Fabrication of efficient low-bandgap perovskite solar cells by combining formamidinium tin iodide with methylammonium lead iodide
Abstract
Mixed tin (Sn)-lead (Pb) perovskites with high Sn content exhibit low bandgaps suitable for fabricating the bottom cell of perovskite-based tandem solar cells. In this work, we report on the fabrication of efficient mixed Sn-Pb perovskite solar cells using precursors combining formamidinium tin iodide (FASnI3) and methylammonium lead iodide (MAPbI3). The best-performing cell fabricated using a (FASnI3)0.6(MAPbI3)0.4 absorber with an absorption edge of ~1.2 eV achieved a power conversion efficiency (PCE) of 15.08 (15.00)% with an open-circuit voltage of 0.795 (0.799) V, a short-circuit current density of 26.86(26.82) mA/cm2, and a fill factor of 70.6(70.0)% when measured under forward (reverse) voltage scan. In conclusion, the average PCE of 50 cells we have fabricated is 14.39 ± 0.33%, indicating good reproducibility.
- Authors:
-
- The Univ. of Toledo, Toledo, OH (United States); Southeast Univ., Nanjing (China)
- The Univ. of Toledo, Toledo, OH (United States)
- The Univ. of Toledo, Toledo, OH (United States); Wuhan Univ., Wuhan (China)
- Wuhan Univ., Wuhan (China)
- National Renewable Energy Lab. (NREL), Golden, CO (United States)
- Southeast Univ., Nanjing (China)
- Publication Date:
- Research Org.:
- National Renewable Energy Laboratory (NREL), Golden, CO (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE)
- OSTI Identifier:
- 1328732
- Report Number(s):
- NREL/JA-5900-67260
Journal ID: ISSN 0002-7863
- Grant/Contract Number:
- AC36-08GO28308
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of the American Chemical Society
- Additional Journal Information:
- Journal Volume: 138; Journal Issue: 38; Journal ID: ISSN 0002-7863
- Publisher:
- American Chemical Society (ACS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; 36 MATERIALS SCIENCE; perovskites solar cells; precusors; methylammonium lead iodide; formamidinium tin iodide
Citation Formats
Liao, Weiqiang, Zhao, Dewei, Yu, Yue, Shrestha, Niraj, Ghimire, Kiran, Grice, Corey R., Wang, Changlei, Xiao, Yuqing, Cimaroli, Alexander J., Ellingson, Randy J., Podraza, Nikolas J., Zhu, Kai, Xiong, Ren -Gen, and Yan, Yanfa. Fabrication of efficient low-bandgap perovskite solar cells by combining formamidinium tin iodide with methylammonium lead iodide. United States: N. p., 2016.
Web. doi:10.1021/jacs.6b08337.
Liao, Weiqiang, Zhao, Dewei, Yu, Yue, Shrestha, Niraj, Ghimire, Kiran, Grice, Corey R., Wang, Changlei, Xiao, Yuqing, Cimaroli, Alexander J., Ellingson, Randy J., Podraza, Nikolas J., Zhu, Kai, Xiong, Ren -Gen, & Yan, Yanfa. Fabrication of efficient low-bandgap perovskite solar cells by combining formamidinium tin iodide with methylammonium lead iodide. United States. https://doi.org/10.1021/jacs.6b08337
Liao, Weiqiang, Zhao, Dewei, Yu, Yue, Shrestha, Niraj, Ghimire, Kiran, Grice, Corey R., Wang, Changlei, Xiao, Yuqing, Cimaroli, Alexander J., Ellingson, Randy J., Podraza, Nikolas J., Zhu, Kai, Xiong, Ren -Gen, and Yan, Yanfa. Tue .
"Fabrication of efficient low-bandgap perovskite solar cells by combining formamidinium tin iodide with methylammonium lead iodide". United States. https://doi.org/10.1021/jacs.6b08337. https://www.osti.gov/servlets/purl/1328732.
@article{osti_1328732,
title = {Fabrication of efficient low-bandgap perovskite solar cells by combining formamidinium tin iodide with methylammonium lead iodide},
author = {Liao, Weiqiang and Zhao, Dewei and Yu, Yue and Shrestha, Niraj and Ghimire, Kiran and Grice, Corey R. and Wang, Changlei and Xiao, Yuqing and Cimaroli, Alexander J. and Ellingson, Randy J. and Podraza, Nikolas J. and Zhu, Kai and Xiong, Ren -Gen and Yan, Yanfa},
abstractNote = {Mixed tin (Sn)-lead (Pb) perovskites with high Sn content exhibit low bandgaps suitable for fabricating the bottom cell of perovskite-based tandem solar cells. In this work, we report on the fabrication of efficient mixed Sn-Pb perovskite solar cells using precursors combining formamidinium tin iodide (FASnI3) and methylammonium lead iodide (MAPbI3). The best-performing cell fabricated using a (FASnI3)0.6(MAPbI3)0.4 absorber with an absorption edge of ~1.2 eV achieved a power conversion efficiency (PCE) of 15.08 (15.00)% with an open-circuit voltage of 0.795 (0.799) V, a short-circuit current density of 26.86(26.82) mA/cm2, and a fill factor of 70.6(70.0)% when measured under forward (reverse) voltage scan. In conclusion, the average PCE of 50 cells we have fabricated is 14.39 ± 0.33%, indicating good reproducibility.},
doi = {10.1021/jacs.6b08337},
journal = {Journal of the American Chemical Society},
number = 38,
volume = 138,
place = {United States},
year = {Tue Sep 13 00:00:00 EDT 2016},
month = {Tue Sep 13 00:00:00 EDT 2016}
}
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- Li, Can; Ma, Ruiman; He, Xinjun
- Advanced Energy Materials, Vol. 10, Issue 8
Influence of chromium hyperdoping on the electronic structure of CH3NH3PbI3 perovskite: a first-principles insight
journal, February 2018
- García, Gregorio; Palacios, Pablo; Menéndez-Proupin, Eduardo
- Scientific Reports, Vol. 8, Issue 1
Mixed-Organic-Cation Tin Iodide for Lead-Free Perovskite Solar Cells with an Efficiency of 8.12%
journal, July 2017
- Zhao, Ziran; Gu, Feidan; Li, Yunlong
- Advanced Science, Vol. 4, Issue 11
Fabrication and Characterization of CH 3 NH 3 PbI 3 Perovskite Solar Cells Added with Polysilanes
journal, October 2018
- Oku, Takeo; Nomura, Junya; Suzuki, Atsushi
- International Journal of Photoenergy, Vol. 2018
Three-dimensional organic–inorganic hybrid sodium halide perovskite: C 4 H 12 N 2 ·NaI 3 and a hydrogen-bonded supramolecular three-dimensional network in 3C 4 H 12 N 2 ·NaI 4 ·3I·H 2 O
journal, May 2018
- Chen, Xiao-Gang; Gao, Ji-Xing; Hua, Xiu-Ni
- Acta Crystallographica Section C Structural Chemistry, Vol. 74, Issue 6
Understanding and Eliminating Hysteresis for Highly Efficient Planar Perovskite Solar Cells
journal, May 2017
- Wang, Changlei; Xiao, Chuanxiao; Yu, Yue
- Advanced Energy Materials, Vol. 7, Issue 17
Highly Efficient Porphyrin-Based OPV/Perovskite Hybrid Solar Cells with Extended Photoresponse and High Fill Factor
journal, November 2017
- Gao, Ke; Zhu, Zonglong; Xu, Bo
- Advanced Materials, Vol. 29, Issue 47
Enhanced Uniformity and Stability of Pb–Sn Perovskite Solar Cells via Me 4 NBr Passivation
journal, May 2019
- Du, Xingzhi; Qiu, Renzheng; Zou, Taoyu
- Advanced Materials Interfaces, Vol. 6, Issue 14
Highly Sensitive Low-Bandgap Perovskite Photodetectors with Response from Ultraviolet to the Near-Infrared Region
journal, September 2017
- Wang, Wenbin; Zhao, Dewei; Zhang, Fujun
- Advanced Functional Materials, Vol. 27, Issue 42
Lead-Free Hybrid Perovskite Absorbers for Viable Application: Can We Eat the Cake and Have It too?
journal, November 2017
- Liang, Lusheng; Gao, Peng
- Advanced Science, Vol. 5, Issue 2
Combining Efficiency and Stability in Mixed Tin–Lead Perovskite Solar Cells by Capping Grains with an Ultrathin 2D Layer
journal, March 2020
- Wei, Mingyang; Xiao, Ke; Walters, Grant
- Advanced Materials, Vol. 32, Issue 12
FAPb 0.5 Sn 0.5 I 3 : A Narrow Bandgap Perovskite Synthesized through Evaporation Methods for Solar Cell Applications
journal, August 2019
- Igual-Muñoz, Ana M.; Ávila, Jorge; Boix, Pablo P.
- Solar RRL, Vol. 4, Issue 2
Perovskite Photovoltaics: The Significant Role of Ligands in Film Formation, Passivation, and Stability
journal, January 2019
- Zhang, Hong; Nazeeruddin, Mohammad Khaja; Choy, Wallace C. H.
- Advanced Materials, Vol. 31, Issue 8
Doping of [In2(phen) 3 Cl 6 ]·CH 3 CN·2H 2 O Indium-Based Metal-Organic Framework into Hole Transport Layer for Enhancing Perovskite Solar Cell Efficiencies
journal, April 2018
- Li, Mengru; Xia, Debin; Yang, Yulin
- Advanced Energy Materials, Vol. 8, Issue 12
Improved Efficiency and Stability of Pb/Sn Binary Perovskite Solar Cells Fabricated by Galvanic Displacement Reaction
journal, January 2019
- Zhu, Zonglong; Li, Nan; Zhao, Dongbin
- Advanced Energy Materials, Vol. 9, Issue 7
Homogenous Alloys of Formamidinium Lead Triiodide and Cesium Tin Triiodide for Efficient Ideal‐Bandgap Perovskite Solar Cells
journal, July 2017
- Zong, Yingxia; Wang, Ning; Zhang, Lin
- Angewandte Chemie, Vol. 129, Issue 41
Crystallization, Properties, and Challenges of Low-Bandgap Sn-Pb Binary Perovskites
journal, July 2018
- Zhu, Hugh Lu; Choy, Wallace C. H.
- Solar RRL, Vol. 2, Issue 10
FAPb 0.5 Sn 0.5 I 3 : A Narrow Bandgap Perovskite Synthesized through Evaporation Methods for Solar Cell Applications
journal, August 2019
- Igual-Muñoz, Ana M.; Ávila, Jorge; Boix, Pablo P.
- Solar RRL, Vol. 4, Issue 2
Low-bandgap mixed tin–lead iodide perovskite absorbers with long carrier lifetimes for all-perovskite tandem solar cells
journal, March 2017
- Zhao, Dewei; Yu, Yue; Wang, Changlei
- Nature Energy, Vol. 2, Issue 4
Controlling the Growth Kinetics and Optoelectronic Properties of 2D/3D Lead–Tin Perovskite Heterojunctions
text, January 2019
- Ruggeri, Edoardo; Anaya, Miguel; Gałkowski, Krzysztof
- Apollo - University of Cambridge Repository
Vacuum‐Assisted Growth of Low‐Bandgap Thin Films (FA$_{0.8}$MA$_{0.2}$Sn$_{0.5}$Pb$_{0.5}$I$_{3}$) for All‐Perovskite Tandem Solar Cells
text, January 2020
- Abdollahi Nejand, Bahram; Hossain, Ihteaz M.; Jakoby, Marius
- Karlsruhe
Tin(iv) dopant removal through anti-solvent engineering enabling tin based perovskite solar cells with high charge carrier mobilities
text, January 2019
- Bandara, Rmi; Jayawardena, Kdgi; Adeyemo, Stephanie
- Apollo - University of Cambridge Repository
High Open-Circuit Voltages in Tin-Rich Low-Bandgap Perovskite-Based Planar Heterojunction Photovoltaics
journal, November 2016
- Zhao, Baodan; Abdi-Jalebi, Mojtaba; Tabachnyk, Maxim
- Advanced Materials, Vol. 29, Issue 2
Tailoring metal halide perovskites through metal substitution: Influence on photovoltaic and material properties
text, January 2017
- Klug, Mt; Osherov, A.; Haghighirad, Aa
- Apollo - University of Cambridge Repository
Mixed-Organic-Cation Tin Iodide for Lead-Free Perovskite Solar Cells with an Efficiency of 8.12%
journal, July 2017
- Zhao, Ziran; Gu, Feidan; Li, Yunlong
- Advanced Science, Vol. 4, Issue 11
Lead-Free Hybrid Perovskite Absorbers for Viable Application: Can We Eat the Cake and Have It too?
journal, November 2017
- Liang, Lusheng; Gao, Peng
- Advanced Science, Vol. 5, Issue 2
Long-lived hot-carrier light emission and large blue shift in formamidinium tin triiodide perovskites
journal, January 2018
- Fang, Hong-Hua; Adjokatse, Sampson; Shao, Shuyan
- Nature Communications, Vol. 9, Issue 1
Influence of chromium hyperdoping on the electronic structure of CH3NH3PbI3 perovskite: a first-principles insight
journal, February 2018
- García, Gregorio; Palacios, Pablo; Menéndez-Proupin, Eduardo
- Scientific Reports, Vol. 8, Issue 1
The effect of oxygen on the efficiency of planar p–i–n metal halide perovskite solar cells with a PEDOT:PSS hole transport layer
journal, January 2018
- Bruijnaers, Bardo J.; Schiepers, Eric; Weijtens, Christ H. L.
- Journal of Materials Chemistry A, Vol. 6, Issue 16