Nuclear forward scattering of synchrotron radiation by 99Ru
Abstract
In this study, we measured nuclear forward scattering spectra utilizing the 99Ru transition, 89.571(3) keV, with a notably mixed E2/M1 multipolarity. The extension of the standard evaluation routines to include mixed multipolarity allows us to extract electric and magnetic hyperfine interactions from 99Ru-containing compounds. This paves the way for several other high-energy Mössbauer transitions, E~90 keV. Lastly, the high energy of such transitions allows for operando nuclear forward scattering studies in real devices.
- Authors:
-
- European Synchrotron Radiation Facility (ESRF), Grenoble (France)
- Julich Research Centre (Germany). Julich Centre for Neutron Science (JCNS); Univ. of Liege, (Belgium). Faculty of Sciences
- Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
- Julich Research Centre (Germany). Julich Centre for Neutron Science (JCNS)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Univ. Montpellier II, Montpellier (France); Network Electrochemical Energy Storage (France)
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1265272
- Alternate Identifier(s):
- OSTI ID: 1180345
- Grant/Contract Number:
- AC05-00OR22725; VH NG-407
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review Letters
- Additional Journal Information:
- Journal Volume: 113; Journal Issue: 14; Journal ID: ISSN 0031-9007
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY
Citation Formats
Bessas, D., Merkel, D. G., Chumakov, A. I., Ruffer, R., Hermann, Raphael P., Sergueev, I., Mahmoud, A., Klobes, B., McGuire, Michael A., Sougrati, M. T., and Stievano, L. Nuclear forward scattering of synchrotron radiation by 99Ru. United States: N. p., 2014.
Web. doi:10.1103/PhysRevLett.113.147601.
Bessas, D., Merkel, D. G., Chumakov, A. I., Ruffer, R., Hermann, Raphael P., Sergueev, I., Mahmoud, A., Klobes, B., McGuire, Michael A., Sougrati, M. T., & Stievano, L. Nuclear forward scattering of synchrotron radiation by 99Ru. United States. https://doi.org/10.1103/PhysRevLett.113.147601
Bessas, D., Merkel, D. G., Chumakov, A. I., Ruffer, R., Hermann, Raphael P., Sergueev, I., Mahmoud, A., Klobes, B., McGuire, Michael A., Sougrati, M. T., and Stievano, L. Fri .
"Nuclear forward scattering of synchrotron radiation by 99Ru". United States. https://doi.org/10.1103/PhysRevLett.113.147601. https://www.osti.gov/servlets/purl/1265272.
@article{osti_1265272,
title = {Nuclear forward scattering of synchrotron radiation by 99Ru},
author = {Bessas, D. and Merkel, D. G. and Chumakov, A. I. and Ruffer, R. and Hermann, Raphael P. and Sergueev, I. and Mahmoud, A. and Klobes, B. and McGuire, Michael A. and Sougrati, M. T. and Stievano, L.},
abstractNote = {In this study, we measured nuclear forward scattering spectra utilizing the 99Ru transition, 89.571(3) keV, with a notably mixed E2/M1 multipolarity. The extension of the standard evaluation routines to include mixed multipolarity allows us to extract electric and magnetic hyperfine interactions from 99Ru-containing compounds. This paves the way for several other high-energy Mössbauer transitions, E~90 keV. Lastly, the high energy of such transitions allows for operando nuclear forward scattering studies in real devices.},
doi = {10.1103/PhysRevLett.113.147601},
journal = {Physical Review Letters},
number = 14,
volume = 113,
place = {United States},
year = {Fri Oct 03 00:00:00 EDT 2014},
month = {Fri Oct 03 00:00:00 EDT 2014}
}
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