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Title: Energies and densities of electrons confined in elliptical and ellipsoidal quantum dots

Abstract

Here, we consider a droplet of electrons confined within an external harmonic potential well of elliptical or ellipsoidal shape, a geometry commonly encountered in work with semiconductor quantum dots and other nanoscale or mesoscale structures. For droplet sizes exceeding the effective Bohr radius, the dominant contribution to average system parameters in the Thomas– Fermi approximation comes from the potential energy terms, which allows us to derive expressions describing the electron droplet’s shape and dimensions, its density, total and capacitive energy, and chemical potential. Our analytical results are in very good agreement with experimental data and numerical calculations, and make it possible to follow the dependence of the properties of the system on its parameters (the total number of electrons, the axial ratios and curvatures of the confinement potential, and the dielectric constant of the material). One interesting feature is that the eccentricity of the electron droplet is not the same as that of its confining potential well.

Authors:
 [1];  [2]
  1. Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division; Univ. of Southern California, Los Angeles, CA (United States). Dept. of Physics and Astronomy
  2. Univ. of Southern California, Los Angeles, CA (United States). Dept. of Physics and Astronomy
Publication Date:
Research Org.:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)
OSTI Identifier:
1352650
Alternate Identifier(s):
OSTI ID: 1287745
Grant/Contract Number:  
AC02-06CH11357; AC-02-06CH11357
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Physics. Condensed Matter
Additional Journal Information:
Journal Volume: 28; Journal Issue: 39; Journal ID: ISSN 0953-8984
Publisher:
IOP Publishing
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Thomas–Fermi theory; nanoclusters; quantum dots; self-consistent field

Citation Formats

Halder, Avik, and Kresin, Vitaly V. Energies and densities of electrons confined in elliptical and ellipsoidal quantum dots. United States: N. p., 2016. Web. doi:10.1088/0953-8984/28/39/395302.
Halder, Avik, & Kresin, Vitaly V. Energies and densities of electrons confined in elliptical and ellipsoidal quantum dots. United States. https://doi.org/10.1088/0953-8984/28/39/395302
Halder, Avik, and Kresin, Vitaly V. Tue . "Energies and densities of electrons confined in elliptical and ellipsoidal quantum dots". United States. https://doi.org/10.1088/0953-8984/28/39/395302. https://www.osti.gov/servlets/purl/1352650.
@article{osti_1352650,
title = {Energies and densities of electrons confined in elliptical and ellipsoidal quantum dots},
author = {Halder, Avik and Kresin, Vitaly V.},
abstractNote = {Here, we consider a droplet of electrons confined within an external harmonic potential well of elliptical or ellipsoidal shape, a geometry commonly encountered in work with semiconductor quantum dots and other nanoscale or mesoscale structures. For droplet sizes exceeding the effective Bohr radius, the dominant contribution to average system parameters in the Thomas– Fermi approximation comes from the potential energy terms, which allows us to derive expressions describing the electron droplet’s shape and dimensions, its density, total and capacitive energy, and chemical potential. Our analytical results are in very good agreement with experimental data and numerical calculations, and make it possible to follow the dependence of the properties of the system on its parameters (the total number of electrons, the axial ratios and curvatures of the confinement potential, and the dielectric constant of the material). One interesting feature is that the eccentricity of the electron droplet is not the same as that of its confining potential well.},
doi = {10.1088/0953-8984/28/39/395302},
journal = {Journal of Physics. Condensed Matter},
number = 39,
volume = 28,
place = {United States},
year = {Tue Aug 09 00:00:00 EDT 2016},
month = {Tue Aug 09 00:00:00 EDT 2016}
}

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Cited by: 5 works
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Works referenced in this record:

Few-electron quantum dots
journal, May 2001

  • Kouwenhoven, L. P.; Austing, D. G.; Tarucha, S.
  • Reports on Progress in Physics, Vol. 64, Issue 6
  • DOI: 10.1088/0034-4885/64/6/201

Spectroscopy of Quantum Levels in Charge-Tunable InGaAs Quantum Dots
journal, October 1994


Ellipsoidal deformation of vertical quantum dots
journal, October 1999


Excitation of three-dimensional quantum dots
journal, October 1993


Collective resonances and response properties of electrons in metal clusters
journal, November 1992


Shell-correction method for calculating the binding energy of metal clusters: Application to multiply charged anions
journal, September 1993


Erratum: Thomas-Fermi and related theories of atoms and molecules
journal, January 1982


Large two-dimensional electronic systems: Self-consistent energies and densities at low cost
journal, January 2013


Dynamic response of quantum dots
journal, May 1991


Flat Thomas-Fermi artificial atoms
journal, July 2014


Prediction of quantum dot characteristics through universal scaling relations
journal, August 2014


Electrons Trapped in an Anisotropic Parabolic Potential Well, Thomas-Fermi Approach
journal, February 2008


Elliptical multielectron dimples on liquid and solid helium surfaces
journal, July 1983


Contact Mechanics
book, January 1985


Electronic structures in circular, elliptic, and triangular quantum dots
journal, September 1997


Shell Filling and Spin Effects in a Few Electron Quantum Dot
journal, October 1996


Ellipsoidal shell structure in free-electron metal clusters
journal, July 1985


The physics of simple metal clusters: experimental aspects and simple models
journal, July 1993


The Spectroscopy of Quantum Dot Arrays
journal, June 1993

  • Heitmann, Detlef; Kotthaus, Jörg P.
  • Physics Today, Vol. 46, Issue 6
  • DOI: 10.1063/1.881355

Localization in Artificial Disorder: Two Coupled Quantum Dots
journal, September 2000


Electronic structure of quantum dots
journal, November 2002


Artificial Atoms
journal, January 1993


Capacitive nature of atomic-sized structures
journal, October 1995


Demagnetizing Factors of the General Ellipsoid
journal, June 1945


XCVII. The demagnetizing factors for ellipsoids
journal, December 1945

  • Stoner, Edmund C.
  • The London, Edinburgh, and Dublin Philosophical Magazine and Journal of Science, Vol. 36, Issue 263
  • DOI: 10.1080/14786444508521510

Electronic structure of three-dimensional isotropic quantum dots by four-component relativistic coupled cluster methods
journal, February 2011

  • Yakobi, Hana; Eliav, Ephraim; Kaldor, Uzi
  • The Journal of Chemical Physics, Vol. 134, Issue 5
  • DOI: 10.1063/1.3533778

Shell filling of artificial atoms within density-functional theory
journal, April 1998


Electronic structure of three-dimensional quantum dots
journal, March 2003


Recent Advances in Two-Dimensional Materials beyond Graphene
journal, October 2015


Works referencing / citing this record:

Donor Impurity-Related Optical Absorption in GaAs Elliptic-Shaped Quantum Dots
journal, January 2017

  • Londoño, M. A.; Restrepo, R. L.; Ojeda, J. H.
  • Journal of Nanomaterials, Vol. 2017
  • DOI: 10.1155/2017/5970540