DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Kinetics of diffusion-controlled annihilation with sparse initial conditions

Abstract

Here, we study diffusion-controlled single-species annihilation with sparse initial conditions. In this random process, particles undergo Brownian motion, and when two particles meet, both disappear. We also focus on sparse initial conditions where particles occupy a subspace of dimension δ that is embedded in a larger space of dimension d. Furthermore, we find that the co-dimension Δ = d - δ governs the behavior. All particles disappear when the co-dimension is sufficiently small, Δ ≤ 2; otherwise, a finite fraction of particles indefinitely survive. We establish the asymptotic behavior of the probability S(t) that a test particle survives until time t. When the subspace is a line, δ = 1, we find inverse logarithmic decay, $$S\sim {(\mathrm{ln}t)}^{-1}$$, in three dimensions, and a modified power-law decay, $$S\sim (\mathrm{ln}t){t}^{-1/2}$$, in two dimensions. In general, the survival probability decays algebraically when Δ < 2, and there is an inverse logarithmic decay at the critical co-dimension Δ = 2.

Authors:
ORCiD logo [1];  [2]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States). Theoretical Division and Center for Nonlinear Studies
  2. Boston Univ., MA (United States). Dept. of Physics
Publication Date:
Research Org.:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1337109
Report Number(s):
LA-UR-16-25627
Journal ID: ISSN 1751-8113
Grant/Contract Number:  
AC52-06NA25396
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Physics. A, Mathematical and Theoretical
Additional Journal Information:
Journal Volume: 49; Journal Issue: 50; Journal ID: ISSN 1751-8113
Publisher:
IOP Publishing
Country of Publication:
United States
Language:
English
Subject:
97 MATHEMATICS AND COMPUTING; Mathematics

Citation Formats

Ben-Naim, Eli, and Krapivsky, Paul. Kinetics of diffusion-controlled annihilation with sparse initial conditions. United States: N. p., 2016. Web. doi:10.1088/1751-8113/49/50/504005.
Ben-Naim, Eli, & Krapivsky, Paul. Kinetics of diffusion-controlled annihilation with sparse initial conditions. United States. https://doi.org/10.1088/1751-8113/49/50/504005
Ben-Naim, Eli, and Krapivsky, Paul. Fri . "Kinetics of diffusion-controlled annihilation with sparse initial conditions". United States. https://doi.org/10.1088/1751-8113/49/50/504005. https://www.osti.gov/servlets/purl/1337109.
@article{osti_1337109,
title = {Kinetics of diffusion-controlled annihilation with sparse initial conditions},
author = {Ben-Naim, Eli and Krapivsky, Paul},
abstractNote = {Here, we study diffusion-controlled single-species annihilation with sparse initial conditions. In this random process, particles undergo Brownian motion, and when two particles meet, both disappear. We also focus on sparse initial conditions where particles occupy a subspace of dimension δ that is embedded in a larger space of dimension d. Furthermore, we find that the co-dimension Δ = d - δ governs the behavior. All particles disappear when the co-dimension is sufficiently small, Δ ≤ 2; otherwise, a finite fraction of particles indefinitely survive. We establish the asymptotic behavior of the probability S(t) that a test particle survives until time t. When the subspace is a line, δ = 1, we find inverse logarithmic decay, $S\sim {(\mathrm{ln}t)}^{-1}$, in three dimensions, and a modified power-law decay, $S\sim (\mathrm{ln}t){t}^{-1/2}$, in two dimensions. In general, the survival probability decays algebraically when Δ < 2, and there is an inverse logarithmic decay at the critical co-dimension Δ = 2.},
doi = {10.1088/1751-8113/49/50/504005},
journal = {Journal of Physics. A, Mathematical and Theoretical},
number = 50,
volume = 49,
place = {United States},
year = {Fri Dec 16 00:00:00 EST 2016},
month = {Fri Dec 16 00:00:00 EST 2016}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 5 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Diffusion-Limited Aggregation, a Kinetic Critical Phenomenon
journal, November 1981


Pattern Formation and Dynamics in Nonequilibrium Systems
book, January 2009


Front propagation into unstable states
journal, November 2003


Applications of field-theoretic renormalization group methods to reaction–diffusion problems
journal, April 2005

  • Täuber, Uwe C.; Howard, Martin; Vollmayr-Lee, Benjamin P.
  • Journal of Physics A: Mathematical and General, Vol. 38, Issue 17
  • DOI: 10.1088/0305-4470/38/17/R01

Diffusion-limited exciton fusion reaction in one-dimensional tetramethylammonium manganese trichloride (TMMC)
journal, April 1993


One-dimensional diffusion-limited relaxation of photoexcitations in suspensions of single-walled carbon nanotubes
journal, July 2006


Measurement of a Reaction-Diffusion Crossover in Exciton-Exciton Recombination inside Carbon Nanotubes Using Femtosecond Optical Absorption
journal, November 2013


Role of density fluctuations in bimolecular reaction kinetics
journal, February 1978


Asymptotics for interacting particle systems onZ d
journal, June 1980

  • Bramson, Maury; Griffeath, David
  • Zeitschrift f�r Wahrscheinlichkeitstheorie und Verwandte Gebiete, Vol. 53, Issue 2
  • DOI: 10.1007/BF01013315

Particle–antiparticle annihilation in diffusive motion
journal, March 1983

  • Toussaint, Doug; Wilczek, Frank
  • The Journal of Chemical Physics, Vol. 78, Issue 5
  • DOI: 10.1063/1.445022

Kinetics of diffusion‐controlled processes in dense polymer systems. I. Nonentangled regimes
journal, March 1982

  • de Gennes, P. G.
  • The Journal of Chemical Physics, Vol. 76, Issue 6
  • DOI: 10.1063/1.443328

Fluctuation-dominated kinetics in diffusion-controlled reactions
journal, July 1985


Diffusion-limited reactions in one dimension
journal, May 1983

  • Torney, David C.; McConnell, Harden M.
  • The Journal of Physical Chemistry, Vol. 87, Issue 11
  • DOI: 10.1021/j100234a023

Exact solutions for a diffusion-reaction process in one dimension
journal, March 1988


Exact solution for a steady-state aggregation model in one dimension
journal, April 1989


Statics and dynamics of a diffusion-limited reaction: Anomalous kinetics, nonequilibrium self-ordering, and a dynamic transition
journal, September 1990

  • ben-Avraham, Daniel; Burschka, Martin A.; Doering, Charles R.
  • Journal of Statistical Physics, Vol. 60, Issue 5-6
  • DOI: 10.1007/BF01025990

Complete Exact Solution of Diffusion-Limited Coalescence, A + A A
journal, November 1998


Correlation functions for diffusion-limited annihilation, A + A 0
journal, November 2001


Alternating kinetics of annihilating random walks near a free interface
journal, March 1998

  • Frachebourg, L.; Krapivsky, P. L.; Redner, S.
  • Journal of Physics A: Mathematical and General, Vol. 31, Issue 12
  • DOI: 10.1088/0305-4470/31/12/005

Finite-size scaling studies of one-dimensional reaction-diffusion systems. Part I. Analytical results
journal, March 1995

  • Krebs, Klaus; Pfannmüller, Markus P.; Wehefritz, Birgit
  • Journal of Statistical Physics, Vol. 78, Issue 5-6
  • DOI: 10.1007/BF02180138

A Guide to First-Passage Processes
book, January 2001


Kinetic description of diffusion-limited reactions in random catalytic media
journal, January 1998

  • Oshanin, G.; Blumen, A.
  • The Journal of Chemical Physics, Vol. 108, Issue 3
  • DOI: 10.1063/1.475476

Reaction kinetics of cluster impurities
journal, February 1996


�ber eine Aufgabe der Wahrscheinlichkeitsrechnung betreffend die Irrfahrt im Stra�ennetz
journal, March 1921


Works referencing / citing this record:

Annihilation of single-species charged particles based on Dyson gas dynamics
journal, January 2020


Annihilation of single-species charged particles based on the Dyson gas dynamics
text, January 2019