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Title: Commensurate antiferromagnetic excitations as a signature of the pseudogap in the tetragonal high-Tc cuprate HgBa2CuO4+δ

Abstract

We report that antiferromagnetic correlations have been argued to be the cause of the d-wave superconductivity and the pseudogap phenomena exhibited by the cuprates. Although the antiferromagnetic response in the pseudogap state has been reported for a number of compounds, there exists no information for structurally simple HgBa2CuO4+δ. We report neutron-scattering results for HgBa2CuO4+δ (superconducting transition temperature Tc≈71 K, pseudogap temperature T*≈305 K) that demonstrate the absence of the two most prominent features of the magnetic excitation spectrum of the cuprates: the X-shaped ‘hourglass’ response and the resonance mode in the superconducting state. Instead, the response is Y-shaped, gapped and significantly enhanced below T*, and hence a prominent signature of the pseudogap state.

Authors:
 [1];  [2];  [3];  [2];  [2];  [2];  [2];  [4];  [5];  [6];  [3];  [7];  [5]; ORCiD logo [3];  [2]
  1. Univ. of Minnesota, Minneapolis, MN (United States); Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  2. Univ. of Minnesota, Minneapolis, MN (United States)
  3. CEA-CNRS, Gif sur Yvette (France)
  4. Univ. of Minnesota, Minneapolis, MN (United States); Jilin Univ., Changchun (China)
  5. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  6. Neutron source Heinz Maier-Leibnitz (FRM II), Garching (Germany)
  7. Inst. Laue-Langevin (ILL), Grenoble (France)
Publication Date:
Research Org.:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Spallation Neutron Source (SNS)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1259490
Alternate Identifier(s):
OSTI ID: 1287028
Grant/Contract Number:  
SC0006858; LANLF100; FG02-08ER46544; ANR-14-CE05-0007; ANR-14-OHRI-0010; AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Nature Communications
Additional Journal Information:
Journal Volume: 7; Journal ID: ISSN 2041-1723
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Chan, M. K., Dorow, C. J., Mangin-Thro, L., Tang, Y., Ge, Y., Veit, M. J., Yu, G., Zhao, X., Christianson, A. D., Park, J. T., Sidis, Y., Steffens, P., Abernathy, D. L., Bourges, P., and Greven, M. Commensurate antiferromagnetic excitations as a signature of the pseudogap in the tetragonal high-Tc cuprate HgBa2CuO4+δ. United States: N. p., 2016. Web. doi:10.1038/ncomms10819.
Chan, M. K., Dorow, C. J., Mangin-Thro, L., Tang, Y., Ge, Y., Veit, M. J., Yu, G., Zhao, X., Christianson, A. D., Park, J. T., Sidis, Y., Steffens, P., Abernathy, D. L., Bourges, P., & Greven, M. Commensurate antiferromagnetic excitations as a signature of the pseudogap in the tetragonal high-Tc cuprate HgBa2CuO4+δ. United States. https://doi.org/10.1038/ncomms10819
Chan, M. K., Dorow, C. J., Mangin-Thro, L., Tang, Y., Ge, Y., Veit, M. J., Yu, G., Zhao, X., Christianson, A. D., Park, J. T., Sidis, Y., Steffens, P., Abernathy, D. L., Bourges, P., and Greven, M. Fri . "Commensurate antiferromagnetic excitations as a signature of the pseudogap in the tetragonal high-Tc cuprate HgBa2CuO4+δ". United States. https://doi.org/10.1038/ncomms10819. https://www.osti.gov/servlets/purl/1259490.
@article{osti_1259490,
title = {Commensurate antiferromagnetic excitations as a signature of the pseudogap in the tetragonal high-Tc cuprate HgBa2CuO4+δ},
author = {Chan, M. K. and Dorow, C. J. and Mangin-Thro, L. and Tang, Y. and Ge, Y. and Veit, M. J. and Yu, G. and Zhao, X. and Christianson, A. D. and Park, J. T. and Sidis, Y. and Steffens, P. and Abernathy, D. L. and Bourges, P. and Greven, M.},
abstractNote = {We report that antiferromagnetic correlations have been argued to be the cause of the d-wave superconductivity and the pseudogap phenomena exhibited by the cuprates. Although the antiferromagnetic response in the pseudogap state has been reported for a number of compounds, there exists no information for structurally simple HgBa2CuO4+δ. We report neutron-scattering results for HgBa2CuO4+δ (superconducting transition temperature Tc≈71 K, pseudogap temperature T*≈305 K) that demonstrate the absence of the two most prominent features of the magnetic excitation spectrum of the cuprates: the X-shaped ‘hourglass’ response and the resonance mode in the superconducting state. Instead, the response is Y-shaped, gapped and significantly enhanced below T*, and hence a prominent signature of the pseudogap state.},
doi = {10.1038/ncomms10819},
journal = {Nature Communications},
number = ,
volume = 7,
place = {United States},
year = {Fri Mar 04 00:00:00 EST 2016},
month = {Fri Mar 04 00:00:00 EST 2016}
}

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Works referenced in this record:

Progress in Neutron Scattering Studies of Spin Excitations in High- T c Cuprates
journal, January 2012

  • Fujita, Masaki; Hiraka, Haruhiro; Matsuda, Masaaki
  • Journal of the Physical Society of Japan, Vol. 81, Issue 1
  • DOI: 10.1143/JPSJ.81.011007

Inelastic neutron scattering study of spin excitations in the superconducting state of high temperature superconductors
journal, September 2007


Emergence of Coherent Magnetic Excitations in the High Temperature Underdoped La 2 x Sr x CuO 4 Superconductor at Low Temperatures
journal, April 2009


How to detect fluctuating stripes in the high-temperature superconductors
journal, October 2003


Magnetic collective mode dispersion in high-temperature superconductors
journal, February 2001


Spin dynamics in the pseudogap state of a high-temperature superconductor
journal, September 2007

  • Hinkov, V.; Bourges, P.; Pailhès, S.
  • Nature Physics, Vol. 3, Issue 11
  • DOI: 10.1038/nphys720

A common thread: The pairing interaction for unconventional superconductors
journal, October 2012


Pseudogap state near a quantum critical point
journal, June 2013

  • Efetov, K. B.; Meier, H.; Pépin, C.
  • Nature Physics, Vol. 9, Issue 7
  • DOI: 10.1038/nphys2641

Density wave instabilities in a correlated two-dimensional metal
journal, October 2014


Charge order in the pseudogap phase of cuprate superconductors
journal, January 2015


Charge order and its connection with Fermi-liquid charge transport in a pristine high-Tc cuprate
journal, December 2014

  • Tabis, W.; Li, Y.; Tacon, M. Le
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms6875

Unusual magnetic order in the pseudogap region of the superconductor HgBa2CuO4+δ
journal, September 2008


Magnetic order in the pseudogap phase of HgBa 2 CuO 4 + δ studied by spin-polarized neutron diffraction
journal, December 2011


Effect of chemical inhomogeneity in bismuth-based copper oxide superconductors
journal, February 2004


Universal sheet resistance and revised phase diagram of the cuprate high-temperature superconductors
journal, July 2013

  • Barisic, N.; Chan, M. K.; Li, Y.
  • Proceedings of the National Academy of Sciences, Vol. 110, Issue 30
  • DOI: 10.1073/pnas.1301989110

Spectroscopic evidence for Fermi liquid-like energy and temperature dependence of the relaxation rate in the pseudogap phase of the cuprates
journal, March 2013

  • Mirzaei, S. I.; Stricker, D.; Hancock, J. N.
  • Proceedings of the National Academy of Sciences, Vol. 110, Issue 15
  • DOI: 10.1073/pnas.1218846110

Universal quantum oscillations in the underdoped cuprate superconductors
journal, November 2013

  • Barišić, Neven; Badoux, Sven; Chan, Mun K.
  • Nature Physics, Vol. 9, Issue 12
  • DOI: 10.1038/nphys2792

Evidence for competing magnetic instabilities in underdoped YBa 2 Cu 3 O 6 + x
journal, March 2011


Resonant x-ray scattering study of charge-density wave correlations in YBa 2 Cu 3 O 6 + x
journal, August 2014


Long-Range Incommensurate Charge Fluctuations in (Y,Nd)Ba2Cu3O6+x
journal, July 2012


Direct observation of competition between superconductivity and charge density wave order in YBa2Cu3O6.67
journal, October 2012

  • Chang, J.; Blackburn, E.; Holmes, A. T.
  • Nature Physics, Vol. 8, Issue 12
  • DOI: 10.1038/nphys2456

Neutron scattering study of the magnetic phase diagram of underdoped YBa 2 Cu 3 O 6+ x
journal, October 2010


Insulator-to-Metal Crossover in the Normal State of La 2 x Sr x CuO 4 Near Optimum Doping
journal, December 1996


Metal-insulator quantum critical point beneath the high Tc superconducting dome
journal, March 2010

  • Sebastian, S. E.; Harrison, N.; Altarawneh, M. M.
  • Proceedings of the National Academy of Sciences, Vol. 107, Issue 14
  • DOI: 10.1073/pnas.0913711107

Magnetic resonance in the model high-temperature superconductor HgBa 2 CuO 4 + δ
journal, February 2010


A universal relationship between magnetic resonance and superconducting gap in unconventional superconductors
journal, October 2009

  • Yu, G.; Li, Y.; Motoyama, E. M.
  • Nature Physics, Vol. 5, Issue 12
  • DOI: 10.1038/nphys1426

Angle-resolved photoemission spectroscopy study of Hg Ba 2 Cu O 4 + δ
journal, May 2014


Two energy scales and two distinct quasiparticle dynamics in the superconducting state of underdoped cuprates
journal, July 2006

  • Le Tacon, M.; Sacuto, A.; Georges, A.
  • Nature Physics, Vol. 2, Issue 8
  • DOI: 10.1038/nphys362

The pseudogap: friend or foe of high T c ?
journal, December 2005


Theory of the pseudogap state of the cuprates
journal, April 2006


Three-component electronic structure of the cuprates derived from spectroscopic-imaging scanning tunneling microscopy
journal, May 2012


Spin-Stripe Density Varies Linearly With the Hole Content in Single-Layer Bi 2 + x Sr 2 x CuO 6 + y Cuprate Superconductors
journal, January 2013


Dispersion of the odd magnetic resonant mode in near-optimally doped Bi 2 Sr 2 CaCu 2 O 8 + δ
journal, December 2007


Crystal Growth and Characterization of the Model High-Temperature Superconductor HgBa2CuO4+δ
journal, December 2006


Demonstrating the model nature of the high-temperature superconductor HgBa 2 CuO 4 + δ
journal, August 2008


Thermoelectric power and resistivity of HgBa 2 CuO 4 + δ over a wide doping range
journal, December 2000


Pronounced In-Plane Anisotropy of Phonon Anomalies in YBa 2 Cu 3 O 6.6
journal, June 2002


Evaluation of CuO 2 plane hole doping in YBa 2 Cu 3 O 6 + x single crystals
journal, May 2006


Neutron scattering study of the magnetic phase diagram of underdoped YBa2Cu3O6+x
text, January 2010


Spin dynamics in the pseudogap state of a high-temperature superconductor
text, January 2008


Metal-insulator quantum critical point beneath the high Tc superconducting dome
text, January 2009


Progress in Neutron Scattering Studies of Spin Excitations in High-Tc Cuprates
text, January 2011


Long-range incommensurate charge fluctuations in (Y,Nd)Ba2Cu3O(6+x)
text, January 2012


Charge Order in the Pseudogap Phase of Cuprate Superconductors
text, January 2014


The Magnetic Excitation Spectrum and Thermodynamics of High-$T_c$ Superconductors
text, January 2000


The pseudogap: friend or foe of high Tc?
text, January 2005


Magnetic order in the pseudogap phase of high-$T_C$ superconductors
text, January 2005


Unusual magnetic order in the pseudogap region of the superconductor HgBa2CuO4+δ
journal, September 2008


Charge order and its connection with Fermi-liquid charge transport in a pristine high-Tc cuprate
journal, December 2014

  • Tabis, W.; Li, Y.; Tacon, M. Le
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms6875

A universal relationship between magnetic resonance and superconducting gap in unconventional superconductors
journal, October 2009

  • Yu, G.; Li, Y.; Motoyama, E. M.
  • Nature Physics, Vol. 5, Issue 12
  • DOI: 10.1038/nphys1426

Spectroscopic evidence for Fermi liquid-like energy and temperature dependence of the relaxation rate in the pseudogap phase of the cuprates
journal, March 2013

  • Mirzaei, S. I.; Stricker, D.; Hancock, J. N.
  • Proceedings of the National Academy of Sciences, Vol. 110, Issue 15
  • DOI: 10.1073/pnas.1218846110

Quantum phase transitions of metals in two spatial dimensions. II. Spin density wave order
journal, August 2010


In-Plane Magnetoresistance Obeys Kohler’s Rule in the Pseudogap Phase of Cuprate Superconductors
journal, October 2014


Magnetic Order in the Pseudogap Phase of High- T C Superconductors
journal, May 2006


Metal-insulator quantum critical point beneath the high Tc superconducting dome
text, January 2009


The Three Component Electronic Structure of the Cuprates Derived from SI-STM
text, January 2012


Works referencing / citing this record:

Anomalies in the pseudogap phase of the cuprates: competing ground states and the role of umklapp scattering
journal, October 2019

  • Robinson, Neil J.; Johnson, Peter D.; Rice, T. Maurice
  • Reports on Progress in Physics, Vol. 82, Issue 12
  • DOI: 10.1088/1361-6633/ab31ed

Magnetic susceptibility and simulated neutron signal in the two-dimensional Hubbard model
journal, August 2019


Bond particle theory for the pseudogap phase of underdoped cuprates
journal, August 2019


Effective SU(2) theory for the pseudogap state
journal, March 2017


Origin of kinks in the energy dispersion of strongly correlated matter
journal, April 2017


Controlling Feynman diagrammatic expansions: Physical nature of the pseudogap in the two-dimensional Hubbard model
journal, July 2017


Synchrotron x-ray scattering study of charge-density-wave order in HgBa 2 CuO 4 + δ
journal, October 2017


Low-energy antiferromagnetic spin fluctuations limit the coherent superconducting gap in cuprates
journal, December 2018


Doping-dependent charge order correlations in electron-doped cuprates
journal, August 2016

  • da Silva Neto, Eduardo H.; Yu, Biqiong; Minola, Matteo
  • Science Advances, Vol. 2, Issue 8
  • DOI: 10.1126/sciadv.1600782

Unusual behavior of cuprates explained by heterogeneous charge localization
journal, January 2019


Doping-dependent charge order correlations in electron-doped cuprates
text, January 2016


Synchrotron X-Ray Scattering Study of Charge-Density-Wave Order in $HgBa_{2}CuO_{4+δ}$
text, January 2017


Doping-dependent charge order correlations in electron-doped cuprates
journal, August 2016

  • da Silva Neto, Eduardo H.; Yu, Biqiong; Minola, Matteo
  • Science Advances, Vol. 2, Issue 8
  • DOI: 10.1126/sciadv.1600782