excellent performance of such devices results from the vertically oriented and interpenetrating configuration of CuSe NS building blocks, which can increase the available surface and facilitate the diffusion of electrolyte ions. Moreover, as a prototype for application, three such solid devices in series can be used to light up a red light-emitting diode.},
doi = {10.1021/acsomega.6b00535},
journal = {ACS Omega},
number = 3,
volume = 2,
place = {United States},
year = {Wed Mar 22 00:00:00 EDT 2017},
month = {Wed Mar 22 00:00:00 EDT 2017}
}
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Materials and fabrication of electrode scaffolds for deposition of MnO2 and their true performance in supercapacitors
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Carbon/carbon nanotube-supported RuO2 nanoparticles with a hollow interior as excellent electrode materials for supercapacitors
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Three-Dimensional Network of N-Doped Carbon Ultrathin Nanosheets with Closely Packed Mesopores: Controllable Synthesis and Application in Electrochemical Energy Storage
journal, April 2016
- Zhu, Shan; Li, Jiajun; Ma, Liying
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Study on Thermal Evolution of the CuSe Phase in Nanoparticle-Based Absorber Layers for Solution-Processed Chalcopyrite Photovoltaic Devices
journal, July 2013
- Seo, Yeong-Hui; Lee, Byung-Seok; Jo, Yejin
- ACS Applied Materials & Interfaces, Vol. 5, Issue 15
Synthesis and Characterization of Hexagonal CuSe Nanotubes by Templating against Trigonal Se Nanotubes
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A Facile and Template-Free Hydrothermal Synthesis of Mn 3 O 4 Nanorods on Graphene Sheets for Supercapacitor Electrodes with Long Cycle Stability
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Metallic Few-Layered VS 2 Ultrathin Nanosheets: High Two-Dimensional Conductivity for In-Plane Supercapacitors
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- Feng, Jun; Sun, Xu; Wu, Changzheng
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Facile Microwave-Assisted Synthesis of Multiphase CuInSe 2 Nanoparticles and Role of Secondary CuSe Phase on Photovoltaic Device Performance
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- Seo, Yeong-Hui; Lee, Byung-Seok; Jo, Yejin
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Printable Thin Film Supercapacitors Using Single-Walled Carbon Nanotubes
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Two-Dimensional Tin Selenide Nanostructures for Flexible All-Solid-State Supercapacitors
journal, March 2014
- Zhang, Chunli; Yin, Huanhuan; Han, Min
- ACS Nano, Vol. 8, Issue 4
Hierarchical MnMoO4/CoMoO4 heterostructured nanowires with enhanced supercapacitor performance
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- Mai, Li-Qiang; Yang, Fan; Zhao, Yun-Long
- Nature Communications, Vol. 2, Issue 1
Scalable synthesis of hierarchically structured carbon nanotube–graphene fibres for capacitive energy storage
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- Yu, Dingshan; Goh, Kunli; Wang, Hong
- Nature Nanotechnology, Vol. 9, Issue 7
Facile Microwave-Assisted Synthesis of Klockmannite CuSe Nanosheets and Their Exceptional Electrical Properties
journal, August 2014
- Liu, Yong-Qiang; Wang, Feng-Xia; Xiao, Yan
- Scientific Reports, Vol. 4, Issue 1
Microwave-assisted elemental direct reaction route to nanocrystalline copper chalcogenides CuSe and Cu2TeElectronic supplementary information (ESI) available: XPS spectra of the products. See http://www.rsc.org/suppdata/jm/b2/b205558a/
journal, August 2002
- Zhang, Yong; Qiao, Zheng-Ping; Chen, Xiao-Ming
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Thin film CdSe/CuSe photovoltaic on a flexible single walled carbon nanotube substrate
journal, January 2013
- Hamilton, Christopher E.; Flood, Dennis J.; Barron, Andrew R.
- Physical Chemistry Chemical Physics, Vol. 15, Issue 11
Hydrothermal synthesis of hexagonal CuSe nanoflakes with excellent sunlight-driven photocatalytic activity
journal, January 2014
- Gu, Yanjie; Su, Yanjie; Chen, Da
- CrystEngComm, Vol. 16, Issue 39
Three-dimensional graphene materials: preparation, structures and application in supercapacitors
journal, January 2014
- Cao, Xiehong; Yin, Zongyou; Zhang, Hua
- Energy Environ. Sci., Vol. 7, Issue 6
Directly deposited MoS 2 thin film electrodes for high performance supercapacitors
journal, January 2015
- Choudhary, Nitin; Patel, Mumukshu; Ho, Yee-Hsien
- Journal of Materials Chemistry A, Vol. 3, Issue 47
Carbon-Based Supercapacitors Produced by Activation of Graphene
journal, May 2011
- Zhu, Y.; Murali, S.; Stoller, M. D.
- Science, Vol. 332, Issue 6037, p. 1537-1541
Graphene, related two-dimensional crystals, and hybrid systems for energy conversion and storage
journal, January 2015
- Bonaccorso, Francesco; Colombo, Luigi; Yu, Guihua
- Science, Vol. 347, Issue 6217
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