Robust antiferromagnetism preventing superconductivity in pressurized (Ba0.61K0.39)Mn2Bi2
Abstract
BaMn2Bi2 possesses an iso-structure of iron pnictide superconductors and similar antiferromagnetic (AFM) ground state to that of cuprates, therefore, it receives much more attention on its properties and is expected to be the parent compound of a new family of superconductors. When doped with potassium (K), BaMn2Bi2 undergoes a transition from an AFM insulator to an AFM metal. Consequently, it is of great interest to suppress the AFM order in the K-doped BaMn2Bi2 with the aim of exploring the potential superconductivity. In this paper, we report that external pressure up to 35.6 GPa cannot suppress the AFM order in the K-doped BaMn2Bi2 to develop superconductivity in the temperature range of 300 K–1.5 K, but induces a tetragonal (T) to an orthorhombic (OR) phase transition at ~20 GPa. Theoretical calculations for the T and OR phases, on basis of our high-pressure XRD data, indicate that the AFM order is robust in the pressurized Ba0.61K0.39Mn2Bi2. We conclude that both of our experimental and theoretical results suggest that the robust AFM order essentially prevents the emergence of superconductivity.
- Authors:
-
- Chinese Academy of Sciences (CAS), Beijing (China)
- Chinese Academy of Sciences (CAS), Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1259688
- Alternate Identifier(s):
- OSTI ID: 1286829
- Grant/Contract Number:
- XDB07020300; 2011CBA00100; 11427805; 91321207; AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Scientific Reports
- Additional Journal Information:
- Journal Volume: 4; Journal ID: ISSN 2045-2322
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; condensed-matter physics; physics; superconducting properties and materials
Citation Formats
Gu, Dachun, Dai, Xia, Le, Congcong, Sun, Liling, Wu, Qi, Saparov, Bayrammurad, Guo, Jing, Gao, Peiwen, Zhang, Shan, Zhou, Yazhou, Zhang, Chao, Jin, Shifeng, Xiong, Lun, Li, Rui, Li, Yanchun, Li, Xiaodong, Liu, Jing, Sefat, Athena S., Hu, Jiangping, and Zhao, Zhongxian. Robust antiferromagnetism preventing superconductivity in pressurized (Ba0.61K0.39)Mn2Bi2. United States: N. p., 2014.
Web. doi:10.1038/srep07342.
Gu, Dachun, Dai, Xia, Le, Congcong, Sun, Liling, Wu, Qi, Saparov, Bayrammurad, Guo, Jing, Gao, Peiwen, Zhang, Shan, Zhou, Yazhou, Zhang, Chao, Jin, Shifeng, Xiong, Lun, Li, Rui, Li, Yanchun, Li, Xiaodong, Liu, Jing, Sefat, Athena S., Hu, Jiangping, & Zhao, Zhongxian. Robust antiferromagnetism preventing superconductivity in pressurized (Ba0.61K0.39)Mn2Bi2. United States. https://doi.org/10.1038/srep07342
Gu, Dachun, Dai, Xia, Le, Congcong, Sun, Liling, Wu, Qi, Saparov, Bayrammurad, Guo, Jing, Gao, Peiwen, Zhang, Shan, Zhou, Yazhou, Zhang, Chao, Jin, Shifeng, Xiong, Lun, Li, Rui, Li, Yanchun, Li, Xiaodong, Liu, Jing, Sefat, Athena S., Hu, Jiangping, and Zhao, Zhongxian. Fri .
"Robust antiferromagnetism preventing superconductivity in pressurized (Ba0.61K0.39)Mn2Bi2". United States. https://doi.org/10.1038/srep07342. https://www.osti.gov/servlets/purl/1259688.
@article{osti_1259688,
title = {Robust antiferromagnetism preventing superconductivity in pressurized (Ba0.61K0.39)Mn2Bi2},
author = {Gu, Dachun and Dai, Xia and Le, Congcong and Sun, Liling and Wu, Qi and Saparov, Bayrammurad and Guo, Jing and Gao, Peiwen and Zhang, Shan and Zhou, Yazhou and Zhang, Chao and Jin, Shifeng and Xiong, Lun and Li, Rui and Li, Yanchun and Li, Xiaodong and Liu, Jing and Sefat, Athena S. and Hu, Jiangping and Zhao, Zhongxian},
abstractNote = {BaMn2Bi2 possesses an iso-structure of iron pnictide superconductors and similar antiferromagnetic (AFM) ground state to that of cuprates, therefore, it receives much more attention on its properties and is expected to be the parent compound of a new family of superconductors. When doped with potassium (K), BaMn2Bi2 undergoes a transition from an AFM insulator to an AFM metal. Consequently, it is of great interest to suppress the AFM order in the K-doped BaMn2Bi2 with the aim of exploring the potential superconductivity. In this paper, we report that external pressure up to 35.6 GPa cannot suppress the AFM order in the K-doped BaMn2Bi2 to develop superconductivity in the temperature range of 300 K–1.5 K, but induces a tetragonal (T) to an orthorhombic (OR) phase transition at ~20 GPa. Theoretical calculations for the T and OR phases, on basis of our high-pressure XRD data, indicate that the AFM order is robust in the pressurized Ba0.61K0.39Mn2Bi2. We conclude that both of our experimental and theoretical results suggest that the robust AFM order essentially prevents the emergence of superconductivity.},
doi = {10.1038/srep07342},
journal = {Scientific Reports},
number = ,
volume = 4,
place = {United States},
year = {Fri Dec 05 00:00:00 EST 2014},
month = {Fri Dec 05 00:00:00 EST 2014}
}
Web of Science
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