Ultrafast X-ray Auger probing of photoexcited molecular dynamics
Abstract
Here, molecules can efficiently and selectively convert light energy into other degrees of freedom. Disentangling the underlying ultrafast motion of electrons and nuclei of the photoexcited molecule presents a challenge to current spectroscopic approaches. Here we explore the photoexcited dynamics of molecules by an interaction with an ultrafast X-ray pulse creating a highly localized core hole that decays via Auger emission. We discover that the Auger spectrum as a function of photoexcitation—X-ray-probe delay contains valuable information about the nuclear and electronic degrees of freedom from an element-specific point of view. For the nucleobase thymine, the oxygen Auger spectrum shifts towards high kinetic energies, resulting from a particular C–O bond stretch in the ππ* photoexcited state. A subsequent shift of the Auger spectrum towards lower kinetic energies displays the electronic relaxation of the initial photoexcited state within 200 fs. Ab-initio simulations reinforce our interpretation and indicate an electronic decay to the nπ* state.
- Authors:
-
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- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., Stanford, CA (United States)
- Univ. di Perugia, Perugia (Italy)
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Western Michigan Univ., Kalamazoo MI (United States); Univ. of Connecticut, Storrs, CT (United States)
- Western Michigan Univ., Kalamazoo MI (United States)
- Uppsala Univ., Uppsala (Sweden); Univ. of Gothenburg, Gothenburg (Sweden)
- Uppsala Univ., Uppsala (Sweden)
- Max-Born-Institut, Berlin (Germany); UNIST, Ulsan (Republic of Korea)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1339539
- Report Number(s):
- SLAC-PUB-16907
Journal ID: ISSN 2041-1723
- Grant/Contract Number:
- AC02-76SF00515
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 5; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 74 ATOMIC AND MOLECULAR PHYSICS; PHYS; atomic and molecular physics; molecular dynamics
Citation Formats
McFarland, B. K., Farrell, J. P., Miyabe, S., Tarantelli, F., Aguilar, A., Berrah, N., Bostedt, C., Bozek, J. D., Bucksbaum, P. H., Castagna, J. C., Coffee, R. N., Cryan, J. P., Fang, L., Feifel, R., Gaffney, K. J., Glownia, J. M., Martinez, T. J., Mucke, M., Murphy, B., Natan, A., Osipov, T., Petrović, V. S., Schorb, S., Schultz, Th., Spector, L. S., Swiggers, M., Tenney, I., Wang, S., White, J. L., White, W., and Gühr, M. Ultrafast X-ray Auger probing of photoexcited molecular dynamics. United States: N. p., 2014.
Web. doi:10.1038/ncomms5235.
McFarland, B. K., Farrell, J. P., Miyabe, S., Tarantelli, F., Aguilar, A., Berrah, N., Bostedt, C., Bozek, J. D., Bucksbaum, P. H., Castagna, J. C., Coffee, R. N., Cryan, J. P., Fang, L., Feifel, R., Gaffney, K. J., Glownia, J. M., Martinez, T. J., Mucke, M., Murphy, B., Natan, A., Osipov, T., Petrović, V. S., Schorb, S., Schultz, Th., Spector, L. S., Swiggers, M., Tenney, I., Wang, S., White, J. L., White, W., & Gühr, M. Ultrafast X-ray Auger probing of photoexcited molecular dynamics. United States. https://doi.org/10.1038/ncomms5235
McFarland, B. K., Farrell, J. P., Miyabe, S., Tarantelli, F., Aguilar, A., Berrah, N., Bostedt, C., Bozek, J. D., Bucksbaum, P. H., Castagna, J. C., Coffee, R. N., Cryan, J. P., Fang, L., Feifel, R., Gaffney, K. J., Glownia, J. M., Martinez, T. J., Mucke, M., Murphy, B., Natan, A., Osipov, T., Petrović, V. S., Schorb, S., Schultz, Th., Spector, L. S., Swiggers, M., Tenney, I., Wang, S., White, J. L., White, W., and Gühr, M. Mon .
"Ultrafast X-ray Auger probing of photoexcited molecular dynamics". United States. https://doi.org/10.1038/ncomms5235. https://www.osti.gov/servlets/purl/1339539.
@article{osti_1339539,
title = {Ultrafast X-ray Auger probing of photoexcited molecular dynamics},
author = {McFarland, B. K. and Farrell, J. P. and Miyabe, S. and Tarantelli, F. and Aguilar, A. and Berrah, N. and Bostedt, C. and Bozek, J. D. and Bucksbaum, P. H. and Castagna, J. C. and Coffee, R. N. and Cryan, J. P. and Fang, L. and Feifel, R. and Gaffney, K. J. and Glownia, J. M. and Martinez, T. J. and Mucke, M. and Murphy, B. and Natan, A. and Osipov, T. and Petrović, V. S. and Schorb, S. and Schultz, Th. and Spector, L. S. and Swiggers, M. and Tenney, I. and Wang, S. and White, J. L. and White, W. and Gühr, M.},
abstractNote = {Here, molecules can efficiently and selectively convert light energy into other degrees of freedom. Disentangling the underlying ultrafast motion of electrons and nuclei of the photoexcited molecule presents a challenge to current spectroscopic approaches. Here we explore the photoexcited dynamics of molecules by an interaction with an ultrafast X-ray pulse creating a highly localized core hole that decays via Auger emission. We discover that the Auger spectrum as a function of photoexcitation—X-ray-probe delay contains valuable information about the nuclear and electronic degrees of freedom from an element-specific point of view. For the nucleobase thymine, the oxygen Auger spectrum shifts towards high kinetic energies, resulting from a particular C–O bond stretch in the ππ* photoexcited state. A subsequent shift of the Auger spectrum towards lower kinetic energies displays the electronic relaxation of the initial photoexcited state within 200 fs. Ab-initio simulations reinforce our interpretation and indicate an electronic decay to the nπ* state.},
doi = {10.1038/ncomms5235},
journal = {Nature Communications},
number = ,
volume = 5,
place = {United States},
year = {Mon Jun 23 00:00:00 EDT 2014},
month = {Mon Jun 23 00:00:00 EDT 2014}
}
Web of Science
Works referenced in this record:
Zur Quantentheorie der Molekeln
journal, January 1927
- Born, M.; Oppenheimer, R.
- Annalen der Physik, Vol. 389, Issue 20
Conical Intersections: Electronic Structure, Dynamics and Spectroscopy
book, July 2004
- Domcke, Wolfgang; Yarkony, David R.; Köppel, Horst
- Advanced Series in Physical Chemistry, Vol. 15
Isomerization Through Conical Intersections
journal, May 2007
- Levine, Benjamin G.; Martínez, Todd J.
- Annual Review of Physical Chemistry, Vol. 58, Issue 1
Electronically excited states and photodynamics: a continuing challenge
journal, January 2012
- Plasser, Felix; Barbatti, Mario; Aquino, Adélia J. A.
- Theoretical Chemistry Accounts, Vol. 131, Issue 1
Perspective: Nonadiabatic dynamics theory
journal, December 2012
- Tully, John C.
- The Journal of Chemical Physics, Vol. 137, Issue 22
Femtosecond Time-Resolved Photoelectron Spectroscopy
journal, April 2004
- Stolow, Albert; Bragg, Arthur E.; Neumark, Daniel M.
- Chemical Reviews, Vol. 104, Issue 4
Ultrafast X-ray Absorption Spectroscopy
journal, April 2004
- Bressler, Christian; Chergui, Majed
- Chemical Reviews, Vol. 104, Issue 4
Photo-Induced Spin-State Conversion in Solvated Transition Metal Complexes Probed via Time-Resolved Soft X-ray Spectroscopy
journal, May 2010
- Huse, Nils; Kim, Tae Kyu; Jamula, Lindsey
- Journal of the American Chemical Society, Vol. 132, Issue 19
Femtosecond and Subfemtosecond X-Ray Pulses from a Self-Amplified Spontaneous-Emission–Based Free-Electron Laser
journal, February 2004
- Emma, P.; Bane, K.; Cornacchia, M.
- Physical Review Letters, Vol. 92, Issue 7
Thymine Dimerization in DNA Is an Ultrafast Photoreaction
journal, February 2007
- Schreier, W. J.; Schrader, T. E.; Koller, F. O.
- Science, Vol. 315, Issue 5812
Ultrafast Excited-State Dynamics in Nucleic Acids
journal, April 2004
- Crespo-Hernández, Carlos E.; Cohen, Boiko; Hare, Patrick M.
- Chemical Reviews, Vol. 104, Issue 4
Intrinsic Lifetimes of the Excited State of DNA and RNA Bases
journal, November 2002
- Kang, Hyuk; Lee, Kang Taek; Jung, Boyong
- Journal of the American Chemical Society, Vol. 124, Issue 44
Excited states dynamics of DNA and RNA bases: Characterization of a stepwise deactivation pathway in the gas phase
journal, February 2005
- Canuel, Clélia; Mons, Michel; Piuzzi, François
- The Journal of Chemical Physics, Vol. 122, Issue 7
Thymine relaxation after UV irradiation: the role of tautomerization and πσ* states
journal, January 2009
- González-Vázquez, Jesús; González, Leticia; Samoylova, Elena
- Physical Chemistry Chemical Physics, Vol. 11, Issue 20
Electronic relaxation dynamics in DNA and RNA bases studied by time-resolved photoelectron spectroscopy
journal, January 2004
- Ullrich, Susanne; Schultz, Thomas; Zgierski, Marek Z.
- Physical Chemistry Chemical Physics, Vol. 6, Issue 10
Ab Initio Molecular Dynamics and Time-Resolved Photoelectron Spectroscopy of Electronically Excited Uracil and Thymine
journal, August 2007
- Hudock, Hanneli R.; Levine, Benjamin G.; Thompson, Alexis L.
- The Journal of Physical Chemistry A, Vol. 111, Issue 34
Photodynamics Simulations of Thymine: Relaxation into the First Excited Singlet State †
journal, November 2009
- Szymczak, Jaroslaw J.; Barbatti, Mario; Soo Hoo, Jason T.
- The Journal of Physical Chemistry A, Vol. 113, Issue 45
Conical Intersections in Thymine
journal, December 2006
- Perun, Serhiy; Sobolewski, Andrzej L.; Domcke, Wolfgang
- The Journal of Physical Chemistry A, Vol. 110, Issue 49
Unified Model for the Ultrafast Decay of Pyrimidine Nucleobases
journal, December 2006
- Merchán, Manuela; González-Luque, Remedios; Climent, Teresa
- The Journal of Physical Chemistry B, Vol. 110, Issue 51
Photophysics of the π,π* and n,π* States of Thymine: MS-CASPT2 Minimum-Energy Paths and CASSCF on-the-Fly Dynamics
journal, September 2009
- Asturiol, David; Lasorne, Benjamin; Robb, Michael A.
- The Journal of Physical Chemistry A, Vol. 113, Issue 38
Higher-order approximations for the particle-particle propagator
journal, October 1984
- Schirmer, J.; Barth, A.
- Zeitschrift f�r Physik A Atoms and Nuclei, Vol. 317, Issue 3
The calculation of molecular double ionization spectra by Green’s functions
journal, October 2006
- Tarantelli, Francesco
- Chemical Physics, Vol. 329, Issue 1-3
Toward a systematic molecular orbital theory for excited states
journal, January 1992
- Foresman, James B.; Head-Gordon, Martin; Pople, John A.
- The Journal of Physical Chemistry, Vol. 96, Issue 1
Internal conversion to the electronic ground state occurs via two distinct pathways for pyrimidine bases in aqueous solution
journal, December 2006
- Hare, P. M.; Crespo-Hernandez, C. E.; Kohler, B.
- Proceedings of the National Academy of Sciences, Vol. 104, Issue 2
Singlet Excited-State Behavior of Uracil and Thymine in Aqueous Solution: A Combined Experimental and Computational Study of 11 Uracil Derivatives
journal, January 2006
- Gustavsson, Thomas; Bányász, Ákos; Lazzarotto, Elodie
- Journal of the American Chemical Society, Vol. 128, Issue 2
First lasing and operation of an ångstrom-wavelength free-electron laser
journal, August 2010
- Emma, P.; Akre, R.; Arthur, J.
- Nature Photonics, Vol. 4, Issue 9
Operation of a free-electron laser from the extreme ultraviolet to the water window
journal, June 2007
- Ackermann, W.; Asova, G.; Ayvazyan, V.
- Nature Photonics, Vol. 1, Issue 6
A compact X-ray free-electron laser emitting in the sub-ångström region
journal, June 2012
- Ishikawa, Tetsuya; Aoyagi, Hideki; Asaka, Takao
- Nature Photonics, Vol. 6, Issue 8
X-ray–optical cross-correlator for gas-phase experiments at the Linac Coherent Light Source free-electron laser
journal, March 2012
- Schorb, S.; Gorkhover, T.; Cryan, J. P.
- Applied Physics Letters, Vol. 100, Issue 12
Femtosecond electronic response of atoms to ultra-intense X-rays
journal, July 2010
- Young, L.; Kanter, E. P.; Krässig, B.
- Nature, Vol. 466, Issue 7302
Dynamics of Hollow Atom Formation in Intense X-Ray Pulses Probed by Partial Covariance Mapping
journal, August 2013
- Frasinski, L. J.; Zhaunerchyk, V.; Mucke, M.
- Physical Review Letters, Vol. 111, Issue 7
The High Resolution L 2,3 MM and M 4,5 NN Auger Spectra from Krypton and M 4,5 NN and N 4,5 OO Auger Spectra from Xenon
journal, August 1972
- Werme, L. O.; Bergmark, T.; Siegbahn, K.
- Physica Scripta, Vol. 6, Issue 2-3
Works referencing / citing this record:
Diffractive imaging of a rotational wavepacket in nitrogen molecules with femtosecond megaelectronvolt electron pulses
journal, April 2016
- Yang, Jie; Guehr, Markus; Vecchione, Theodore
- Nature Communications, Vol. 7, Issue 1
Probing ultrafast ππ*/nπ* internal conversion in organic chromophores via K-edge resonant absorption
journal, June 2017
- Wolf, T. J. A.; Myhre, R. H.; Cryan, J. P.
- Nature Communications, Vol. 8, Issue 1
UV-induced long-lived decays in solvated pyrimidine nucleosides resolved at the MS-CASPT2/MM level
journal, January 2018
- Pepino, Ana Julieta; Segarra-Martí, Javier; Nenov, Artur
- Physical Chemistry Chemical Physics, Vol. 20, Issue 10
Photophysics of indole upon X-ray absorption
journal, January 2018
- Kierspel, Thomas; Bomme, Cédric; Di Fraia, Michele
- Physical Chemistry Chemical Physics, Vol. 20, Issue 30
Multistate hybrid time-dependent density functional theory with surface hopping accurately captures ultrafast thymine photodeactivation
journal, January 2019
- Parker, Shane M.; Roy, Saswata; Furche, Filipp
- Physical Chemistry Chemical Physics, Vol. 21, Issue 35
Stochastic stimulated electronic x-ray Raman spectroscopy
journal, February 2016
- Kimberg, Victor; Rohringer, Nina
- Structural Dynamics, Vol. 3, Issue 3
Photoelectron spectra of 2-thiouracil, 4-thiouracil, and 2,4-dithiouracil
journal, February 2016
- Ruckenbauer, Matthias; Mai, Sebastian; Marquetand, Philipp
- The Journal of Chemical Physics, Vol. 144, Issue 7
Perspective: Opportunities for ultrafast science at SwissFEL
journal, November 2017
- Abela, Rafael; Beaud, Paul; van Bokhoven, Jeroen A.
- Structural Dynamics, Vol. 4, Issue 6
Time-resolved electron spectroscopy for chemical analysis of photodissociation: Photoelectron spectra of Fe(CO) 5 , Fe(CO) 4 , and Fe(CO) 3
journal, July 2018
- Leitner, T.; Josefsson, I.; Mazza, T.
- The Journal of Chemical Physics, Vol. 149, Issue 4
An efficient approximate algorithm for nonadiabatic molecular dynamics
journal, December 2018
- Hanasaki, Kota; Kanno, Manabu; Niehaus, Thomas A.
- The Journal of Chemical Physics, Vol. 149, Issue 24
Roadmap of ultrafast x-ray atomic and molecular physics
journal, January 2018
- Young, Linda; Ueda, Kiyoshi; Gühr, Markus
- Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 51, Issue 3
A pump–probe scheme with a single chirped pulse to image electron and nuclear dynamics in molecules
journal, December 2018
- Jelovina, Denis; Feist, Johannes; Martín, Fernando
- New Journal of Physics, Vol. 20, Issue 12
Photochemical pathways in nucleobases measured with an X-ray FEL
journal, April 2019
- Wolf, Thomas J. A.; Gühr, Markus
- Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2145
Development of ultrafast capabilities for X-ray free-electron lasers at the linac coherent light source
journal, April 2019
- Coffee, Ryan N.; Cryan, James P.; Duris, Joseph
- Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2145
Nonlinear resonant Auger spectroscopy in CO using an x-ray pump-control scheme
journal, December 2016
- Zhang, Song Bin; Kimberg, Victor; Rohringer, Nina
- Physical Review A, Vol. 94, Issue 6
Laser control over the ultrafast Coulomb explosion of after Auger decay: A quantum-dynamics investigation
journal, April 2017
- Hanna, Athiya Mahmud; Vendrell, Oriol; Ourmazd, Abbas
- Physical Review A, Vol. 95, Issue 4
Time-resolved inner-shell photoelectron spectroscopy: From a bound molecule to an isolated atom
journal, April 2018
- Brauße, Felix; Goldsztejn, Gildas; Amini, Kasra
- Physical Review A, Vol. 97, Issue 4
SNP hot-spots in the clam parasite QPX
journal, June 2018
- Bassim, Sleiman; Allam, Bassem
- BMC Genomics, Vol. 19, Issue 1
Short-wavelength free-electron laser sources and science: a review
text, January 2017
- Seddon, E. A.; Clarke, J. A.; Dunning, D. J.
- Deutsches Elektronen-Synchrotron, DESY, Hamburg
The LAMP instrument at the Linac Coherent Light Source free-electron laser
text, January 2018
- Osipov, Timur; Bostedt, Christoph; Castagna, J. -C.
- Deutsches Elektronen-Synchrotron, DESY, Hamburg
Probing Dynamics in Colloidal Crystals with Pump-Probe Experiments at LCLS: Methodology and Analysis
journal, May 2017
- Mukharamova, Nastasia; Lazarev, Sergey; Meijer, Janne-Mieke
- Applied Sciences, Vol. 7, Issue 5
The LAMP instrument at the Linac Coherent Light Source free-electron laser
journal, March 2018
- Osipov, Timur; Bostedt, Christoph; Castagna, J. -C.
- Review of Scientific Instruments, Vol. 89, Issue 3
Pulse Duration of Seeded Free-Electron Lasers
text, January 2017
- Finetti, Paola; Höppner, Hauke; Allaria, Enrico
- GSI Helmholtzzentrum fuer Schwerionenforschung, GSI, Darmstadt
Roadmap of ultrafast x-ray atomic and molecular physics
text, January 2019
- Young, Linda; Ueda, Kiyoshi; Gühr, Markus
- Universität Potsdam
Photophysics of indole upon X-ray absorption
text, January 2018
- Kierspel, Thomas; Bomme, Cedric; Di Fraia, Michele
- Deutsches Elektronen-Synchrotron, DESY, Hamburg
Time-resolved electron spectroscopy for chemical analysis of photodissociation: Photoelectron spectra of Fe(CO)$_5$ , Fe(CO)$_4$ , and Fe(CO)$_3$
text, January 2018
- Leitner, T.; Josefsson, I.; Mazza, T.
- Deutsches Elektronen-Synchrotron, DESY, Hamburg
Perspective: Opportunities for ultrafast science at SwissFEL
text, January 2017
- Abela, Rafael; Beaud, Paul; Van Bokhoven, Jeroen A.
- AIP Publishing
Probing Dynamics in Colloidal crystals with pump-probe experiments at LCLS Methodololgy and analysis
text, January 2017
- Vartaniants, Ivan; Mukharamova, Nastsia; Lazarev, Sergey
- Deutsches Elektronen-Synchrotron, DESY, Hamburg
Time-resolved inner-shell photoelectron spectroscopy: From a bound molecule to an isolated atom
text, January 2018
- Brauße, Felix; Goldsztejn, Gildas; Amini, Kasra
- Deutsches Elektronen-Synchrotron, DESY, Hamburg
Perspective: Opportunities for ultrafast science at SwissFEL
text, January 2017
- Abela, Rafael; Beaud, Paul; Van Bokhoven, Jeroen A.
- ETH Zurich
Short-wavelength free-electron laser sources and science: a review
journal, October 2017
- Seddon, E. A.; Clarke, J. A.; Dunning, D. J.
- Reports on Progress in Physics, Vol. 80, Issue 11
Roadmap of ultrafast x-ray atomic and molecular physics
text, January 2018
- Young, Linda; Ueda, Kiyoshi; Gühr, Markus
- Deutsches Elektronen-Synchrotron, DESY, Hamburg
Observation of Quantum Interferences via Light Induced Conical Intersections in Diatomic Molecules
text, January 2015
- Natan, Adi; Ware, Matthew R.; Prabhudesai, Vaibhav S.
- arXiv
Photophysics of indole upon x-ray absorption
text, January 2018
- Kierspel, Thomas; Bomme, Cédric; Di Fraia, Michele
- arXiv
Diffractive imaging of a rotational wavepacket in nitrogen molecules with femtosecond megaelectronvolt electron pulses
journal, April 2016
- Yang, Jie; Guehr, Markus; Vecchione, Theodore
- Nature Communications, Vol. 7, Issue 1
Elucidating the origins of multimode vibrational coherences of polyatomic molecules induced by intense laser fields
journal, September 2017
- Wei, Zhengrong; Li, Jialin; Wang, Lin
- Nature Communications, Vol. 8, Issue 1
Monitoring conical intersections in the ring opening of furan by attosecond stimulated X-ray Raman spectroscopy
journal, October 2015
- Hua, Weijie; Oesterling, Sven; Biggs, Jason D.
- Structural Dynamics, Vol. 3, Issue 2
Development of ultrafast capabilities for X-ray free-electron lasers at the linac coherent light source
journal, April 2019
- Coffee, Ryan N.; Cryan, James P.; Duris, Joseph
- Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2145
Machine Learning for Absorption Cross Sections
journal, July 2020
- Xue, Bao-Xin; Barbatti, Mario; Dral, Pavlo O.
- ChemRxiv
An Experimental Protocol for Femtosecond NIR/UV - XUV Pump-Probe Experiments with Free-Electron Lasers
text, January 2018
- Rolles, Daniel; Boll, Rebecca; Erk, Benjamin
- Deutsches Elektronen-Synchrotron, DESY, Hamburg
Spectroscopic Signature of Chemical Bond Dissociation Revealed by Calculated Core-Electron Spectra
text, January 2019
- Inhester, Ludger; Li, Zheng; Zhu, Xiaolei
- Deutsches Elektronen-Synchrotron, DESY, Hamburg
New Insights into the State Trapping of UV-Excited Thymine
journal, November 2016
- Stojanović, Ljiljana; Bai, Shuming; Nagesh, Jayashree
- Molecules, Vol. 21, Issue 11
Assessment of the Potential Energy Hypersurfaces in Thymine within Multiconfigurational Theory: CASSCF vs. CASPT2
journal, December 2016
- Segarra-Martí, Javier; Francés-Monerris, Antonio; Roca-Sanjuán, Daniel
- Molecules, Vol. 21, Issue 12
Perspective: Opportunities for ultrafast science at SwissFEL
text, January 2017
- Abela, Rafael; Beaud, Paul; Van Bokhoven, Jeroen A.
- ETH Zurich
Attosecond photoionization dynamics with stimulated core-valence transitions
text, January 2015
- You, Jhih-An; Rohringer, Nina; Dahlström, Jan Marcus
- arXiv
Stochastic stimulated electronic x-ray Raman spectroscopy
preprint, January 2015
- Kimberg, Victor; Rohringer, Nina
- arXiv
Fullerene Dynamics with X-Ray Free-Electron Lasers
book, April 2018
- Berrah, Nora
- Fullerenes and Relative Materials - Properties and Applications