Orientation-resolved domain mapping in tetragonal using polarized Raman spectroscopy
Abstract
Here, we present microscopically resolved, polarized spectroscopy of Raman scattering collected from tetragonal SrTiO3. The anisotropic response of first-order Raman peaks within a single tetragonal domain has been measured. From these data, we assign symmetries to the phonons seen in the first-order Raman spectrum which is normally complicated by uncontrolled domain structure. Using a translation stage, we map the local domain orientation of a 3–μm3 crystal volume near the laser focus and compare it to wide-field polarized images. This technique can be performed with readily available instruments and is relevant to the study of a wide range of related materials, interfaces, and devices.
- Authors:
-
- Stanford Univ., Stanford, CA (United States)
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Stanford Univ., Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1361076
- Alternate Identifier(s):
- OSTI ID: 1336852
- Grant/Contract Number:
- N66001-11-1-4106; AC02-76SF00515; DGE-114747
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review B
- Additional Journal Information:
- Journal Volume: 94; Journal Issue: 21; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Gray, Jr., Dodd J., Merz, Tyler A., Hikita, Yasuyuki, Hwang, Harold Y., and Mabuchi, Hideo. Orientation-resolved domain mapping in tetragonal SrTiO3 using polarized Raman spectroscopy. United States: N. p., 2016.
Web. doi:10.1103/PhysRevB.94.214107.
Gray, Jr., Dodd J., Merz, Tyler A., Hikita, Yasuyuki, Hwang, Harold Y., & Mabuchi, Hideo. Orientation-resolved domain mapping in tetragonal SrTiO3 using polarized Raman spectroscopy. United States. https://doi.org/10.1103/PhysRevB.94.214107
Gray, Jr., Dodd J., Merz, Tyler A., Hikita, Yasuyuki, Hwang, Harold Y., and Mabuchi, Hideo. Fri .
"Orientation-resolved domain mapping in tetragonal SrTiO3 using polarized Raman spectroscopy". United States. https://doi.org/10.1103/PhysRevB.94.214107. https://www.osti.gov/servlets/purl/1361076.
@article{osti_1361076,
title = {Orientation-resolved domain mapping in tetragonal SrTiO3 using polarized Raman spectroscopy},
author = {Gray, Jr., Dodd J. and Merz, Tyler A. and Hikita, Yasuyuki and Hwang, Harold Y. and Mabuchi, Hideo},
abstractNote = {Here, we present microscopically resolved, polarized spectroscopy of Raman scattering collected from tetragonal SrTiO3. The anisotropic response of first-order Raman peaks within a single tetragonal domain has been measured. From these data, we assign symmetries to the phonons seen in the first-order Raman spectrum which is normally complicated by uncontrolled domain structure. Using a translation stage, we map the local domain orientation of a 3–μm3 crystal volume near the laser focus and compare it to wide-field polarized images. This technique can be performed with readily available instruments and is relevant to the study of a wide range of related materials, interfaces, and devices.},
doi = {10.1103/PhysRevB.94.214107},
journal = {Physical Review B},
number = 21,
volume = 94,
place = {United States},
year = {Fri Dec 16 00:00:00 EST 2016},
month = {Fri Dec 16 00:00:00 EST 2016}
}
Web of Science
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Works referencing / citing this record:
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