Covalently Bound Clusters of Alpha-Substituted PDI—Rival Electron Acceptors to Fullerene for Organic Solar Cells
Abstract
Here, a cluster type of electron acceptor, TPB, bearing four α-perylenediimides (PDIs), was developed, in which the four PDIs form a cross-like molecular conformation while still partially conjugated with the BDT-Th core. The blend TPB:PTB7-Th films shows favorable morphology and efficient charge dissociation. The inverted solar cells exhibited the highest PCE of 8.47 % with the extraordinary high Jsc values (>18 mA/cm2), comparable with those of the corresponding PC71BM/PBT7-Th based solar cells.
- Authors:
-
- Univ. of Chicago, IL (United States). James Franck Inst., Dept. of Chemistry
- Univ. of Chicago, IL (United States). James Franck Inst., Dept. of Chemistry
- Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division; Univ. of Chicago, IL (United States). Inst. for Molecular Engineering
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1352625
- Grant/Contract Number:
- AC02-06CH11357; DMR-1263006; SC0001059
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of the American Chemical Society
- Additional Journal Information:
- Journal Volume: 138; Journal Issue: 23; Journal ID: ISSN 0002-7863
- Publisher:
- American Chemical Society (ACS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Citation Formats
Wu, Qinghe, Zhao, Donglin, Schneider, Alexander M., Chen, Wei, and Yu, Luping. Covalently Bound Clusters of Alpha-Substituted PDI—Rival Electron Acceptors to Fullerene for Organic Solar Cells. United States: N. p., 2016.
Web. doi:10.1021/jacs.6b03562.
Wu, Qinghe, Zhao, Donglin, Schneider, Alexander M., Chen, Wei, & Yu, Luping. Covalently Bound Clusters of Alpha-Substituted PDI—Rival Electron Acceptors to Fullerene for Organic Solar Cells. United States. https://doi.org/10.1021/jacs.6b03562
Wu, Qinghe, Zhao, Donglin, Schneider, Alexander M., Chen, Wei, and Yu, Luping. Tue .
"Covalently Bound Clusters of Alpha-Substituted PDI—Rival Electron Acceptors to Fullerene for Organic Solar Cells". United States. https://doi.org/10.1021/jacs.6b03562. https://www.osti.gov/servlets/purl/1352625.
@article{osti_1352625,
title = {Covalently Bound Clusters of Alpha-Substituted PDI—Rival Electron Acceptors to Fullerene for Organic Solar Cells},
author = {Wu, Qinghe and Zhao, Donglin and Schneider, Alexander M. and Chen, Wei and Yu, Luping},
abstractNote = {Here, a cluster type of electron acceptor, TPB, bearing four α-perylenediimides (PDIs), was developed, in which the four PDIs form a cross-like molecular conformation while still partially conjugated with the BDT-Th core. The blend TPB:PTB7-Th films shows favorable morphology and efficient charge dissociation. The inverted solar cells exhibited the highest PCE of 8.47 % with the extraordinary high Jsc values (>18 mA/cm2), comparable with those of the corresponding PC71BM/PBT7-Th based solar cells.},
doi = {10.1021/jacs.6b03562},
journal = {Journal of the American Chemical Society},
number = 23,
volume = 138,
place = {United States},
year = {Tue May 24 00:00:00 EDT 2016},
month = {Tue May 24 00:00:00 EDT 2016}
}
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