Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4
Abstract
A quantum spin liquid (QSL) is an exotic state of matter in which electrons’ spins are quantum entangled over long distances, but do not show magnetic order in the zero-temperature limit. The observation of QSL states is a central aim of experimental physics, because they host collective excitations that transcend our knowledge of quantum matter; however, examples in real materials are scarce. We report neutron-scattering experiments on YbMgGaO4, a QSL candidate in which Yb3+ ions with effective spin-1/2 occupy a triangular lattice. Furthermore, our measurements reveal a continuum of magnetic excitations—the essential experimental hallmark of a QSL7—at very low temperature (0.06 K). The origin of this peculiar excitation spectrum is a crucial question, because isotropic nearest-neighbour interactions do not yield a QSL ground state on the triangular lattice. In using measurements the field-polarized state, we identify antiferromagnetic next-nearest-neighbour interactions spin-space anisotropies and chemical disorder between the magnetic layers as key ingredients in YbMgGaO4.
- Authors:
-
- Georgia Inst. of Technology, Atlanta, GA (United States). School of Physics
- Univ. of Tennessee, Knoxville, TN (United States). Dept. of Physics and Astronomy
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Quantum Condensed Matter Division
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Spallation Neutron Source (SNS)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)
- OSTI Identifier:
- 1361300
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Physics
- Additional Journal Information:
- Journal Volume: 13; Journal Issue: 2; Journal ID: ISSN 1745-2473
- Publisher:
- Nature Publishing Group (NPG)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; electronic properties and materials; magnetic properties and materials; quantum fluids and solids
Citation Formats
Paddison, Joseph A. M., Daum, Marcus, Dun, Zhiling, Ehlers, Georg, Liu, Yaohua, Stone, Matthew B., Zhou, Haidong, and Mourigal, Martin. Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4. United States: N. p., 2016.
Web. doi:10.1038/nphys3971.
Paddison, Joseph A. M., Daum, Marcus, Dun, Zhiling, Ehlers, Georg, Liu, Yaohua, Stone, Matthew B., Zhou, Haidong, & Mourigal, Martin. Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4. United States. https://doi.org/10.1038/nphys3971
Paddison, Joseph A. M., Daum, Marcus, Dun, Zhiling, Ehlers, Georg, Liu, Yaohua, Stone, Matthew B., Zhou, Haidong, and Mourigal, Martin. Mon .
"Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4". United States. https://doi.org/10.1038/nphys3971. https://www.osti.gov/servlets/purl/1361300.
@article{osti_1361300,
title = {Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4},
author = {Paddison, Joseph A. M. and Daum, Marcus and Dun, Zhiling and Ehlers, Georg and Liu, Yaohua and Stone, Matthew B. and Zhou, Haidong and Mourigal, Martin},
abstractNote = {A quantum spin liquid (QSL) is an exotic state of matter in which electrons’ spins are quantum entangled over long distances, but do not show magnetic order in the zero-temperature limit. The observation of QSL states is a central aim of experimental physics, because they host collective excitations that transcend our knowledge of quantum matter; however, examples in real materials are scarce. We report neutron-scattering experiments on YbMgGaO4, a QSL candidate in which Yb3+ ions with effective spin-1/2 occupy a triangular lattice. Furthermore, our measurements reveal a continuum of magnetic excitations—the essential experimental hallmark of a QSL7—at very low temperature (0.06 K). The origin of this peculiar excitation spectrum is a crucial question, because isotropic nearest-neighbour interactions do not yield a QSL ground state on the triangular lattice. In using measurements the field-polarized state, we identify antiferromagnetic next-nearest-neighbour interactions spin-space anisotropies and chemical disorder between the magnetic layers as key ingredients in YbMgGaO4.},
doi = {10.1038/nphys3971},
journal = {Nature Physics},
number = 2,
volume = 13,
place = {United States},
year = {Mon Dec 05 00:00:00 EST 2016},
month = {Mon Dec 05 00:00:00 EST 2016}
}
Web of Science
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- arXiv
Intertwined dipolar and multipolar order in the triangular-lattice magnet TmMgGaO$_4$
text, January 2018
- Shen, Yao; Liu, Changle; Qin, Yayuan
- arXiv
Anisotropic-Exchange Magnets on a Triangular Lattice: Spin Waves, Accidental Degeneracies, and Dual Spin Liquids
text, January 2018
- Maksimov, P. A.; Zhu, Zhenyue; White, Steven R.
- arXiv
Experimental signatures of a three-dimensional quantum spin liquid in effective spin-1/2 Ce2Zr2O7 pyrochlore
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- Gao, Bin; Chen, Tong; Tam, David W.
- arXiv
Quantum magnetisms in uniform triangular lattices Li2AMo3O8 (A = In, Sc)
text, January 2019
- Iida, K.; Yoshida, H.; Okabe, H.
- arXiv
Kondo screening in a charge-insulating spinon metal
text, January 2019
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- arXiv
Neural Gutzwiller-projected variational wave functions
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- arXiv
Nature of the randomness-induced quantum spin liquids in two dimensions
text, January 2019
- Kawamura, Hikaru; Uematsu, Kazuki
- arXiv
Novel Excitations near Quantum Criticality in Geometrically Frustrated Antiferromagnet CsFeCl$_{3}$
preprint, January 2019
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- arXiv
A quantum liquid of magnetic octupoles on the pyrochlore lattice
text, January 2019
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- arXiv
Frustrated Magnetism in Triangular Lattice TlYbS$_2$ Crystals Grown via Molten Flux
text, January 2020
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- arXiv
Quantum-disordered state of magnetic and electric dipoles in an organic Mott system
journal, November 2017
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Quasi-continuous transition from a Fermi liquid to a spin liquid in κ-(ET)2Cu2(CN)3
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Author Correction: The nature of spin excitations in the one-third magnetization plateau phase of Ba3CoSb2O9
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Intertwined dipolar and multipolar order in the triangular-lattice magnet TmMgGaO4
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Quantum-disordered state of magnetic and electric dipoles in a hydrogen-bonded Mott system
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- arXiv
Quantum magnetisms in uniform triangular lattices Li2AMo3O8 (A = In, Sc)
text, January 2019
- Iida, K.; Yoshida, H.; Okabe, H.
- arXiv