Title: Ultrafast energy- and momentum-resolved dynamics of magnetic correlations in the photo-doped Mott insulator Sr₂IrO₄

Abstract

Measuring how the magnetic correlations evolve in doped Mott insulators has greatly improved our understanding of the pseudogap, non-Fermi liquids and high-temperature superconductivity^{1, 2, 3, 4}. Recently, photo-excitation has been used to induce similarly exotic states transiently^{5, 6, 7}. However, the lack of available probes of magnetic correlations in the time domain hinders our understanding of these photo-induced states and how they could be controlled. Here, we implement magnetic resonant inelastic X-ray scattering at a free-electron laser to directly determine the magnetic dynamics after photo-doping the Mott insulator Sr₂IrO₄. We find that the non-equilibrium state, 2 ps after the excitation, exhibits strongly suppressed long-range magnetic order, but hosts photo-carriers that induce strong, non-thermal magnetic correlations. These two-dimensional (2D) in-plane Néel correlations recover within a few picoseconds, whereas the three-dimensional (3D) long-range magnetic order restores on a fluence-dependent timescale of a few hundred picoseconds. In conclusion, the marked difference in these two timescales implies that the dimensionality of magnetic correlations is vital for our understanding of ultrafast magnetic dynamics.

Authors:

Dean, M. P. M.  ^[1];

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• Search DOE PAGES for ORCID "0000-0001-5139-3543"

Cao, Y.  ^[1];

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• Search DOE PAGES for ORCID "0000-0002-3989-158X"

Liu, X. ^[2]; Wall, S.  ^[3];

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Zhu, D. ^[4]; Mankowsky, R. ^[5]; Thampy, V. ^[1]; Chen, X. M. ^[1]; Vale, J. G. ^[6]; Casa, D. ^[7]; Kim, Jungho ^[7]; Said, A. H. ^[7]; Juhas, P. ^[1]; Alonso-Mori, R. ^[4]; Glownia, J. M. ^[4]; Robert, A. ^[4]; Robinson, J. ^[4]; Sikorski, M. ^[4]; Song, S.  ^[4];

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Kozina, M. ^[4] more »; Lemke, H. ^[4]; Patthey, L. ^[8]; Owada, S. ^[9]; Katayama, T. ^[10]; Yabashi, M.  ^[9];

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Tanaka, Yoshikazu ^[9]; Togashi, T. ^[10]; Liu, J. ^[11]; Rayan Serrao, C.  ^[12];

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• Search DOE PAGES for ORCID "0000-0003-4737-0693"

Kim, B. J. ^[13]; Huber, L. ^[14]; Chang, C. -L. ^[15]; McMorrow, D. F. ^[6]; Forst, M. ^[5]; Hill, J. P. ^[1] « less

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+ Show Author Affiliations

1. Brookhaven National Lab. (BNL), Upton, NY (United States)
2. Chinese Academy of Sciences (CAS), Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China)
3. The Barcelona Institute of Science and Technology, Castelldefels (Barcelona) (Spain)
4. SLAC National Accelerator Lab., Menlo Park, CA (United States)
5. Max Planck Institute for the Structure and Dynamics of Matter, Hamburg (Germany)
6. Univ. College London, London (United Kingdom)
7. Argonne National Lab. (ANL), Argonne, IL (United States)
8. Paul Scherrer Inst. (PSI), Villigen (Switzerland)
9. RIKEN SPring-8 Center, Hyogo (Japan)
10. Japan Synchrotron Radiation Institute, Hyogo (Japan)
11. Univ. of Tennessee, Knoxville, TN (United States)
12. Univ. of California, Berkeley, CA (United States)
13. Max Planck Institute for Solid State Research, Stuttgart (Germany)
14. ETH Zurich, Zurich (Switzerland)
15. Univ. of Groningen, Groningen (The Netherlands)

Publication Date:

Mon May 09 00:00:00 EDT 2016

Research Org.:

Brookhaven National Lab. (BNL), Upton, NY (United States)

Sponsoring Org.:

USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:

1311357

Report Number(s):

BNL-112461-2016-JA
Journal ID: ISSN 1476-1122; R&D Project: PO011; KC0201060

Grant/Contract Number:  

SC00112704

Resource Type:

Accepted Manuscript

Journal Name:

Nature Materials

Additional Journal Information:

Journal Volume: 15; Journal Issue: 6; Journal ID: ISSN 1476-1122

Publisher:

Nature Publishing Group

Country of Publication:

United States

Language:

English

Subject:

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY