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Title: Mixed cation FA x PEA 1- x PbI 3 with enhanced phase and ambient stability toward high-performance perovskite solar cells

Abstract

In this study, different from the commonly explored strategy of incorporating a smaller cation, MA+ and Cs+ into FAPbI3 lattice to improve efficiency and stability, it is revealed that the introduction of phenylethylammonium iodide (PEAI) into FAPbI3 perovksite to form mixed cation FAxPEA1–xPbI3 can effectively enhance both phase and ambient stability of FAPbI3 as well as the resulting performance of the derived devices. From our experimental and theoretical calculation results, it is proposed that the larger PEA cation is capable of assembling on both the lattice surface and grain boundaries to form quais-3D perovskite structures. The surrounding of PEA+ ions at the crystal grain boundaries not only can serve as molecular locks to tighten FAPbI3 domains but also passivate the surface defects to improve both phase and moisture stablity. Consequently, a high-performance (PCE:17.7%) and ambient stable FAPbI3 solar cell could be developed

Authors:
 [1];  [2];  [2];  [2];  [2];  [2];  [2];  [3];  [2]
+ Show Author Affiliations
  1. Univ. of Washington, Seattle, WA (United States); Tsinghua Univ., Beijing (China)
  2. Univ. of Washington, Seattle, WA (United States)
  3. Tsinghua Univ., Beijing (China)
Publication Date:
Research Org.:
Univ. of Washington, Seattle, WA (United States)
Sponsoring Org.:
USDOE Office of Energy Efficiency and Renewable Energy (EERE)
Contributing Org.:
This work was supported by the Office of Naval Research (N00014- 14-1-0246), the Asian Office of Aerospace R&D (FA2386-15-1-4106), the Department of Energy SunShot (DE-EE0006710 ) and the National Natural Science Foundation of China under Grant No. 51273104 and 91433205. A.K.-Y.J. thanks the Boeing-Johnson Foundation for financial support. Computations were conducted through the use of advanced computational, storage, and networking infrastructure provided by the Hyak supercomputer system at the University of Washington, funded by the Student Technology Fee. N.L. thanks China Scholarship Council (201506210171) for financial support. Theoretical research is supported by the National Science Foundation (CHE-1464497 and CHE-1565520 to X.L.).
OSTI Identifier:
1343600
Report Number(s):
DOE-UW-Jen-29
Journal ID: ISSN 1614-6832
Grant/Contract Number:  
EE0006710
Resource Type:
Accepted Manuscript
Journal Name:
Advanced Energy Materials
Additional Journal Information:
Journal Volume: 7; Journal Issue: 1; Journal ID: ISSN 1614-6832
Publisher:
Wiley
Country of Publication:
United States
Language:
English
Subject:
14 SOLAR ENERGY; 36 MATERIALS SCIENCE

Citation Formats

Li, Nan, Zhu, Zonglong, Chueh, Chu -Chen, Liu, Hongbin, Peng, Bo, Petrone, Alessio, Li, Xiaosong, Wang, Liduo, and Jen, Alex K. -Y. Mixed cation FA x PEA 1- x PbI 3 with enhanced phase and ambient stability toward high-performance perovskite solar cells. United States: N. p., 2016. Web. doi:10.1002/aenm.201601307.
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Li, Nan, Zhu, Zonglong, Chueh, Chu -Chen, Liu, Hongbin, Peng, Bo, Petrone, Alessio, Li, Xiaosong, Wang, Liduo, & Jen, Alex K. -Y. Mixed cation FA x PEA 1- x PbI 3 with enhanced phase and ambient stability toward high-performance perovskite solar cells. United States. https://doi.org/10.1002/aenm.201601307
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Li, Nan, Zhu, Zonglong, Chueh, Chu -Chen, Liu, Hongbin, Peng, Bo, Petrone, Alessio, Li, Xiaosong, Wang, Liduo, and Jen, Alex K. -Y. Mon . "Mixed cation FA x PEA 1- x PbI 3 with enhanced phase and ambient stability toward high-performance perovskite solar cells". United States. https://doi.org/10.1002/aenm.201601307. https://www.osti.gov/servlets/purl/1343600.
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@article{osti_1343600,
title = {Mixed cation FA x PEA 1- x PbI 3 with enhanced phase and ambient stability toward high-performance perovskite solar cells},
author = {Li, Nan and Zhu, Zonglong and Chueh, Chu -Chen and Liu, Hongbin and Peng, Bo and Petrone, Alessio and Li, Xiaosong and Wang, Liduo and Jen, Alex K. -Y.},
abstractNote = {In this study, different from the commonly explored strategy of incorporating a smaller cation, MA+ and Cs+ into FAPbI3 lattice to improve efficiency and stability, it is revealed that the introduction of phenylethylammonium iodide (PEAI) into FAPbI3 perovksite to form mixed cation FAxPEA1–xPbI3 can effectively enhance both phase and ambient stability of FAPbI3 as well as the resulting performance of the derived devices. From our experimental and theoretical calculation results, it is proposed that the larger PEA cation is capable of assembling on both the lattice surface and grain boundaries to form quais-3D perovskite structures. The surrounding of PEA+ ions at the crystal grain boundaries not only can serve as molecular locks to tighten FAPbI3 domains but also passivate the surface defects to improve both phase and moisture stablity. Consequently, a high-performance (PCE:17.7%) and ambient stable FAPbI3 solar cell could be developed},
doi = {10.1002/aenm.201601307},
journal = {Advanced Energy Materials},
number = 1,
volume = 7,
place = {United States},
year = {Mon Sep 26 00:00:00 EDT 2016},
month = {Mon Sep 26 00:00:00 EDT 2016}
}
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    • Sustainable Energy & Fuels, Vol. 2, Issue 11
    • DOI: 10.1039/c8se00282g

    Narrow band gap and high mobility of lead-free perovskite single crystal Sn-doped MA 3 Sb 2 I 9
    journal, January 2018

    • Ju, Dianxing; Jiang, Xiaomei; Xiao, Hang
    • Journal of Materials Chemistry A, Vol. 6, Issue 42
    • DOI: 10.1039/c8ta08315k

    Stability progress of perovskite solar cells dependent on the crystalline structure: From 3D ABX 3 to 2D Ruddlesden–Popper perovskite absorbers
    journal, January 2019

    • Arabpour Roghabadi, Farzaneh; Alidaei, Maryam; Mousavi, Seyede Maryam
    • Journal of Materials Chemistry A, Vol. 7, Issue 11
    • DOI: 10.1039/c8ta10444a

    Synthesis, post-synthetic modification and stability of a 2D styryl ammonium lead iodide hybrid material
    journal, January 2020

    • Peng, Yong; Albero, Josep; Garcia, Hermenegildo
    • Dalton Transactions, Vol. 49, Issue 2
    • DOI: 10.1039/c9dt04285g

    Orientationally engineered 2D/3D perovskite for high efficiency solar cells
    journal, January 2020

    • Abbas, Muhammad Sohail; Hussain, Sabir; Zhang, Jinaqi
    • Sustainable Energy & Fuels, Vol. 4, Issue 1
    • DOI: 10.1039/c9se00817a

    Self-assembled propylammonium cations at grain boundaries and the film surface to improve the efficiency and stability of perovskite solar cells
    journal, January 2019

    • Fei, Chengbin; Zhou, Meng; Ogle, Jonathan
    • Journal of Materials Chemistry A, Vol. 7, Issue 41
    • DOI: 10.1039/c9ta01755k

    Water in hybrid perovskites: Bulk MAPbI 3 degradation via super-hydrous state
    journal, April 2019

    • Kakekhani, Arvin; Katti, Radhika N.; Rappe, Andrew M.
    • APL Materials, Vol. 7, Issue 4
    • DOI: 10.1063/1.5087290

    Mixed Halide Perovskite Solar Cells: Progress and Challenges
    journal, February 2019

    • Hamed, Mohammed S. G.; Mola, Genene Tessema
    • Critical Reviews in Solid State and Materials Sciences, Vol. 45, Issue 2
    • DOI: 10.1080/10408436.2018.1549976

    Engineering Multiphase Metal Halide Perovskites Thin Films for Stable and Efficient Solar Cells
    text, January 2020

    In Situ Growth of 2D Perovskite Capping Layer for Stable and Efficient Perovskite Solar Cells
    journal, February 2018

    • Chen, Peng; Bai, Yang; Wang, Songcan
    • Advanced Functional Materials, Vol. 28, Issue 17
    • DOI: 10.1002/adfm.201706923

    Precursor Solution Annealing Forms Cubic-Phase Perovskite and Improves Humidity Resistance of Solar Cells
    journal, July 2018

    • Khlyabich, Petr P.; Hamill, J. Clay; Loo, Yueh-Lin
    • Advanced Functional Materials, Vol. 28, Issue 35
    • DOI: 10.1002/adfm.201801508

    Self-Adhesive Macroporous Carbon Electrodes for Efficient and Stable Perovskite Solar Cells
    journal, August 2018

    • Zhang, Huiyin; Xiao, Junyan; Shi, Jiangjian
    • Advanced Functional Materials, Vol. 28, Issue 39
    • DOI: 10.1002/adfm.201802985

    Realizing Efficient Lead-Free Formamidinium Tin Triiodide Perovskite Solar Cells via a Sequential Deposition Route
    journal, December 2017

    Causes and Solutions of Recombination in Perovskite Solar Cells
    journal, September 2018

    Surface‐2D/Bulk‐3D Heterophased Perovskite Nanograins for Long‐Term‐Stable Light‐Emitting Diodes
    journal, November 2019

    • Han, Tae‐Hee; Lee, Jin‐Wook; Choi, Yung Ji
    • Advanced Materials, Vol. 32, Issue 1
    • DOI: 10.1002/adma.201905674

    Surface Electronic Modification of Perovskite Thin Film with Water-Resistant Electron Delocalized Molecules for Stable and Efficient Photovoltaics
    journal, January 2018

    • Wen, Tian Yu; Yang, Shuang; Liu, Peng Fei
    • Advanced Energy Materials, Vol. 8, Issue 13
    • DOI: 10.1002/aenm.201703143

    Low-Dimensional Perovskites: From Synthesis to Stability in Perovskite Solar Cells
    journal, September 2018

    • Yusoff, Abd. Rashid bin Mohd.; Nazeeruddin, Mohammad Khaja
    • Advanced Energy Materials, Vol. 8, Issue 26
    • DOI: 10.1002/aenm.201801726

    Improved Efficiency and Stability of Pb/Sn Binary Perovskite Solar Cells Fabricated by Galvanic Displacement Reaction
    journal, January 2019

    • Zhu, Zonglong; Li, Nan; Zhao, Dongbin
    • Advanced Energy Materials, Vol. 9, Issue 7
    • DOI: 10.1002/aenm.201802774

    2D and Quasi‐2D Halide Perovskites: Applications and Progress
    journal, September 2019

    • Kim, Hyojung; Huynh, Kim Anh; Kim, Soo Young
    • physica status solidi (RRL) – Rapid Research Letters, Vol. 14, Issue 2
    • DOI: 10.1002/pssr.201900435

    Formamidinium-Based Lead Halide Perovskites: Structure, Properties, and Fabrication Methodologies
    journal, May 2018

    Inorganic halide perovskite materials and solar cells
    journal, December 2019

    • Zhang, Cuiling; Arumugam, Gowri Manohari; Liu, Chong
    • APL Materials, Vol. 7, Issue 12
    • DOI: 10.1063/1.5117306

    Interfacial crosslinked quasi-2D perovskite with boosted carrier transport and enhanced stability
    journal, August 2018

    • Zhang, Taiyang; Hui, Yong; Chen, Liang
    • Journal of Physics D: Applied Physics, Vol. 51, Issue 40
    • DOI: 10.1088/1361-6463/aad7de

    An efficient implementation of two-component relativistic density functional theory with torque-free auxiliary variables
    journal, July 2018

    • Petrone, Alessio; Williams-Young, David B.; Sun, Shichao
    • The European Physical Journal B, Vol. 91, Issue 7
    • DOI: 10.1140/epjb/e2018-90170-1

    Imperfections and their passivation in halide perovskite solar cells
    text, January 2019

    • J., Huang,; B., Chen,; P. N., Rudd,
    • The University of North Carolina at Chapel Hill University Libraries
    • DOI: 10.17615/kzq8-3k31

    Attaining High Photovoltaic Efficiency and Stability with Multidimensional Perovskites.
    text, January 2018

    • Kosasih, Felix; Ducati, Caterina
    • Apollo - University of Cambridge Repository
    • DOI: 10.17863/cam.33139

    Effects of Decaphenylcyclopentasilane Addition on Photovoltaic Properties of Perovskite Solar Cells
    journal, December 2018

    Defect and Contact Passivation for Perovskite Solar Cells
    journal, April 2019

    • Aydin, Erkan; Bastiani, Michele; Wolf, Stefaan
    • Advanced Materials, Vol. 31, Issue 25
    • DOI: 10.1002/adma.201900428

    Controlling the Growth Kinetics and Optoelectronic Properties of 2D/3D Lead–Tin Perovskite Heterojunctions
    journal, November 2019

    • Ruggeri, Edoardo; Anaya, Miguel; Gałkowski, Krzysztof
    • Advanced Materials, Vol. 31, Issue 51
    • DOI: 10.1002/adma.201905247

    Alternative Perovskites for Photovoltaics
    journal, April 2018

    • Jodlowski, AlexanderD.; Rodríguez-Padrón, Daily; Luque, Rafael
    • Advanced Energy Materials, Vol. 8, Issue 21
    • DOI: 10.1002/aenm.201703120

    High‐Performance Perovskite Solar Cells with Enhanced Environmental Stability Based on a ( p ‐FC 6 H 4 C 2 H 4 NH 3 ) 2 [PbI 4 ] Capping Layer
    journal, January 2019

    • Zhou, Qin; Liang, Lusheng; Hu, Junjie
    • Advanced Energy Materials, Vol. 9, Issue 12
    • DOI: 10.1002/aenm.201802595

    Engineering Multiphase Metal Halide Perovskites Thin Films for Stable and Efficient Solar Cells
    journal, January 2020

    • Kim, Min; Figueroa‐Tapia, Jetsabel M.; Prato, Mirko
    • Advanced Energy Materials, Vol. 10, Issue 8
    • DOI: 10.1002/aenm.201903221

    Mixed 3D-2D passivation treatment for mixed-cation lead mixed-halide perovskite solar cells for higher efficiency and better stability
    conference, February 2018

    • Cho, Yongyoon; Soufiani, Arman Mahboubi; Yun, Jae Sung
    • Proceedings of the 10th International Conference on Hybrid and Organic Photovoltaics
    • DOI: 10.29363/nanoge.hopv.2018.080

    Design of Mixed‐Cation Tri‐Layered Pb‐Free Halide Perovskites for Optoelectronic Applications
    journal, May 2019

    • Liu, Zhun; Zhao, Xingang; Zunger, Alex
    • Advanced Electronic Materials, Vol. 5, Issue 6
    • DOI: 10.1002/aelm.201900234

    Stable Formamidinium-Based Perovskite Solar Cells via In Situ Grain Encapsulation
    journal, May 2018

    • Liu, Tanghao; Zhou, Yuanyuan; Li, Zhen
    • Advanced Energy Materials, Vol. 8, Issue 22
    • DOI: 10.1002/aenm.201800232

    Controlling the Growth Kinetics and Optoelectronic Properties of 2D/3D Lead–Tin Perovskite Heterojunctions
    text, January 2019

    • Ruggeri, Edoardo; Anaya, Miguel; Gałkowski, Krzysztof
    • Apollo - University of Cambridge Repository
    • DOI: 10.17863/cam.45923

    2D perovskite stabilized phase-pure formamidinium perovskite solar cells
    journal, August 2018

    Mixed-Dimensional Naphthylmethylammonium-Methylammonium Lead Iodide Perovskites with Improved Thermal Stability
    journal, January 2020

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