DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Direct measurements of the ionization potential depression in a dense plasma

Abstract

We have used the Linac Coherent Light Source to generate solid-density aluminum plasmas at temperatures of up to 180 eV. By varying the photon energy of the x rays that both create and probe the plasma, and observing the K-α fluorescence, we can directly measure the position of the K edge of the highly charged ions within the system. Lastly, the results are found to disagree with the predictions of the extensively used Stewart-Pyatt model, but are consistent with the earlier model of Ecker and Kroll, which predicts significantly greater depression of the ionization potential.

Authors:
 [1];  [1];  [2];  [3];  [4];  [5];  [5];  [3];  [6];  [7];  [5];  [1];  [5];  [7];  [7];  [7];  [1];  [8];  [1];  [7] more »;  [7];  [9];  [7];  [5];  [7];  [7];  [10];  [7];  [7];  [3];  [7];  [1] « less
  1. Univ. of Oxford, Oxford (United Kingdom)
  2. Atomic and Molecular Data Unit, Vienna (Austria)
  3. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  4. AWE Aldermaston, Reading (United Kingdom)
  5. Institute of Physics ASCR, Prague (Czech Republic)
  6. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of California, Berkeley, CA (United States)
  7. SLAC National Accelerator Lab., Menlo Park, CA (United States)
  8. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  9. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
  10. Friedrich-Schiller-Univ., Jena (Germany)
Publication Date:
Research Org.:
Univ. of California, Berkeley, CA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1334506
Alternate Identifier(s):
OSTI ID: 1103070
Grant/Contract Number:  
FG52-06NA26212
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review Letters
Additional Journal Information:
Journal Volume: 109; Journal Issue: 6; Journal ID: ISSN 0031-9007
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
70 PLASMA PHYSICS AND FUSION TECHNOLOGY

Citation Formats

Ciricosta, O., Vinko, S. M., Chung, H. -K., Cho, B. -I., Brown, C. R. D., Burian, T., Chalupsky, J., Engelhorn, K., Falcone, R. W., Graves, C., Hajkova, V., Higginbotham, A., Juha, L., Krzywinski, J., Lee, H. J., Messerschmidt, M., Murphy, C. D., Ping, Y., Rackstraw, D. S., Scherz, A., Schlotter, W., Toleikis, S., Turner, J. J., Vysin, L., Wang, T., Wu, B., Zastrau, U., Zhu, D., Lee, R. W., Heimann, P., Nagler, B., and Wark, Justin S. Direct measurements of the ionization potential depression in a dense plasma. United States: N. p., 2012. Web. doi:10.1103/PhysRevLett.109.065002.
Ciricosta, O., Vinko, S. M., Chung, H. -K., Cho, B. -I., Brown, C. R. D., Burian, T., Chalupsky, J., Engelhorn, K., Falcone, R. W., Graves, C., Hajkova, V., Higginbotham, A., Juha, L., Krzywinski, J., Lee, H. J., Messerschmidt, M., Murphy, C. D., Ping, Y., Rackstraw, D. S., Scherz, A., Schlotter, W., Toleikis, S., Turner, J. J., Vysin, L., Wang, T., Wu, B., Zastrau, U., Zhu, D., Lee, R. W., Heimann, P., Nagler, B., & Wark, Justin S. Direct measurements of the ionization potential depression in a dense plasma. United States. https://doi.org/10.1103/PhysRevLett.109.065002
Ciricosta, O., Vinko, S. M., Chung, H. -K., Cho, B. -I., Brown, C. R. D., Burian, T., Chalupsky, J., Engelhorn, K., Falcone, R. W., Graves, C., Hajkova, V., Higginbotham, A., Juha, L., Krzywinski, J., Lee, H. J., Messerschmidt, M., Murphy, C. D., Ping, Y., Rackstraw, D. S., Scherz, A., Schlotter, W., Toleikis, S., Turner, J. J., Vysin, L., Wang, T., Wu, B., Zastrau, U., Zhu, D., Lee, R. W., Heimann, P., Nagler, B., and Wark, Justin S. Mon . "Direct measurements of the ionization potential depression in a dense plasma". United States. https://doi.org/10.1103/PhysRevLett.109.065002. https://www.osti.gov/servlets/purl/1334506.
@article{osti_1334506,
title = {Direct measurements of the ionization potential depression in a dense plasma},
author = {Ciricosta, O. and Vinko, S. M. and Chung, H. -K. and Cho, B. -I. and Brown, C. R. D. and Burian, T. and Chalupsky, J. and Engelhorn, K. and Falcone, R. W. and Graves, C. and Hajkova, V. and Higginbotham, A. and Juha, L. and Krzywinski, J. and Lee, H. J. and Messerschmidt, M. and Murphy, C. D. and Ping, Y. and Rackstraw, D. S. and Scherz, A. and Schlotter, W. and Toleikis, S. and Turner, J. J. and Vysin, L. and Wang, T. and Wu, B. and Zastrau, U. and Zhu, D. and Lee, R. W. and Heimann, P. and Nagler, B. and Wark, Justin S.},
abstractNote = {We have used the Linac Coherent Light Source to generate solid-density aluminum plasmas at temperatures of up to 180 eV. By varying the photon energy of the x rays that both create and probe the plasma, and observing the K-α fluorescence, we can directly measure the position of the K edge of the highly charged ions within the system. Lastly, the results are found to disagree with the predictions of the extensively used Stewart-Pyatt model, but are consistent with the earlier model of Ecker and Kroll, which predicts significantly greater depression of the ionization potential.},
doi = {10.1103/PhysRevLett.109.065002},
journal = {Physical Review Letters},
number = 6,
volume = 109,
place = {United States},
year = {Mon Aug 06 00:00:00 EDT 2012},
month = {Mon Aug 06 00:00:00 EDT 2012}
}

Journal Article:

Citation Metrics:
Cited by: 200 works
Citation information provided by
Web of Science

Figures / Tables:

FIG. 1 FIG. 1: (Color online) Experimentally recorded K-α emission spectra from hot solid density aluminum. SCFLY simulations with different IPD models are compared with the experimental data for a subset of the X-ray laser photon energies. From the bottom the spectra corresponding to 1580, 1600, 1630, 1650, 1720 and 1830 eVmore » pump photon energies are shown. The spectra have been artificially displaced in intensity for clarity, and a Bremsstrahlung component (at the maximum temperature provided by the simulations) has been added to the calculated spectra. The grey shading indicates the difference between the calculations using different IPD models.« less

Save / Share:

Works referenced in this record:

Lowering of the Ionization Energy for a Plasma in Thermodynamic Equilibrium
journal, January 1963


Lowering of Ionization Potentials in Plasmas
journal, April 1966

  • Stewart, John C.; Pyatt, Kedar D. , Jr.
  • The Astrophysical Journal, Vol. 144
  • DOI: 10.1086/148714

Pressure ionization in laser-fusion target simulation
journal, May 1980

  • Zimmerman, G. B.; More, R. M.
  • Journal of Quantitative Spectroscopy and Radiative Transfer, Vol. 23, Issue 5
  • DOI: 10.1016/0022-4073(80)90055-2

High Density Plasma Effects on Atomic and Ionic Spectra
journal, November 1982


Electronic energy-levels in dense plasmas
journal, March 1982


Astrophysical Opacity
journal, January 1994


Interiors of Giant Planets Inside and Outside the Solar System
journal, October 1999


The physics basis for ignition using indirect-drive targets on the National Ignition Facility
journal, February 2004

  • Lindl, John D.; Amendt, Peter; Berger, Richard L.
  • Physics of Plasmas, Vol. 11, Issue 2
  • DOI: 10.1063/1.1578638

Cretin—a radiative transfer capability for laboratory plasmas
journal, October 2001


FLYCHK: Generalized population kinetics and spectral model for rapid spectroscopic analysis for all elements
journal, December 2005


A model for ionization balance and L-shell spectroscopy of non-LTE plasmas
journal, August 1987


Blue Shift of the K Absorption Edge in Laser-Shocked Solids
journal, September 1989


Pressure Ionization and Line Merging in Strongly Coupled Plasmas Produced by 100-fs Laser Pulses
journal, May 1998


Ionic Depression of Series Limits in Cne-Electron Spectra.
journal, September 1939

  • Inglis, D. R.; Teller, E.
  • The Astrophysical Journal, Vol. 90
  • DOI: 10.1086/144118

Creation and diagnosis of a solid-density plasma with an X-ray free-electron laser
journal, January 2012

  • Vinko, S. M.; Ciricosta, O.; Cho, B. I.
  • Nature, Vol. 482, Issue 7383
  • DOI: 10.1038/nature10746

Extension of atomic configuration sets of the Non-LTE model in the application to the Kα diagnostics of hot dense matter
journal, May 2007


Simulations of neon irradiated by intense X-ray laser radiation
journal, September 2011

  • Ciricosta, Orlando; Chung, Hyun-Kyung; Lee, Richard W.
  • High Energy Density Physics, Vol. 7, Issue 3
  • DOI: 10.1016/j.hedp.2011.02.003

Spot size characterization of focused non-Gaussian X-ray laser beams
journal, January 2010

  • Chalupský, J.; Krzywinski, J.; Juha, L.
  • Optics Express, Vol. 18, Issue 26
  • DOI: 10.1364/OE.18.027836

Analysis of K α line emission from aluminum plasmas created by intense proton beams
journal, April 1993


Two-electron one-photon transition in aluminum following double- K -shell ionization
journal, July 1988


Works referencing / citing this record:

Ionization dynamics of dense matter generated by intense ultrashort X-ray pulses
journal, February 2019

  • Shihab, Mohammed; Bornath, Thomas; Redmer, Ronald
  • Contributions to Plasma Physics, Vol. 59, Issue 4-5
  • DOI: 10.1002/ctpp.201800156

Atomic inner-shell laser at 1.5-ångström wavelength pumped by an X-ray free-electron laser
journal, August 2015

  • Yoneda, Hitoki; Inubushi, Yuichi; Nagamine, Kazunori
  • Nature, Vol. 524, Issue 7566
  • DOI: 10.1038/nature14894

Measurements of continuum lowering in solid-density plasmas created from elements and compounds
journal, May 2016

  • Ciricosta, O.; Vinko, S. M.; Barbrel, B.
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms11713

Density functional theory calculations of continuum lowering in strongly coupled plasmas
journal, March 2014

  • Vinko, S. M.; Ciricosta, O.; Wark, J. S.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms4533

Femtosecond X-ray-induced explosion of C60 at extreme intensity
journal, June 2014

  • Murphy, B. F.; Osipov, T.; Jurek, Z.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5281

Ultrabright X-ray laser scattering for dynamic warm dense matter physics
journal, March 2015


Thermal conductivity measurements of proton-heated warm dense aluminum
journal, August 2017


Transient space localization of electrons ejected from continuum atomic processes in hot dense plasma
journal, December 2018


Lineshape measurements of He- β spectra on the ORION laser facility
journal, October 2016

  • Beiersdorfer, P.; Brown, G. V.; Shepherd, R.
  • Physics of Plasmas, Vol. 23, Issue 10
  • DOI: 10.1063/1.4965233

Spectroscopy of Na I and K I atoms embedded in weakly coupled plasma environment
journal, November 2017

  • Das, Madhulita; Pradhan, Ananta C.
  • Physics of Plasmas, Vol. 24, Issue 11
  • DOI: 10.1063/1.4986022

Equation of motion approach for describing allowed transitions in Ne and Al 3+ under classical and quantum plasmas
journal, April 2018

  • Chaudhuri, Supriya K.; Mukherjee, Prasanta K.; Chaudhuri, Rajat K.
  • Physics of Plasmas, Vol. 25, Issue 4
  • DOI: 10.1063/1.5011791

Fluorescence and absorption spectroscopy for warm dense matter studies and ICF plasma diagnostics
journal, May 2018

  • Hansen, S. B.; Harding, E. C.; Knapp, P. F.
  • Physics of Plasmas, Vol. 25, Issue 5
  • DOI: 10.1063/1.5018580

Challenges of x-ray spectroscopy in investigations of matter under extreme conditions
journal, March 2019

  • Renner, O.; Rosmej, F. B.
  • Matter and Radiation at Extremes, Vol. 4, Issue 2
  • DOI: 10.1063/1.5086344

Quantum statistical approach for ionization potential depression in multi-component dense plasmas
journal, December 2019


Role of lattice structure and low temperature resistivity in fast-electron-beam filamentation in carbon
journal, November 2015


Applications of laser wakefield accelerator-based light sources
journal, September 2016


Analytic model of a multi-electron atom
journal, November 2017

  • Skoromnik, O. D.; Feranchuk, I. D.; Leonau, A. U.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 50, Issue 24
  • DOI: 10.1088/1361-6455/aa92e6

Ionization potential depression in an atomic-solid-plasma picture
journal, April 2018

  • Rosmej, F. B.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 51, Issue 9
  • DOI: 10.1088/1361-6455/aab80f

Characterizing the ionization potential depression in dense carbon plasmas with high-precision spectrally resolved x-ray scattering
journal, November 2018

  • Kraus, D.; Bachmann, B.; Barbrel, B.
  • Plasma Physics and Controlled Fusion, Vol. 61, Issue 1
  • DOI: 10.1088/1361-6587/aadd6c

Intense VUV–xenon-cluster interaction revisited
journal, December 2019


Electron-ion thermal equilibration dynamics in femtosecond heated warm dense copper
journal, February 2018


X-ray scattering measurements on imploding CH spheres at the National Ignition Facility
journal, July 2016


Nuclear excitation by electron capture in optical-laser-generated plasmas
journal, June 2018


Path integral Monte Carlo simulations of warm dense aluminum
journal, June 2018


Measurement of Charged-Particle Stopping in Warm Dense Plasma
journal, May 2015


Short-wavelength free-electron laser sources and science: a review
text, January 2017

  • Seddon, E. A.; Clarke, J. A.; Dunning, D. J.
  • Deutsches Elektronen-Synchrotron, DESY, Hamburg
  • DOI: 10.3204/pubdb-2018-00596

Short-wavelength free-electron laser sources and science: a review
journal, October 2017

  • Seddon, E. A.; Clarke, J. A.; Dunning, D. J.
  • Reports on Progress in Physics, Vol. 80, Issue 11
  • DOI: 10.1088/1361-6633/aa7cca

Analytic model of a multi-electron atom
text, January 2017


Ionization potential depression and Pauli blocking in degenerate plasmas at extreme densities
text, January 2018


Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.