Anisotropic Exchange within Decoupled Tetrahedra in the Quantum Breathing Pyrochlore Ba3Yb2Zn5O11

Rau, J. G.; Wu, L. S.; May, A. F.; Poudel, L.; Winn, B.; Garlea, V. O.; Huq, A.; Whitfield, P.; Taylor, A. E.; Lumsden, M. D.; Gingras, M. J.  P.; Christianson, A. D.

doi:10.1103/PhysRevLett.116.257204

Title: Anisotropic Exchange within Decoupled Tetrahedra in the Quantum Breathing Pyrochlore ${Ba}_{3} {Yb}_{2} {Zn}_{5} O_{11}$

Abstract

The low energy spin excitation spectrum of the breathing pyrochlore ${Ba}_{3} {Yb}_{2} {Zn}_{5} O_{11}$ has been investigated with inelastic neutron scattering. Several nearly resolution limited modes with no observable dispersion are observed at 250 mK while, at elevated temperatures, transitions between excited levels become visible. To gain deeper insight, a theoretical model of isolated Yb³⁺ tetrahedra parametrized by four anisotropic exchange constants is constructed. The model reproduces the inelastic neutron scattering data, specific heat, and magnetic susceptibility with high fidelity. The fitted exchange parameters reveal a Heisenberg antiferromagnet with a very large Dzyaloshinskii-Moriya interaction. Ultimately, using this model, we predict the appearance of an unusual octupolar paramagnet at low temperatures and speculate on the development of inter-tetrahedron correlations.

Authors:

Rau, J. G. ^[1]; Wu, L. S. ^[2]; May, A. F. ^[3]; Poudel, L. ^[4]; Winn, B. ^[2]; Garlea, V. O. ^[2]; Huq, A. ^[5]; Whitfield, P. ^[5]; Taylor, A. E. ^[2]; Lumsden, M. D. ^[2]; Gingras, M. J. P. ^[6]; Christianson, A. D. ^[4]

Univ. of Waterloo, ON (Canada)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Quantum Condensed Matter Division
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Quantum Condensed Matter Division; Univ. of Tennessee, Knoxville, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Chemical and Engineering Materials Division
Univ. of Waterloo, ON (Canada); Perimeter Inst. for Theoretical Physics, Waterloo, ON (Canada)

Publication Date:: Fri Jun 24 00:00:00 EDT 2016

Research Org.:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Spallation Neutron Source (SNS)

Sponsoring Org.:: USDOE Office of Science (SC)

OSTI Identifier:: 1260086

Alternate Identifier(s):: OSTI ID: 1259338

Grant/Contract Number:: AC05-00OR22725

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review Letters

Additional Journal Information:: Journal Volume: 116; Journal Issue: 25; Journal ID: ISSN 0031-9007

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS

Citation Formats


                    Rau, J. G., Wu, L. S., May, A. F., Poudel, L., Winn, B., Garlea, V. O., Huq, A., Whitfield, P., Taylor, A. E., Lumsden, M. D., Gingras, M. J.  P., and Christianson, A. D. Anisotropic Exchange within Decoupled Tetrahedra in the Quantum Breathing Pyrochlore Ba3Yb2Zn5O11.  United States: N. p., 2016. 
Web.  doi:10.1103/PhysRevLett.116.257204.

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                    Rau, J. G., Wu, L. S., May, A. F., Poudel, L., Winn, B., Garlea, V. O., Huq, A., Whitfield, P., Taylor, A. E., Lumsden, M. D., Gingras, M. J.  P., & Christianson, A. D. Anisotropic Exchange within Decoupled Tetrahedra in the Quantum Breathing Pyrochlore Ba3Yb2Zn5O11.  United States.  https://doi.org/10.1103/PhysRevLett.116.257204

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                    Rau, J. G., Wu, L. S., May, A. F., Poudel, L., Winn, B., Garlea, V. O., Huq, A., Whitfield, P., Taylor, A. E., Lumsden, M. D., Gingras, M. J.  P., and Christianson, A. D. Fri .  
"Anisotropic Exchange within Decoupled Tetrahedra in the Quantum Breathing Pyrochlore Ba3Yb2Zn5O11".  United States.  https://doi.org/10.1103/PhysRevLett.116.257204.  https://www.osti.gov/servlets/purl/1260086.

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@article{osti_1260086,

  title        = {Anisotropic Exchange within Decoupled Tetrahedra in the Quantum Breathing Pyrochlore Ba3Yb2Zn5O11},

  author       = {Rau, J. G. and Wu, L. S. and May, A. F. and Poudel, L. and Winn, B. and Garlea, V. O. and Huq, A. and Whitfield, P. and Taylor, A. E. and Lumsden, M. D. and Gingras, M. J.  P. and Christianson, A. D.},

  abstractNote = {The low energy spin excitation spectrum of the breathing pyrochlore Ba3Yb2Zn5O11 has been investigated with inelastic neutron scattering. Several nearly resolution limited modes with no observable dispersion are observed at 250 mK while, at elevated temperatures, transitions between excited levels become visible. To gain deeper insight, a theoretical model of isolated Yb3+ tetrahedra parametrized by four anisotropic exchange constants is constructed. The model reproduces the inelastic neutron scattering data, specific heat, and magnetic susceptibility with high fidelity. The fitted exchange parameters reveal a Heisenberg antiferromagnet with a very large Dzyaloshinskii-Moriya interaction. Ultimately, using this model, we predict the appearance of an unusual octupolar paramagnet at low temperatures and speculate on the development of inter-tetrahedron correlations.},

  doi          = {10.1103/PhysRevLett.116.257204},

  journal      = {Physical Review Letters},

  number       = 25,

  volume       = 116,

  place        = {United States},

  year         = {Fri Jun 24 00:00:00 EDT 2016},

  month        = {Fri Jun 24 00:00:00 EDT 2016}

}

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Works referenced in this record:

Weak antiferromagnetism and dimer order in quantum systems of coupled tetrahedra
journal, December 2004

Kotov, Valeri N.; Zhitomirsky, Michael E.; Elhajal, Maged
Physical Review B, Vol. 70, Issue 21
DOI: 10.1103/physrevb.70.214401

Zur Kristallchemie von Ba3In2Zn5O11. Ein tOxoindat/zinkatsol;zinkat mit Zn10O20- und In4O16-Makropolyedern und erstmals O2? in tetraedrischer Koordination durch Zn2+
journal, March 1993

Scheikowski, M.; M�ller-Buschbaum, Hk.
Zeitschrift f�r anorganische und allgemeine Chemie, Vol. 619, Issue 3
DOI: 10.1002/zaac.19936190322

Magnetic Phase Diagram of the Breathing Pyrochlore Antiferromagnet LiGa ₁₋ _x In _x Cr ₄ O ₈
journal, April 2015

Okamoto, Yoshihiko; Nilsen, Gøran J.; Nakazono, Taishi
Journal of the Physical Society of Japan, Vol. 84, Issue 4
DOI: 10.7566/jpsj.84.043707

Crystal Field Excitations in the Breathing Pyrochlore Antiferromagnet Ba ₃ Yb ₂ Zn ₅ O ₁₁
journal, March 2016

Haku, Tendai; Soda, Minoru; Sera, Masakazu
Journal of the Physical Society of Japan, Vol. 85, Issue 3
DOI: 10.7566/jpsj.85.034721

Frustrated Spin Systems
book, November 2012

Diep, H. T.
World Scientific
DOI: 10.1142/8676

Patterns of symmetry breaking in systems of coupled tetrahedra
journal, March 2004

Kotov, Valeri N.; Zhitomirsky, Michael E.; Elhajal, Maged
Journal of Physics: Condensed Matter, Vol. 16, Issue 11
DOI: 10.1088/0953-8984/16/11/047

Magnetic order in a S= frustrated antiferromagnet on a square lattice
journal, May 2004

Bombardi, A.; Paolasini, L.; Carretta, P.
Journal of Magnetism and Magnetic Materials, Vol. 272-276
DOI: 10.1016/j.jmmm.2003.12.498

Powgen: A third-generation highresolution high-throughput powder diffraction instrument at the Spallation Neutron Source
book, December 2011

Huq, A.; Hodges, J. P.; Gourdon, O.
European Powder Diffraction Conference; August 2010, Darmstadt, Germany
DOI: 10.1524/9783486991321-024

Composite Spin and Quadrupole Wave in the Ordered Phase of Tb _2+x Ti _2-x O _7+y
journal, June 2015

Kadowaki, H.; Takatsu, H.; Taniguchi, T.
SPIN, Vol. 05, Issue 02
DOI: 10.1142/s2010324715400032

Spin liquids in frustrated magnets
journal, March 2010

Balents, Leon
Nature, Vol. 464, Issue 7286
DOI: 10.1038/nature08917

Ising-like order by disorder in the pyrochlore antiferromagnet with Dzyaloshinskii-Moriya interactions
journal, December 2008

Canals, B.; Elhajal, M.; Lacroix, C.
Physical Review B, Vol. 78, Issue 21
DOI: 10.1103/physrevb.78.214431

Synthese und Kristallstruktur von Ba6Lu4Zn10O22 mit [OBa6]-Oktaedern
journal, January 1996

Rabbow, Ch.; M�ller-Buschbaum, Hk.
Zeitschrift f�r anorganische und allgemeine Chemie, Vol. 622, Issue 1
DOI: 10.1002/zaac.19966220115

Quantum spin configurations in ${Tb}_{2} {Ti}_{2} O_{7}$
journal, June 2007

Curnoe, S. H.
Physical Review B, Vol. 75, Issue 21
DOI: 10.1103/physrevb.75.212404

Dzyaloshinsky-Moriya-induced order in the spin-liquid phase of the $S = 1 ∕ 2$ pyrochlore antiferromagnet
journal, July 2005

Kotov, Valeri N.; Elhajal, Maged; Zhitomirsky, Michael E.
Physical Review B, Vol. 72, Issue 1
DOI: 10.1103/physrevb.72.014421

Design and operation of the wide angular-range chopper spectrometer ARCS at the Spallation Neutron Source
journal, January 2012

Abernathy, D. L.; Stone, M. B.; Loguillo, M. J.
Review of Scientific Instruments, Vol. 83, Issue 1
DOI: 10.1063/1.3680104

Higgs transition from a magnetic Coulomb liquid to a ferromagnet in Yb2Ti2O7
journal, January 2012

Chang, Lieh-Jeng; Onoda, Shigeki; Su, Yixi
Nature Communications, Vol. 3, Issue 1
DOI: 10.1038/ncomms1989

Quantum spin ice: a search for gapless quantum spin liquids in pyrochlore magnets
journal, May 2014

Gingras, M. J. P.; McClarty, P. A.
Reports on Progress in Physics, Vol. 77, Issue 5
DOI: 10.1088/0034-4885/77/5/056501

Quantum fluctuations in spin-ice-like Pr2Zr2O7
journal, June 2013

Kimura, K.; Nakatsuji, S.; Wen, J-J.
Nature Communications, Vol. 4, Issue 1
DOI: 10.1038/ncomms2914

Recent progress on HYSPEC, and its polarization analysis capabilities
journal, January 2015

Winn, Barry; Filges, Uwe; Garlea, V. Ovidiu
EPJ Web of Conferences, Vol. 83
DOI: 10.1051/epjconf/20158303017

Unusual ordered phases of highly frustrated magnets: a review
journal, April 2015

Starykh, Oleg A.
Reports on Progress in Physics, Vol. 78, Issue 5
DOI: 10.1088/0034-4885/78/5/052502

Frustrated Spin Systems
book, January 2005

Diep, H. T.
World Scientific
DOI: 10.1142/5697

The frustration-based approach of supercooled liquids and the glass transition: a review and critical assessment
journal, December 2005

Tarjus, G.; Kivelson, S. A.; Nussinov, Z.
Journal of Physics: Condensed Matter, Vol. 17, Issue 50
DOI: 10.1088/0953-8984/17/50/R01

Multipolar interactions in $f$ -electron systems: The paradigm of actinide dioxides
journal, June 2009

Santini, Paolo; Carretta, Stefano; Amoretti, Giuseppe
Reviews of Modern Physics, Vol. 81, Issue 2
DOI: 10.1103/RevModPhys.81.807

Paramagnetism in the kagome compounds $(Zn, Mg, Cd) {Cu}_{3} {(OH)}_{6} {Cl}_{2}$
journal, December 2015

Iqbal, Yasir; Jeschke, Harald O.; Reuther, Johannes
Physical Review B, Vol. 92, Issue 22
DOI: 10.1103/PhysRevB.92.220404

Kapellasite: A Kagome Quantum Spin Liquid with Competing Interactions
journal, July 2012

Fåk, B.; Kermarrec, E.; Messio, L.
Physical Review Letters, Vol. 109, Issue 3
DOI: 10.1103/PhysRevLett.109.037208

Quadrupolar Phases of the $S = 1$ Bilinear-Biquadratic Heisenberg Model on the Triangular Lattice
journal, August 2006

Läuchli, Andreas; Mila, Frédéric; Penc, Karlo
Physical Review Letters, Vol. 97, Issue 8
DOI: 10.1103/PhysRevLett.97.087205

Dynamically Induced Frustration as a Route to a Quantum Spin Ice State in ${Tb}_{2} {Ti}_{2} O_{7}$ via Virtual Crystal Field Excitations and Quantum Many-Body Effects
journal, April 2007

Molavian, Hamid R.; Gingras, Michel J. P.; Canals, Benjamin
Physical Review Letters, Vol. 98, Issue 15
DOI: 10.1103/PhysRevLett.98.157204

Quantum Melting of Spin Ice: Emergent Cooperative Quadrupole and Chirality
journal, July 2010

Onoda, Shigeki; Tanaka, Yoichi
Physical Review Letters, Vol. 105, Issue 4
DOI: 10.1103/PhysRevLett.105.047201

Quantum Excitations in Quantum Spin Ice
journal, October 2011

Ross, Kate A.; Savary, Lucile; Gaulin, Bruce D.
Physical Review X, Vol. 1, Issue 2
DOI: 10.1103/PhysRevX.1.021002

Order by Quantum Disorder in ${Er}_{2} {Ti}_{2} O_{7}$
journal, October 2012

Savary, Lucile; Ross, Kate A.; Gaulin, Bruce D.
Physical Review Letters, Vol. 109, Issue 16
DOI: 10.1103/PhysRevLett.109.167201

Quantum Order by Disorder and Accidental Soft Mode in ${Er}_{2} {Ti}_{2} O_{7}$
journal, August 2012

Zhitomirsky, M. E.; Gvozdikova, M. V.; Holdsworth, P. C. W.
Physical Review Letters, Vol. 109, Issue 7
DOI: 10.1103/PhysRevLett.109.077204

Ground state phase diagram of generic $X Y$ pyrochlore magnets with quantum fluctuations
journal, October 2013

Wong, Anson W. C.; Hao, Zhihao; Gingras, Michel J. P.
Physical Review B, Vol. 88, Issue 14
DOI: 10.1103/PhysRevB.88.144402

Order by virtual crystal field fluctuations in pyrochlore XY antiferromagnets
journal, May 2016

Rau, Jeffrey G.; Petit, Sylvain; Gingras, Michel J. P.
Physical Review B, Vol. 93, Issue 18
DOI: 10.1103/PhysRevB.93.184408

Phase transitions, partial disorder and multi- k structures in Gd ₂ Ti ₂ O ₇
journal, July 2004

Stewart, J. R.; Ehlers, G.; Wills, A. S.
Journal of Physics: Condensed Matter, Vol. 16, Issue 28
DOI: 10.1088/0953-8984/16/28/L01

Cooperative Paramagnetism in the Geometrically Frustrated Pyrochlore Antiferromagnet ${Tb}_{2} {Ti}_{2} O_{7}$
journal, February 1999

Gardner, J. S.; Dunsiger, S. R.; Gaulin, B. D.
Physical Review Letters, Vol. 82, Issue 5
DOI: 10.1103/PhysRevLett.82.1012

Lightly stuffed pyrochlore structure of single-crystalline Yb $_{2}$ Ti $_{2}$ O $_{7}$ grown by the optical floating zone technique
journal, November 2012

Ross, K. A.; Proffen, Th.; Dabkowska, H. A.
Physical Review B, Vol. 86, Issue 17
DOI: 10.1103/PhysRevB.86.174424

Long-range order and spin-liquid states of polycrystalline Tb $_{2 + x}$ Ti $_{2 - x}$ O $_{7 + y}$
journal, February 2013

Taniguchi, T.; Kadowaki, H.; Takatsu, H.
Physical Review B, Vol. 87, Issue 6
DOI: 10.1103/PhysRevB.87.060408

Thermodynamic properties of Yb $_{2}$ Ti $_{2}$ O $_{7}$ pyrochlore as a function of temperature and magnetic field: Validation of a quantum spin ice exchange Hamiltonian
journal, May 2013

Hayre, N. R.; Ross, K. A.; Applegate, R.
Physical Review B, Vol. 87, Issue 18
DOI: 10.1103/PhysRevB.87.184423

Rods of Neutron Scattering Intensity in ${Yb}_{2} {Ti}_{2} O_{7}$ : Compelling Evidence for Significant Anisotropic Exchange in a Magnetic Pyrochlore Oxide
journal, May 2011

Thompson, Jordan D.; McClarty, Paul A.; Rønnow, Henrik M.
Physical Review Letters, Vol. 106, Issue 18
DOI: 10.1103/PhysRevLett.106.187202

Vindication of ${Yb}_{2} {Ti}_{2} O_{7}$ as a Model Exchange Quantum Spin Ice
journal, August 2012

Applegate, R.; Hayre, N. R.; Singh, R. R. P.
Physical Review Letters, Vol. 109, Issue 9
DOI: 10.1103/PhysRevLett.109.097205

Phase transition and thermal order-by-disorder in the pyrochlore antiferromagnet Er $_{2}$ Ti $_{2}$ O $_{7}$ : A high-temperature series expansion study
journal, December 2013

Oitmaa, J.; Singh, R. R. P.; Javanparast, B.
Physical Review B, Vol. 88, Issue 22
DOI: 10.1103/PhysRevB.88.220404

Spin dynamics in the presence of competing ferromagnetic and antiferromagnetic correlations in ${Yb}_{2} {Ti}_{2} O_{7}$
journal, August 2015

Robert, J.; Lhotel, E.; Remenyi, G.
Physical Review B, Vol. 92, Issue 6
DOI: 10.1103/PhysRevB.92.064425

Experimental realization of a quantum breathing pyrochlore antiferromagnet
journal, August 2014

Kimura, K.; Nakatsuji, S.; Kimura, T.
Physical Review B, Vol. 90, Issue 6
DOI: 10.1103/PhysRevB.90.060414

Breathing Pyrochlore Lattice Realized in $A$ -Site Ordered Spinel Oxides ${LiGaCr}_{4} O_{8}$ and ${LiInCr}_{4} O_{8}$
journal, February 2013

Okamoto, Yoshihiko; Nilsen, Gøran J.; Attfield, J. Paul
Physical Review Letters, Vol. 110, Issue 9
DOI: 10.1103/PhysRevLett.110.097203

Novel Phase Transitions in the Breathing Pyrochlore Lattice: ${}^{7}{Li − NMR}$ on ${LiInCr}_{4} O_{8}$ and ${LiGaCr}_{4} O_{8}$
journal, November 2014

Tanaka, Yu; Yoshida, Makoto; Takigawa, Masashi
Physical Review Letters, Vol. 113, Issue 22
DOI: 10.1103/PhysRevLett.113.227204

Ground State Selection and Spin-Liquid Behaviour in the Classical Heisenberg Model on the Breathing Pyrochlore Lattice
journal, October 2015

Benton, Owen; Shannon, Nic
Journal of the Physical Society of Japan, Vol. 84, Issue 10
DOI: 10.7566/JPSJ.84.104710

Antiferromagnetic Quantum Spins on the Pyrochlore Lattice
journal, March 2001

Tsunetsugu, Hirokazu
Journal of the Physical Society of Japan, Vol. 70, Issue 3
DOI: 10.1143/JPSJ.70.640

Spin-singlet order in a pyrochlore antiferromagnet
journal, December 2001

Tsunetsugu, Hirokazu
Physical Review B, Vol. 65, Issue 2
DOI: 10.1103/PhysRevB.65.024415

Recent advances in magnetic structure determination by neutron powder diffraction
journal, October 1993

Rodríguez-Carvajal, Juan
Physica B: Condensed Matter, Vol. 192, Issue 1-2
DOI: 10.1016/0921-4526(93)90108-I

Magnitude of quantum effects in classical spin ices
journal, October 2015

Rau, Jeffrey G.; Gingras, Michel J. P.
Physical Review B, Vol. 92, Issue 14
DOI: 10.1103/PhysRevB.92.144417

Quantum Spin Ices and Topological Phases from Dipolar-Octupolar Doublets on the Pyrochlore Lattice
journal, April 2014

Huang, Yi-Ping; Chen, Gang; Hermele, Michael
Physical Review Letters, Vol. 112, Issue 16
DOI: 10.1103/PhysRevLett.112.167203

Low-energy excitations and ground-state selection in the quantum breathing pyrochlore antiferromagnet ${Ba}_{3} {Yb}_{2} {Zn}_{5} O_{11}$
journal, June 2016

Haku, T.; Kimura, K.; Matsumoto, Y.
Physical Review B, Vol. 93, Issue 22
DOI: 10.1103/PhysRevB.93.220407

Frustrated Spin Systems
book, July 2020

Diep, H. T.
World Scientific
DOI: 10.1142/11660

Ising Like Order by Disorder In The Pyrochlore Antiferromagnet with Dzyaloshinskii-Moriya Interactions
text, January 2008

Canals, Benjamin; Elhajal, Maged; Lacroix, Claudine
arXiv
DOI: 10.48550/arxiv.0807.0352

Quantum Melting of Spin Ice: Emergent Cooperative Quadrupole and Chirality
text, January 2009

Onoda, Shigeki; Tanaka, Yoichi
arXiv
DOI: 10.48550/arxiv.0907.2536

Thermodynamic properties of the Yb2Ti2O7 pyrochlore as a function of temperature and magnetic field: validation of a quantum spin ice exchange Hamiltonian
text, January 2012

Hayre, N. R.; Ross, K. A.; Applegate, R.
arXiv
DOI: 10.48550/arxiv.1211.5934

Quantum spin ices and topological phases from dipolar-octupolar doublets on the pyrochlore lattice
text, January 2013

Huang, Yi-Ping; Chen, Gang; Hermele, Michael
arXiv
DOI: 10.48550/arxiv.1311.1231

Magnetic Phase Diagram of the Breathing Pyrochlore Antiferromagnet LiGa1-xInxCr4O8
text, January 2015

Okamoto, Yoshihiko; Nilsen, Gøran J.; Nakazono, Taishi
arXiv
DOI: 10.48550/arxiv.1503.08902

Ground-state selection and spin-liquid behaviour in the classical Heisenberg model on the breathing pyrochlore lattice
text, January 2015

Benton, Owen; Shannon, Nic
arXiv
DOI: 10.48550/arxiv.1506.01822

Paramagnetism in the kagome compounds (Zn,Mg,Cd)Cu$_{3}$(OH)$_{6}$Cl$_{2}$
text, January 2015

Iqbal, Yasir; Jeschke, Harald O.; Reuther, Johannes
arXiv
DOI: 10.48550/arxiv.1506.03436

Order by virtual crystal field fluctuations in pyrochlore XY antiferromagnets
text, January 2015

Rau, Jeffrey G.; Petit, Sylvain; Gingras, Michel J. P.
arXiv
DOI: 10.48550/arxiv.1510.04292

Weak antiferromagnetism and dimer order in quantum systems of coupled tetrahedra
text, January 2004

Kotov, Valeri N.; Zhitomirsky, Michael E.; Elhajal, Maged
arXiv
DOI: 10.48550/arxiv.cond-mat/0404674

The frustration-based approach of supercooled liquids and the glass transition: a review and critical assessment
text, January 2005

Tarjus, G.; Kivelson, S. A.; Nussinov, Z.
arXiv
DOI: 10.48550/arxiv.cond-mat/0509127

Works referencing / citing this record:

Electric field control of emergent electrodynamics in quantum spin ice
journal, September 2017

Lantagne-Hurtubise, Étienne; Bhattacharjee, Subhro; Moessner, R.
Physical Review B, Vol. 96, Issue 12
DOI: 10.1103/physrevb.96.125145

Spin–orbit coupled molecular quantum magnetism realized in inorganic solid
journal, September 2016

Park, Sang-Youn; Do, S. -H.; Choi, K. -Y.
Nature Communications, Vol. 7, Issue 1
DOI: 10.1038/ncomms12912

Formation of breathing pyrochlore lattices: structural, thermodynamic and crystal chemical aspects
journal, January 2020

Talanov, Mikhail V.; Talanov, Valeriy M.
CrystEngComm, Vol. 22, Issue 7
DOI: 10.1039/c9ce01635j

Electric field response in breathing pyrochlores
journal, August 2019

Mandal, Ipsita
The European Physical Journal B, Vol. 92, Issue 8
DOI: 10.1140/epjb/e2019-100215-4

Flat bands and Dirac cones in breathing lattices
journal, June 2017

Essafi, Karim; Jaubert, L. D. C.; Udagawa, M.
Journal of Physics: Condensed Matter, Vol. 29, Issue 31
DOI: 10.1088/1361-648x/aa782f

Weyl magnons in pyrochlore antiferromagnets with an all-in-all-out order
journal, March 2018

Jian, Shao-Kai; Nie, Wenxing
Physical Review B, Vol. 97, Issue 11
DOI: 10.1103/physrevb.97.115162

Spin ordering induced by lattice distortions in classical Heisenberg antiferromagnets on the breathing pyrochlore lattice
journal, April 2019

Aoyama, Kazushi; Kawamura, Hikaru
Physical Review B, Vol. 99, Issue 14
DOI: 10.1103/physrevb.99.144406

Weyl magnons in breathing pyrochlore antiferromagnets
journal, September 2016

Li, Fei-Ye; Li, Yao-Dong; Kim, Yong Baek
Nature Communications, Vol. 7, Issue 1
DOI: 10.1038/ncomms12691

Magnonic analog of the Edelstein effect in antiferromagnetic insulators
journal, January 2020

Li, Bo; Mook, Alexander; Raeliarijaona, Aldo
Physical Review B, Vol. 101, Issue 2
DOI: 10.1103/physrevb.101.024427

Quantum spin ice on the breathing pyrochlore lattice
text, January 2015

Savary, Lucile; Wang, Xiaoqun; Kee, Hae-Young
arXiv
DOI: 10.48550/arxiv.1511.06972

Flat bands and Dirac cones in breathing lattices
text, January 2016

Essafi, Karim; Jaubert, L. D. C.; Udagawa, M.
arXiv
DOI: 10.48550/arxiv.1610.01748

Behavior of the breathing pyrochlore lattice Ba$_3$Yb$_2$Zn$_5$O$_{11}$ in applied magnetic field
text, January 2018

Rau, J. G.; Wu, L. S.; May, A. F.
arXiv
DOI: 10.48550/arxiv.1809.05131

Electric Field Response In Breathing Pyrochlores
text, January 2019

Mandal, Ipsita
arXiv
DOI: 10.48550/arxiv.1904.07251

Magnonic Analogue of Edelstein Effect in Antiferromagnetic Insulators
text, January 2019

Li, Bo; Mook, Alexander; Raeliarijaona, Aldo
arXiv
DOI: 10.48550/arxiv.1910.00143

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Title: Anisotropic Exchange within Decoupled Tetrahedra in the Quantum Breathing Pyrochlore Ba 3 Yb 2 Zn 5 O 11

Abstract

Citation Formats

Weak antiferromagnetism and dimer order in quantum systems of coupled tetrahedra journal, December 2004

Zur Kristallchemie von Ba3In2Zn5O11. Ein tOxoindat/zinkatsol;zinkat mit Zn10O20- und In4O16-Makropolyedern und erstmals O2? in tetraedrischer Koordination durch Zn2+ journal, March 1993

Magnetic Phase Diagram of the Breathing Pyrochlore Antiferromagnet LiGa 1− x In x Cr 4 O 8 journal, April 2015

Crystal Field Excitations in the Breathing Pyrochlore Antiferromagnet Ba 3 Yb 2 Zn 5 O 11 journal, March 2016

Frustrated Spin Systems book, November 2012

Patterns of symmetry breaking in systems of coupled tetrahedra journal, March 2004

Magnetic order in a S= frustrated antiferromagnet on a square lattice journal, May 2004

Powgen: A third-generation highresolution high-throughput powder diffraction instrument at the Spallation Neutron Source book, December 2011

Composite Spin and Quadrupole Wave in the Ordered Phase of Tb 2+x Ti 2-x O 7+y journal, June 2015

Spin liquids in frustrated magnets journal, March 2010

Ising-like order by disorder in the pyrochlore antiferromagnet with Dzyaloshinskii-Moriya interactions journal, December 2008

Synthese und Kristallstruktur von Ba6Lu4Zn10O22 mit [OBa6]-Oktaedern journal, January 1996

Quantum spin configurations in Tb 2 Ti 2 O 7 journal, June 2007

Dzyaloshinsky-Moriya-induced order in the spin-liquid phase of the S = 1 ∕ 2 pyrochlore antiferromagnet journal, July 2005

Design and operation of the wide angular-range chopper spectrometer ARCS at the Spallation Neutron Source journal, January 2012

Higgs transition from a magnetic Coulomb liquid to a ferromagnet in Yb2Ti2O7 journal, January 2012

Quantum spin ice: a search for gapless quantum spin liquids in pyrochlore magnets journal, May 2014

Quantum fluctuations in spin-ice-like Pr2Zr2O7 journal, June 2013

Recent progress on HYSPEC, and its polarization analysis capabilities journal, January 2015

Unusual ordered phases of highly frustrated magnets: a review journal, April 2015

Frustrated Spin Systems book, January 2005

The frustration-based approach of supercooled liquids and the glass transition: a review and critical assessment journal, December 2005

Multipolar interactions in f -electron systems: The paradigm of actinide dioxides journal, June 2009

Paramagnetism in the kagome compounds ( Zn , Mg , Cd ) Cu 3 ( OH ) 6 Cl 2 journal, December 2015

Kapellasite: A Kagome Quantum Spin Liquid with Competing Interactions journal, July 2012

Quadrupolar Phases of the S = 1 Bilinear-Biquadratic Heisenberg Model on the Triangular Lattice journal, August 2006

Dynamically Induced Frustration as a Route to a Quantum Spin Ice State in Tb 2 Ti 2 O 7 via Virtual Crystal Field Excitations and Quantum Many-Body Effects journal, April 2007

Quantum Melting of Spin Ice: Emergent Cooperative Quadrupole and Chirality journal, July 2010

Quantum Excitations in Quantum Spin Ice journal, October 2011

Order by Quantum Disorder in Er 2 Ti 2 O 7 journal, October 2012

Quantum Order by Disorder and Accidental Soft Mode in Er 2 Ti 2 O 7 journal, August 2012

Ground state phase diagram of generic X Y pyrochlore magnets with quantum fluctuations journal, October 2013

Order by virtual crystal field fluctuations in pyrochlore XY antiferromagnets journal, May 2016

Phase transitions, partial disorder and multi- k structures in Gd 2 Ti 2 O 7 journal, July 2004

Cooperative Paramagnetism in the Geometrically Frustrated Pyrochlore Antiferromagnet Tb 2 Ti 2 O 7 journal, February 1999

Lightly stuffed pyrochlore structure of single-crystalline Yb 2 Ti 2 O 7 grown by the optical floating zone technique journal, November 2012

Long-range order and spin-liquid states of polycrystalline Tb 2 + x Ti 2 − x O 7 + y journal, February 2013

Thermodynamic properties of Yb 2 Ti 2 O 7 pyrochlore as a function of temperature and magnetic field: Validation of a quantum spin ice exchange Hamiltonian journal, May 2013

Rods of Neutron Scattering Intensity in Yb 2 Ti 2 O 7 : Compelling Evidence for Significant Anisotropic Exchange in a Magnetic Pyrochlore Oxide journal, May 2011

Vindication of Yb 2 Ti 2 O 7 as a Model Exchange Quantum Spin Ice journal, August 2012

Phase transition and thermal order-by-disorder in the pyrochlore antiferromagnet Er 2 Ti 2 O 7 : A high-temperature series expansion study journal, December 2013

Spin dynamics in the presence of competing ferromagnetic and antiferromagnetic correlations in Yb 2 Ti 2 O 7 journal, August 2015

Experimental realization of a quantum breathing pyrochlore antiferromagnet journal, August 2014

Breathing Pyrochlore Lattice Realized in A -Site Ordered Spinel Oxides LiGaCr 4 O 8 and LiInCr 4 O 8 journal, February 2013

Novel Phase Transitions in the Breathing Pyrochlore Lattice: Li − NMR 7 on LiInCr 4 O 8 and LiGaCr 4 O 8 journal, November 2014

Ground State Selection and Spin-Liquid Behaviour in the Classical Heisenberg Model on the Breathing Pyrochlore Lattice journal, October 2015

Antiferromagnetic Quantum Spins on the Pyrochlore Lattice journal, March 2001

Spin-singlet order in a pyrochlore antiferromagnet journal, December 2001

Recent advances in magnetic structure determination by neutron powder diffraction journal, October 1993

Magnitude of quantum effects in classical spin ices journal, October 2015

Quantum Spin Ices and Topological Phases from Dipolar-Octupolar Doublets on the Pyrochlore Lattice journal, April 2014

Low-energy excitations and ground-state selection in the quantum breathing pyrochlore antiferromagnet Ba 3 Yb 2 Zn 5 O 11 journal, June 2016

Frustrated Spin Systems book, July 2020

Ising Like Order by Disorder In The Pyrochlore Antiferromagnet with Dzyaloshinskii-Moriya Interactions text, January 2008

Quantum Melting of Spin Ice: Emergent Cooperative Quadrupole and Chirality text, January 2009

Thermodynamic properties of the Yb2Ti2O7 pyrochlore as a function of temperature and magnetic field: validation of a quantum spin ice exchange Hamiltonian text, January 2012

Quantum spin ices and topological phases from dipolar-octupolar doublets on the pyrochlore lattice text, January 2013

Magnetic Phase Diagram of the Breathing Pyrochlore Antiferromagnet LiGa1-xInxCr4O8 text, January 2015

Ground-state selection and spin-liquid behaviour in the classical Heisenberg model on the breathing pyrochlore lattice text, January 2015

Paramagnetism in the kagome compounds (Zn,Mg,Cd)Cu$_{3}$(OH)$_{6}$Cl$_{2}$ text, January 2015

Order by virtual crystal field fluctuations in pyrochlore XY antiferromagnets text, January 2015

Weak antiferromagnetism and dimer order in quantum systems of coupled tetrahedra text, January 2004

The frustration-based approach of supercooled liquids and the glass transition: a review and critical assessment text, January 2005

Electric field control of emergent electrodynamics in quantum spin ice journal, September 2017

Spin–orbit coupled molecular quantum magnetism realized in inorganic solid journal, September 2016

Formation of breathing pyrochlore lattices: structural, thermodynamic and crystal chemical aspects journal, January 2020

Electric field response in breathing pyrochlores journal, August 2019

Flat bands and Dirac cones in breathing lattices journal, June 2017

Weyl magnons in pyrochlore antiferromagnets with an all-in-all-out order journal, March 2018

Spin ordering induced by lattice distortions in classical Heisenberg antiferromagnets on the breathing pyrochlore lattice journal, April 2019

Weyl magnons in breathing pyrochlore antiferromagnets journal, September 2016

Magnonic analog of the Edelstein effect in antiferromagnetic insulators journal, January 2020

Quantum spin ice on the breathing pyrochlore lattice text, January 2015

Flat bands and Dirac cones in breathing lattices text, January 2016

Behavior of the breathing pyrochlore lattice Ba$_3$Yb$_2$Zn$_5$O$_{11}$ in applied magnetic field text, January 2018

Electric Field Response In Breathing Pyrochlores text, January 2019

Magnonic Analogue of Edelstein Effect in Antiferromagnetic Insulators text, January 2019

Title: Anisotropic Exchange within Decoupled Tetrahedra in the Quantum Breathing Pyrochlore ${Ba}_{3} {Yb}_{2} {Zn}_{5} O_{11}$

Weak antiferromagnetism and dimer order in quantum systems of coupled tetrahedra
journal, December 2004

Zur Kristallchemie von Ba3In2Zn5O11. Ein tOxoindat/zinkatsol;zinkat mit Zn10O20- und In4O16-Makropolyedern und erstmals O2? in tetraedrischer Koordination durch Zn2+
journal, March 1993

Magnetic Phase Diagram of the Breathing Pyrochlore Antiferromagnet LiGa ₁₋ _x In _x Cr ₄ O ₈
journal, April 2015

Crystal Field Excitations in the Breathing Pyrochlore Antiferromagnet Ba ₃ Yb ₂ Zn ₅ O ₁₁
journal, March 2016

Frustrated Spin Systems
book, November 2012

Patterns of symmetry breaking in systems of coupled tetrahedra
journal, March 2004

Magnetic order in a S= frustrated antiferromagnet on a square lattice
journal, May 2004

Powgen: A third-generation highresolution high-throughput powder diffraction instrument at the Spallation Neutron Source
book, December 2011

Composite Spin and Quadrupole Wave in the Ordered Phase of Tb _2+x Ti _2-x O _7+y
journal, June 2015

Spin liquids in frustrated magnets
journal, March 2010

Ising-like order by disorder in the pyrochlore antiferromagnet with Dzyaloshinskii-Moriya interactions
journal, December 2008

Synthese und Kristallstruktur von Ba6Lu4Zn10O22 mit [OBa6]-Oktaedern
journal, January 1996

Quantum spin configurations in ${Tb}_{2} {Ti}_{2} O_{7}$
journal, June 2007

Dzyaloshinsky-Moriya-induced order in the spin-liquid phase of the $S = 1 ∕ 2$ pyrochlore antiferromagnet
journal, July 2005

Design and operation of the wide angular-range chopper spectrometer ARCS at the Spallation Neutron Source
journal, January 2012

Higgs transition from a magnetic Coulomb liquid to a ferromagnet in Yb2Ti2O7
journal, January 2012

Quantum spin ice: a search for gapless quantum spin liquids in pyrochlore magnets
journal, May 2014

Quantum fluctuations in spin-ice-like Pr2Zr2O7
journal, June 2013

Recent progress on HYSPEC, and its polarization analysis capabilities
journal, January 2015

Unusual ordered phases of highly frustrated magnets: a review
journal, April 2015

Frustrated Spin Systems
book, January 2005

The frustration-based approach of supercooled liquids and the glass transition: a review and critical assessment
journal, December 2005

Multipolar interactions in $f$ -electron systems: The paradigm of actinide dioxides
journal, June 2009

Paramagnetism in the kagome compounds $(Zn, Mg, Cd) {Cu}_{3} {(OH)}_{6} {Cl}_{2}$
journal, December 2015

Kapellasite: A Kagome Quantum Spin Liquid with Competing Interactions
journal, July 2012

Quadrupolar Phases of the $S = 1$ Bilinear-Biquadratic Heisenberg Model on the Triangular Lattice
journal, August 2006

Dynamically Induced Frustration as a Route to a Quantum Spin Ice State in ${Tb}_{2} {Ti}_{2} O_{7}$ via Virtual Crystal Field Excitations and Quantum Many-Body Effects
journal, April 2007

Quantum Melting of Spin Ice: Emergent Cooperative Quadrupole and Chirality
journal, July 2010

Quantum Excitations in Quantum Spin Ice
journal, October 2011

Order by Quantum Disorder in ${Er}_{2} {Ti}_{2} O_{7}$
journal, October 2012

Quantum Order by Disorder and Accidental Soft Mode in ${Er}_{2} {Ti}_{2} O_{7}$
journal, August 2012

Ground state phase diagram of generic $X Y$ pyrochlore magnets with quantum fluctuations
journal, October 2013

Order by virtual crystal field fluctuations in pyrochlore XY antiferromagnets
journal, May 2016

Phase transitions, partial disorder and multi- k structures in Gd ₂ Ti ₂ O ₇
journal, July 2004

Cooperative Paramagnetism in the Geometrically Frustrated Pyrochlore Antiferromagnet ${Tb}_{2} {Ti}_{2} O_{7}$
journal, February 1999

Lightly stuffed pyrochlore structure of single-crystalline Yb $_{2}$ Ti $_{2}$ O $_{7}$ grown by the optical floating zone technique
journal, November 2012

Long-range order and spin-liquid states of polycrystalline Tb $_{2 + x}$ Ti $_{2 - x}$ O $_{7 + y}$
journal, February 2013

Thermodynamic properties of Yb $_{2}$ Ti $_{2}$ O $_{7}$ pyrochlore as a function of temperature and magnetic field: Validation of a quantum spin ice exchange Hamiltonian
journal, May 2013

Rods of Neutron Scattering Intensity in ${Yb}_{2} {Ti}_{2} O_{7}$ : Compelling Evidence for Significant Anisotropic Exchange in a Magnetic Pyrochlore Oxide
journal, May 2011

Vindication of ${Yb}_{2} {Ti}_{2} O_{7}$ as a Model Exchange Quantum Spin Ice
journal, August 2012

Phase transition and thermal order-by-disorder in the pyrochlore antiferromagnet Er $_{2}$ Ti $_{2}$ O $_{7}$ : A high-temperature series expansion study
journal, December 2013

Spin dynamics in the presence of competing ferromagnetic and antiferromagnetic correlations in ${Yb}_{2} {Ti}_{2} O_{7}$
journal, August 2015

Experimental realization of a quantum breathing pyrochlore antiferromagnet
journal, August 2014

Breathing Pyrochlore Lattice Realized in $A$ -Site Ordered Spinel Oxides ${LiGaCr}_{4} O_{8}$ and ${LiInCr}_{4} O_{8}$
journal, February 2013

Novel Phase Transitions in the Breathing Pyrochlore Lattice: ${}^{7}{Li − NMR}$ on ${LiInCr}_{4} O_{8}$ and ${LiGaCr}_{4} O_{8}$
journal, November 2014

Ground State Selection and Spin-Liquid Behaviour in the Classical Heisenberg Model on the Breathing Pyrochlore Lattice
journal, October 2015

Antiferromagnetic Quantum Spins on the Pyrochlore Lattice
journal, March 2001

Spin-singlet order in a pyrochlore antiferromagnet
journal, December 2001

Recent advances in magnetic structure determination by neutron powder diffraction
journal, October 1993

Magnitude of quantum effects in classical spin ices
journal, October 2015

Quantum Spin Ices and Topological Phases from Dipolar-Octupolar Doublets on the Pyrochlore Lattice
journal, April 2014

Low-energy excitations and ground-state selection in the quantum breathing pyrochlore antiferromagnet ${Ba}_{3} {Yb}_{2} {Zn}_{5} O_{11}$
journal, June 2016

Frustrated Spin Systems
book, July 2020

Ising Like Order by Disorder In The Pyrochlore Antiferromagnet with Dzyaloshinskii-Moriya Interactions
text, January 2008

Quantum Melting of Spin Ice: Emergent Cooperative Quadrupole and Chirality
text, January 2009

Thermodynamic properties of the Yb2Ti2O7 pyrochlore as a function of temperature and magnetic field: validation of a quantum spin ice exchange Hamiltonian
text, January 2012

Quantum spin ices and topological phases from dipolar-octupolar doublets on the pyrochlore lattice
text, January 2013

Magnetic Phase Diagram of the Breathing Pyrochlore Antiferromagnet LiGa1-xInxCr4O8
text, January 2015

Ground-state selection and spin-liquid behaviour in the classical Heisenberg model on the breathing pyrochlore lattice
text, January 2015

Paramagnetism in the kagome compounds (Zn,Mg,Cd)Cu$_{3}$(OH)$_{6}$Cl$_{2}$
text, January 2015

Order by virtual crystal field fluctuations in pyrochlore XY antiferromagnets
text, January 2015

Weak antiferromagnetism and dimer order in quantum systems of coupled tetrahedra
text, January 2004

The frustration-based approach of supercooled liquids and the glass transition: a review and critical assessment
text, January 2005

Electric field control of emergent electrodynamics in quantum spin ice
journal, September 2017

Spin–orbit coupled molecular quantum magnetism realized in inorganic solid
journal, September 2016

Formation of breathing pyrochlore lattices: structural, thermodynamic and crystal chemical aspects
journal, January 2020

Electric field response in breathing pyrochlores
journal, August 2019

Flat bands and Dirac cones in breathing lattices
journal, June 2017

Weyl magnons in pyrochlore antiferromagnets with an all-in-all-out order
journal, March 2018

Spin ordering induced by lattice distortions in classical Heisenberg antiferromagnets on the breathing pyrochlore lattice
journal, April 2019

Weyl magnons in breathing pyrochlore antiferromagnets
journal, September 2016

Magnonic analog of the Edelstein effect in antiferromagnetic insulators
journal, January 2020

Quantum spin ice on the breathing pyrochlore lattice
text, January 2015

Flat bands and Dirac cones in breathing lattices
text, January 2016

Behavior of the breathing pyrochlore lattice Ba$_3$Yb$_2$Zn$_5$O$_{11}$ in applied magnetic field
text, January 2018

Electric Field Response In Breathing Pyrochlores
text, January 2019

Magnonic Analogue of Edelstein Effect in Antiferromagnetic Insulators
text, January 2019