Ultrafast X-ray diffraction probe of terahertz field-driven soft mode dynamics in SrTiO3

Kozina, M.; van Driel, T.; Chollet, M.; Sato, T.; Glownia, J. M.; Wandel, S.; Radovic, M.; Staub, U.; Hoffmann, M. C.

doi:10.1063/1.4983153

Title: Ultrafast X-ray diffraction probe of terahertz field-driven soft mode dynamics in SrTiO₃

Abstract

We use ultrafast x-ray pulses to characterize the lattice response of SrTiO₃ when driven by strong terahertz (THz) fields. We observe transient changes in the diffraction intensity with a delayed onset with respect to the driving field. Fourier analysis reveals two frequency components corresponding to the two lowest energy zone-center optical modes in SrTiO₃. Lastly, the lower frequency mode exhibits clear softening as the temperature is decreased while the higher frequency mode shows slight temperature dependence.

Authors:

Kozina, M. ^[1]; van Driel, T. ^[1]; Chollet, M. ^[1]; Sato, T. ^[1]; Glownia, J. M. ^[1]; Wandel, S. ^[1]; Radovic, M. ^[2]; Staub, U. ^[2]; Hoffmann, M. C. ^[1]

SLAC National Accelerator Lab., Menlo Park, CA (United States)
Paul Scherrer Inst. (PSI), Villigen (Switzerland)

Publication Date:: Wed May 03 00:00:00 EDT 2017

Research Org.:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1353203

Grant/Contract Number:: AC02-76SF00515

Resource Type:: Accepted Manuscript

Journal Name:: Structural Dynamics

Additional Journal Information:: Journal Volume: 4; Journal Issue: 5; Journal ID: ISSN 2329-7778

Publisher:: American Crystallographic Association/AIP

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE

Citation Formats


                    Kozina, M., van Driel, T., Chollet, M., Sato, T., Glownia, J. M., Wandel, S., Radovic, M., Staub, U., and Hoffmann, M. C. Ultrafast X-ray diffraction probe of terahertz field-driven soft mode dynamics in SrTiO3.  United States: N. p., 2017. 
Web.  doi:10.1063/1.4983153.

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                    Kozina, M., van Driel, T., Chollet, M., Sato, T., Glownia, J. M., Wandel, S., Radovic, M., Staub, U., & Hoffmann, M. C. Ultrafast X-ray diffraction probe of terahertz field-driven soft mode dynamics in SrTiO3.  United States.  https://doi.org/10.1063/1.4983153

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                    Kozina, M., van Driel, T., Chollet, M., Sato, T., Glownia, J. M., Wandel, S., Radovic, M., Staub, U., and Hoffmann, M. C. Wed .  
"Ultrafast X-ray diffraction probe of terahertz field-driven soft mode dynamics in SrTiO3".  United States.  https://doi.org/10.1063/1.4983153.  https://www.osti.gov/servlets/purl/1353203.

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@article{osti_1353203,

  title        = {Ultrafast X-ray diffraction probe of terahertz field-driven soft mode dynamics in SrTiO3},

  author       = {Kozina, M. and van Driel, T. and Chollet, M. and Sato, T. and Glownia, J. M. and Wandel, S. and Radovic, M. and Staub, U. and Hoffmann, M. C.},

  abstractNote = {We use ultrafast x-ray pulses to characterize the lattice response of SrTiO3 when driven by strong terahertz (THz) fields. We observe transient changes in the diffraction intensity with a delayed onset with respect to the driving field. Fourier analysis reveals two frequency components corresponding to the two lowest energy zone-center optical modes in SrTiO3. Lastly, the lower frequency mode exhibits clear softening as the temperature is decreased while the higher frequency mode shows slight temperature dependence.},

  doi          = {10.1063/1.4983153},

  journal      = {Structural Dynamics},

  number       = 5,

  volume       = 4,

  place        = {United States},

  year         = {Wed May 03 00:00:00 EDT 2017},

  month        = {Wed May 03 00:00:00 EDT 2017}

}

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Works referencing / citing this record:

Terahertz-driven phonon upconversion in SrTiO3
journal, January 2019

Kozina, M.; Fechner, M.; Marsik, P.
Nature Physics, Vol. 15, Issue 4
DOI: 10.1038/s41567-018-0408-1

Watching ultrafast responses of structure and magnetism in condensed matter with momentum-resolved probes
journal, November 2017

Johnson, S. L.; Savoini, M.; Beaud, P.
Structural Dynamics, Vol. 4, Issue 6
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Perspective: Opportunities for ultrafast science at SwissFEL
journal, November 2017

Abela, Rafael; Beaud, Paul; van Bokhoven, Jeroen A.
Structural Dynamics, Vol. 4, Issue 6
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Perspective: Terahertz science and technology
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Mittleman, Daniel M.
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Soft-mode driven polarity reversal in ferroelectrics mapped by ultrafast x-ray diffraction
journal, March 2018

Hauf, Christoph; Hernandez Salvador, Antonio-Andres; Holtz, Marcel
Structural Dynamics, Vol. 5, Issue 2
DOI: 10.1063/1.5026494

Phonon driven charge dynamics in polycrystalline acetylsalicylic acid mapped by ultrafast x-ray diffraction
journal, January 2019

Hauf, Christoph; Hernandez Salvador, Antonio-Andres; Holtz, Marcel
Structural Dynamics, Vol. 6, Issue 1
DOI: 10.1063/1.5079229

Non-thermal fluence threshold for femtosecond pulsed x-ray radiation damage in perovskite complex oxide epitaxial heterostructures
journal, December 2019

Lee, Hyeon Jun; Ahn, Youngjun; Marks, Samuel D.
Applied Physics Letters, Vol. 115, Issue 25
DOI: 10.1063/1.5128509

Infrared lattice dynamics in negative thermal expansion material in single-crystal ScF ₃
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Handunkanda, Sahan U.; Curry, Erin B.; Voronov, Vladimir
Journal of Physics: Condensed Matter, Vol. 32, Issue 3
DOI: 10.1088/1361-648x/ab4955

Experimental station Bernina at SwissFEL: condensed matter physics on femtosecond time scales investigated by X-ray diffraction and spectroscopic methods
journal, April 2019

Ingold, Gerhard; Abela, Rafael; Arrell, Christopher
Journal of Synchrotron Radiation, Vol. 26, Issue 3
DOI: 10.1107/s160057751900331x

Scientific instrument Femtosecond X-ray Experiments (FXE): instrumentation and baseline experimental capabilities
journal, August 2019

Galler, Andreas; Gawelda, Wojciech; Biednov, Mykola
Journal of Synchrotron Radiation, Vol. 26, Issue 5
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Perspective: Opportunities for ultrafast science at SwissFEL
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Abela, Rafael; Beaud, Paul; Van Bokhoven, Jeroen A.
AIP Publishing
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Watching ultrafast responses of structure and magnetism in condensed matter with momentum-resolved probes
text, January 2017

Johnson, Steven L.; Savoini, Matteo; Beaud, Paul
ETH Zurich
DOI: 10.3929/ethz-b-000228313

Watching ultrafast responses of structure and magnetism in condensed matter with momentum-resolved probes
text, January 2017

Johnson, S. L.; Savoini, M.; Beaud, P.
American Institute of Physics
DOI: 10.5167/uzh-145478

Perspective: Opportunities for ultrafast science at SwissFEL
text, January 2017

Abela, Rafael; Beaud, Paul; Van Bokhoven, Jeroen A.
ETH Zurich
DOI: 10.3929/ethz-b-000231826

Terahertz-Driven Phonon Upconversion in SrTiO3
text, January 2018

Kozina, Michael; Fechner, Michael; Marsik, Premysl
arXiv
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Soft-mode driven polarity reversal in ferroelectrics mapped by ultrafast x-ray diffraction
journal, March 2018

Hauf, Christoph; Hernandez Salvador, Antonio-Andres; Holtz, Marcel
Structural Dynamics, Vol. 5, Issue 2
DOI: 10.1063/1.5026494

Phonon driven charge dynamics in polycrystalline acetylsalicylic acid mapped by ultrafast x-ray diffraction
journal, January 2019

Hauf, Christoph; Hernandez Salvador, Antonio-Andres; Holtz, Marcel
Structural Dynamics, Vol. 6, Issue 1
DOI: 10.1063/1.5079229

Perspective: Opportunities for ultrafast science at SwissFEL
text, January 2017

Abela, Rafael; Beaud, Paul; Van Bokhoven, Jeroen A.
ETH Zurich
DOI: 10.3929/ethz-b-000231826

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Title: Ultrafast X-ray diffraction probe of terahertz field-driven soft mode dynamics in SrTiO3

Abstract

Citation Formats

Effect of quantum fluctuations on structural phase transitions in SrTiO 3 and BaTiO 3 journal, March 1996

Time-Domain Terahertz Spectroscopy of (100) (LaAlO3)0.3-(Sr2AlTaO6)0.7 Substrate journal, January 2001

Coherent terahertz control of antiferromagnetic spin waves journal, November 2010

Optical properties of 4-N,N-dimethylamino-4^′-N^′-methyl-stilbazolium 2,4,6-trimethylbenzenesulfonate crystals at terahertz frequencies journal, January 2008

Local terahertz field enhancement for time-resolved x-ray diffraction journal, February 2017

CSPAD-140k: A versatile detector for LCLS experiments journal, August 2013

Optical constants, band gap, and infrared-active phonons of (LaAlO 3 ) 0.3 (Sr 2 AlTaO 6 ) 0.35 (LSAT) from spectroscopic ellipsometry journal, September 2016

Lattice Dynamics and Phase Transitions of Strontium Titanate journal, May 1964

Femtosecond X-ray measurement of coherent lattice vibrations near the Lindemann stability limit journal, March 2003

Combining THz laser excitation with resonant soft X-ray scattering at the Linac Coherent Light Source journal, April 2015

Origin of ferroelectricity in perovskite oxides journal, July 1992

Ultrafast terahertz-field-driven ionic response in ferroelectric BaTiO 3 journal, November 2016

Enhanced coherent oscillations in the superconducting state of underdoped YB a 2 C u 3 O 6 + x induced via ultrafast terahertz excitation journal, June 2015

Collective Coherent Control: Synchronization of Polarization in Ferroelectric PbTiO 3 by Shaped THz Fields journal, June 2009

Ferroelectric Soft Mode in a SrTiO 3 Thin Film Impulsively Driven to the Anharmonic Regime Using Intense Picosecond Terahertz Pulses journal, February 2012

Terahertz-Field-Induced Large Macroscopic Polarization and Domain-Wall Dynamics in an Organic Molecular Dielectric journal, March 2017

Spectral encoding of x-ray/optical relative delay journal, January 2011

Terahertz ellipsometry study of the soft mode behavior in ultrathin SrTiO 3 films journal, February 2016

Experimental determination of the interatomic potential in LiNbO 3 via ultrafast lattice control journal, April 2017

SrTi O 3 : An intrinsic quantum paraelectric below 4 K journal, April 1979

Hyper-Raman spectra and frequency dependence of soft mode damping in SrTiO3 journal, August 1983

Polar phonons in some compressively stressed epitaxial and polycrystalline SrTiO3 thin films journal, April 2008

Ultrafast Terahertz Gating of the Polarization and Giant Nonlinear Optical Response in BiFeO 3 Thin Films journal, September 2015

Tracking the motion of charges in a terahertz light field by femtosecond X-ray diffraction journal, August 2006

Resonant and nonresonant control over matter and light by intense terahertz transients journal, August 2013

Intense terahertz radiation and their applications journal, August 2016

Large-Amplitude Spin Dynamics Driven by a THz Pulse in Resonance with an Electromagnon journal, March 2014

Structures of the ferroelectric phases of barium titanate journal, March 1993

Terahertz-driven phonon upconversion in SrTiO3 journal, January 2019

Watching ultrafast responses of structure and magnetism in condensed matter with momentum-resolved probes journal, November 2017

Perspective: Opportunities for ultrafast science at SwissFEL journal, November 2017

Perspective: Terahertz science and technology journal, December 2017

Soft-mode driven polarity reversal in ferroelectrics mapped by ultrafast x-ray diffraction journal, March 2018

Phonon driven charge dynamics in polycrystalline acetylsalicylic acid mapped by ultrafast x-ray diffraction journal, January 2019

Non-thermal fluence threshold for femtosecond pulsed x-ray radiation damage in perovskite complex oxide epitaxial heterostructures journal, December 2019

Infrared lattice dynamics in negative thermal expansion material in single-crystal ScF 3 journal, October 2019

Experimental station Bernina at SwissFEL: condensed matter physics on femtosecond time scales investigated by X-ray diffraction and spectroscopic methods journal, April 2019

Scientific instrument Femtosecond X-ray Experiments (FXE): instrumentation and baseline experimental capabilities journal, August 2019

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Watching ultrafast responses of structure and magnetism in condensed matter with momentum-resolved probes text, January 2017

Watching ultrafast responses of structure and magnetism in condensed matter with momentum-resolved probes text, January 2017

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Terahertz-Driven Phonon Upconversion in SrTiO3 text, January 2018

Soft-mode driven polarity reversal in ferroelectrics mapped by ultrafast x-ray diffraction journal, March 2018

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Perspective: Opportunities for ultrafast science at SwissFEL text, January 2017

Title: Ultrafast X-ray diffraction probe of terahertz field-driven soft mode dynamics in SrTiO₃

Effect of quantum fluctuations on structural phase transitions in ${SrTiO}_{3}$ and ${BaTiO}_{3}$
journal, March 1996

Time-Domain Terahertz Spectroscopy of (100) (LaAlO3)0.3-(Sr2AlTaO6)0.7 Substrate
journal, January 2001

Coherent terahertz control of antiferromagnetic spin waves
journal, November 2010

Optical properties of 4-N,N-dimethylamino-4^′-N^′-methyl-stilbazolium 2,4,6-trimethylbenzenesulfonate crystals at terahertz frequencies
journal, January 2008

Local terahertz field enhancement for time-resolved x-ray diffraction
journal, February 2017

CSPAD-140k: A versatile detector for LCLS experiments
journal, August 2013

Optical constants, band gap, and infrared-active phonons of (LaAlO ₃ ) _0.3 (Sr ₂ AlTaO ₆ ) _0.35 (LSAT) from spectroscopic ellipsometry
journal, September 2016

Lattice Dynamics and Phase Transitions of Strontium Titanate
journal, May 1964

Femtosecond X-ray measurement of coherent lattice vibrations near the Lindemann stability limit
journal, March 2003

Combining THz laser excitation with resonant soft X-ray scattering at the Linac Coherent Light Source
journal, April 2015

Origin of ferroelectricity in perovskite oxides
journal, July 1992

Ultrafast terahertz-field-driven ionic response in ferroelectric ${BaTiO}_{3}$
journal, November 2016

Enhanced coherent oscillations in the superconducting state of underdoped $YB a_{2} C u_{3} O_{6 + x}$ induced via ultrafast terahertz excitation
journal, June 2015

Collective Coherent Control: Synchronization of Polarization in Ferroelectric ${PbTiO}_{3}$ by Shaped THz Fields
journal, June 2009

Ferroelectric Soft Mode in a ${SrTiO}_{3}$ Thin Film Impulsively Driven to the Anharmonic Regime Using Intense Picosecond Terahertz Pulses
journal, February 2012

Terahertz-Field-Induced Large Macroscopic Polarization and Domain-Wall Dynamics in an Organic Molecular Dielectric
journal, March 2017

Spectral encoding of x-ray/optical relative delay
journal, January 2011

Terahertz ellipsometry study of the soft mode behavior in ultrathin SrTiO ₃ films
journal, February 2016

Experimental determination of the interatomic potential in LiNbO ₃ via ultrafast lattice control
journal, April 2017

SrTi $O_{3}$ : An intrinsic quantum paraelectric below 4 K
journal, April 1979

Hyper-Raman spectra and frequency dependence of soft mode damping in SrTiO3
journal, August 1983

Polar phonons in some compressively stressed epitaxial and polycrystalline SrTiO3 thin films
journal, April 2008

Ultrafast Terahertz Gating of the Polarization and Giant Nonlinear Optical Response in BiFeO ₃ Thin Films
journal, September 2015

Tracking the motion of charges in a terahertz light field by femtosecond X-ray diffraction
journal, August 2006

Resonant and nonresonant control over matter and light by intense terahertz transients
journal, August 2013

Intense terahertz radiation and their applications
journal, August 2016

Large-Amplitude Spin Dynamics Driven by a THz Pulse in Resonance with an Electromagnon
journal, March 2014

Structures of the ferroelectric phases of barium titanate
journal, March 1993

Terahertz-driven phonon upconversion in SrTiO3
journal, January 2019

Watching ultrafast responses of structure and magnetism in condensed matter with momentum-resolved probes
journal, November 2017

Perspective: Opportunities for ultrafast science at SwissFEL
journal, November 2017

Perspective: Terahertz science and technology
journal, December 2017

Soft-mode driven polarity reversal in ferroelectrics mapped by ultrafast x-ray diffraction
journal, March 2018

Phonon driven charge dynamics in polycrystalline acetylsalicylic acid mapped by ultrafast x-ray diffraction
journal, January 2019

Non-thermal fluence threshold for femtosecond pulsed x-ray radiation damage in perovskite complex oxide epitaxial heterostructures
journal, December 2019

Infrared lattice dynamics in negative thermal expansion material in single-crystal ScF ₃
journal, October 2019

Experimental station Bernina at SwissFEL: condensed matter physics on femtosecond time scales investigated by X-ray diffraction and spectroscopic methods
journal, April 2019

Scientific instrument Femtosecond X-ray Experiments (FXE): instrumentation and baseline experimental capabilities
journal, August 2019

Perspective: Opportunities for ultrafast science at SwissFEL
text, January 2017

Watching ultrafast responses of structure and magnetism in condensed matter with momentum-resolved probes
text, January 2017

Watching ultrafast responses of structure and magnetism in condensed matter with momentum-resolved probes
text, January 2017

Perspective: Opportunities for ultrafast science at SwissFEL
text, January 2017

Terahertz-Driven Phonon Upconversion in SrTiO3
text, January 2018

Soft-mode driven polarity reversal in ferroelectrics mapped by ultrafast x-ray diffraction
journal, March 2018

Phonon driven charge dynamics in polycrystalline acetylsalicylic acid mapped by ultrafast x-ray diffraction
journal, January 2019

Perspective: Opportunities for ultrafast science at SwissFEL
text, January 2017