Roles of Fullerene-Based Interlayers in Enhancing the Performance of Organometal Perovskite Thin-Film Solar Cells
Abstract
Roles of fullerene-based interlayers in enhancing the performance of organometal perovskite thin-film solar cells are elucidated. By studying various fullerenes, a clear correlation between the electron mobility of fullerenes and the resulting performance of derived devices is determined. The metallic characteristics of the bilayer perovskite/fullerene field-effect transistor indicates an effective charge redistribution occurring at the corresponding interface. Lastly, a conventional perovskite thin-film solar cell derived from the C60 electron-transporting layer (ETL) affords a high power conversion efficiency of 15.4%.
- Authors:
-
- Univ. of Washington, Seattle, WA (United States). Dept. of Materials Science and Engineering
- Univ. of Washington, Seattle, WA (United States). Dept. of Materials Science and Engineering; Univ. of Washington, Seattle, WA (United States). Dept. of Chemistry
- Publication Date:
- Research Org.:
- Univ. of Washington, Seattle, WA (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE); US Department of the Navy, Office of Naval Research (ONR); Asian Office of Aerospace R&D; Boeing–Johnson Foundation; National Science Foundation (NSF)
- OSTI Identifier:
- 1343575
- Report Number(s):
- DOE-UW-Jen-10
Journal ID: ISSN 1614-6832
- Grant/Contract Number:
- EE0006710; N00014–14–1–0170; FA2386–11–1–4072; DGE-1256082
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Energy Materials
- Additional Journal Information:
- Journal Volume: 5; Journal Issue: 10; Journal ID: ISSN 1614-6832
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; interfaces; perovskite; planar heterojunctions; solar cells; solution processability
Citation Formats
Liang, Po-Wei, Chueh, Chu-Chen, Williams, Spencer T., and Jen, Alex K. -Y. Roles of Fullerene-Based Interlayers in Enhancing the Performance of Organometal Perovskite Thin-Film Solar Cells. United States: N. p., 2015.
Web. doi:10.1002/aenm.201402321.
Liang, Po-Wei, Chueh, Chu-Chen, Williams, Spencer T., & Jen, Alex K. -Y. Roles of Fullerene-Based Interlayers in Enhancing the Performance of Organometal Perovskite Thin-Film Solar Cells. United States. https://doi.org/10.1002/aenm.201402321
Liang, Po-Wei, Chueh, Chu-Chen, Williams, Spencer T., and Jen, Alex K. -Y. Fri .
"Roles of Fullerene-Based Interlayers in Enhancing the Performance of Organometal Perovskite Thin-Film Solar Cells". United States. https://doi.org/10.1002/aenm.201402321. https://www.osti.gov/servlets/purl/1343575.
@article{osti_1343575,
title = {Roles of Fullerene-Based Interlayers in Enhancing the Performance of Organometal Perovskite Thin-Film Solar Cells},
author = {Liang, Po-Wei and Chueh, Chu-Chen and Williams, Spencer T. and Jen, Alex K. -Y.},
abstractNote = {Roles of fullerene-based interlayers in enhancing the performance of organometal perovskite thin-film solar cells are elucidated. By studying various fullerenes, a clear correlation between the electron mobility of fullerenes and the resulting performance of derived devices is determined. The metallic characteristics of the bilayer perovskite/fullerene field-effect transistor indicates an effective charge redistribution occurring at the corresponding interface. Lastly, a conventional perovskite thin-film solar cell derived from the C60 electron-transporting layer (ETL) affords a high power conversion efficiency of 15.4%.},
doi = {10.1002/aenm.201402321},
journal = {Advanced Energy Materials},
number = 10,
volume = 5,
place = {United States},
year = {Fri Feb 27 00:00:00 EST 2015},
month = {Fri Feb 27 00:00:00 EST 2015}
}
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- Yang, Liyan; Wu, Mingliang; Cai, Feilong
- Journal of Materials Chemistry A, Vol. 6, Issue 22
Achieving high-performance thick-film perovskite solar cells with electron transporting Bingel fullerenes
journal, January 2018
- Yan, Kangrong; Chen, Jiehuan; Ju, Huanxin
- Journal of Materials Chemistry A, Vol. 6, Issue 32
Incorporating deep electron traps into perovskite devices: towards high efficiency solar cells and fast photodetectors
journal, January 2018
- Zhang, Dezhong; Liu, Chunyu; Li, Zhiqi
- Journal of Materials Chemistry A, Vol. 6, Issue 42
Multifunctional asymmetrical molecules for high-performance perovskite and organic solar cells
journal, January 2019
- Gao, Wei; Wu, Fei; Liu, Tao
- Journal of Materials Chemistry A, Vol. 7, Issue 5
Ballistic transport simulation of acceptor–donor C 3 N/C 3 B double-wall hetero-nanotube field effect transistors
journal, January 2019
- Zhao, Jianwei; Cheng, Na; He, Yuanyuan
- Physical Chemistry Chemical Physics, Vol. 21, Issue 35
Impact of charge transport layers on the photochemical stability of MAPbI 3 in thin films and perovskite solar cells
journal, January 2019
- Boldyreva, A. G.; Akbulatov, A. F.; Elnaggar, M.
- Sustainable Energy & Fuels, Vol. 3, Issue 10
Highly efficient flexible MAPbI 3 solar cells with a fullerene derivative-modified SnO 2 layer as the electron transport layer
journal, January 2019
- Zhong, Meiyan; Liang, Yongqi; Zhang, Jianqi
- Journal of Materials Chemistry A, Vol. 7, Issue 12
N,P-coordinated fullerene-like carbon nanostructures with dual active centers toward highly-efficient multi-functional electrocatalysis for CO 2 RR, ORR and Zn-air battery
journal, January 2019
- Xue, Xiaoyi; Yang, Hui; Yang, Tao
- Journal of Materials Chemistry A, Vol. 7, Issue 25
Structural and electronic properties of multifunctional carbon composites of organometal halide perovskites
journal, January 2019
- Klejna, Sylwia
- Journal of Materials Chemistry A, Vol. 7, Issue 43
Perovskite solar cell-hybrid devices: thermoelectrically, electrochemically, and piezoelectrically connected power packs
journal, January 2019
- Zabihi, Fatemeh; Tebyetekerwa, Mike; Xu, Zhen
- Journal of Materials Chemistry A, Vol. 7, Issue 47
High-performance inverted planar perovskite solar cells using a pristine fullerene mixture as an electron-transport layer
journal, January 2019
- Xu, Chongyang; Liu, Zhihai; Lee, Eun-Cheol
- Journal of Materials Chemistry C, Vol. 7, Issue 23
The effect of hole transporting layer in charge accumulation properties of p-i-n perovskite solar cells
journal, July 2017
- Galatopoulos, Fedros; Savva, Achilleas; Papadas, Ioannis T.
- APL Materials, Vol. 5, Issue 7
Understanding the impact of C 60 at the interface of perovskite solar cells via drift-diffusion modeling
journal, March 2019
- Golubev, Timofey; Liu, Dianyi; Lunt, Richard
- AIP Advances, Vol. 9, Issue 3
Recent advances in interfacial engineering of perovskite solar cells
journal, August 2017
- Ye, Meidan; He, Chunfeng; Iocozzia, James
- Journal of Physics D: Applied Physics, Vol. 50, Issue 37
Possible interfacial ion/charge accumulation in thin-film perovskite/fullerene surfactant planar heterojunction solar cells
journal, September 2018
- Liang, Po-Wei; Chen, Chih-I; Chueh, Chu-Chen
- Journal of Physics D: Applied Physics, Vol. 51, Issue 50
First-principles calculation of stability, electronic and optical properties of PCBM-adsorbed MAPbI 3 surface
journal, September 2019
- Tian, Ying; Xue, Hongtao; Tang, Fuling
- Materials Research Express, Vol. 6, Issue 11
Hysteresis Passivation in Planar Perovskite Solar Cells Utilizing Facile Chemical Vapor Deposition Process and PCBM Interlayer
journal, November 2019
- Yang, Chongqiu; Shan, Xiaobiao; Xie, Tao
- Energies, Vol. 12, Issue 23
Efficient Regular Perovskite Solar Cells Based on Pristine [70]Fullerene as Electron-Selective Contact
journal, June 2016
- Collavini, Silvia; Kosta, Ivet; Völker, Sebastian F.
- ChemSusChem, Vol. 9, Issue 11
Versatility of Carbon Enables All Carbon Based Perovskite Solar Cells to Achieve High Efficiency and High Stability
journal, September 2018
- Meng, Xiangyue; Zhou, Junshuai; Hou, Jie
- Advanced Materials, Vol. 30, Issue 36
Nonradiative Recombination in Perovskite Solar Cells: The Role of Interfaces
text, January 2019
- Wolff, Christian M.; Caprioglio, Pietro; Stolterfoht, Martin
- FID GEO
The Effect of Hole Transporting Layer in Charge Accumulation Properties of p-i-n Perovskite Solar Cells
text, January 2018
- Galatopoulos, Fedros; Savva, Achilleas; Papadas, Ioannis T.
- arXiv
Highly Efficient Reproducible Perovskite Solar Cells Prepared by Low-Temperature Processing
journal, April 2016
- Hu, Hao; Wong, Ka; Kollek, Tom
- Molecules, Vol. 21, Issue 4