CO2 hydrogenation over oxide-supported PtCo catalysts: The role of the oxide support in determining the product selectivity
Abstract
Abstract By simply changing the oxide support, the selectivity of a metal–oxide catalysts can be tuned. For the CO 2 hydrogenation over PtCo bimetallic catalysts supported on different reducible oxides (CeO 2 , ZrO 2 , and TiO 2 ), replacing a TiO 2 support by CeO 2 or ZrO 2 selectively strengthens the binding of C,O‐bound and O‐bound species at the PtCo–oxide interface, leading to a different product selectivity. These results reveal mechanistic insights into how the catalytic performance of metal–oxide catalysts can be fine‐tuned.
- Authors:
-
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Columbia Univ., New York, NY (United States)
- Chinese Academy of Science, Dalian (China)
- Brookhaven National Lab. (BNL), Upton, NY (United States); Columbia Univ., New York, NY (United States)
- Publication Date:
- Research Org.:
- Brookhaven National Laboratory (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1333197
- Alternate Identifier(s):
- OSTI ID: 1401667
- Report Number(s):
- BNL-113193-2016-JA
Journal ID: ISSN 1433-7851; R&D Project: CO035; KC0302010
- Grant/Contract Number:
- SC00112704
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Angewandte Chemie (International Edition)
- Additional Journal Information:
- Journal Name: Angewandte Chemie (International Edition); Journal Volume: 55; Journal Issue: 28; Journal ID: ISSN 1433-7851
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Citation Formats
Kattel, Shyam, Yu, Weiting, Yang, Xiaofang, Yan, Binhang, Huang, Yanqiang, Wan, Weiming, Liu, Ping, and Chen, Jingguang G. CO2 hydrogenation over oxide-supported PtCo catalysts: The role of the oxide support in determining the product selectivity. United States: N. p., 2016.
Web. doi:10.1002/anie.201601661.
Kattel, Shyam, Yu, Weiting, Yang, Xiaofang, Yan, Binhang, Huang, Yanqiang, Wan, Weiming, Liu, Ping, & Chen, Jingguang G. CO2 hydrogenation over oxide-supported PtCo catalysts: The role of the oxide support in determining the product selectivity. United States. https://doi.org/10.1002/anie.201601661
Kattel, Shyam, Yu, Weiting, Yang, Xiaofang, Yan, Binhang, Huang, Yanqiang, Wan, Weiming, Liu, Ping, and Chen, Jingguang G. Mon .
"CO2 hydrogenation over oxide-supported PtCo catalysts: The role of the oxide support in determining the product selectivity". United States. https://doi.org/10.1002/anie.201601661. https://www.osti.gov/servlets/purl/1333197.
@article{osti_1333197,
title = {CO2 hydrogenation over oxide-supported PtCo catalysts: The role of the oxide support in determining the product selectivity},
author = {Kattel, Shyam and Yu, Weiting and Yang, Xiaofang and Yan, Binhang and Huang, Yanqiang and Wan, Weiming and Liu, Ping and Chen, Jingguang G.},
abstractNote = {Abstract By simply changing the oxide support, the selectivity of a metal–oxide catalysts can be tuned. For the CO 2 hydrogenation over PtCo bimetallic catalysts supported on different reducible oxides (CeO 2 , ZrO 2 , and TiO 2 ), replacing a TiO 2 support by CeO 2 or ZrO 2 selectively strengthens the binding of C,O‐bound and O‐bound species at the PtCo–oxide interface, leading to a different product selectivity. These results reveal mechanistic insights into how the catalytic performance of metal–oxide catalysts can be fine‐tuned.},
doi = {10.1002/anie.201601661},
journal = {Angewandte Chemie (International Edition)},
number = 28,
volume = 55,
place = {United States},
year = {Mon May 09 00:00:00 EDT 2016},
month = {Mon May 09 00:00:00 EDT 2016}
}
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