Dirac node arcs in PtSn4

Wu, Yun; Wang, Lin -Lin; Mun, Eundeok; Johnson, D. D.; Mou, Daixiang; Huang, Lunan; Lee, Yongbin; Bud’ko, S. L.; Canfield, P. C.; Kaminski, Adam

doi:10.1038/nphys3712

Title: Dirac node arcs in PtSn₄

Abstract

In topological quantum materials^1,2,3 the conduction and valence bands are connected at points or along lines in the momentum space. A number of studies have demonstrated that several materials are indeed Dirac/Weyl semimetals^4,5,6,7,8. However, there is still no experimental confirmation of materials with line nodes, in which the Dirac nodes form closed loops in the momentum space^2,3. Here we report the discovery of a novel topological structure—Dirac node arcs—in the ultrahigh magnetoresistive material PtSn₄ using laser-based angle-resolved photoemission spectroscopy data and density functional theory calculations. Unlike the closed loops of line nodes, the Dirac node arc structure arises owing to the surface states and resembles the Dirac dispersion in graphene that is extended along a short line in the momentum space. Here, we propose that this reported Dirac node arc structure is a novel topological state that provides an exciting platform for studying the exotic properties of Dirac fermions.

Authors:

Wu, Yun ^[1]; Wang, Lin -Lin ^[2];

^[1];

^[1]; Huang, Lunan ^[1]; Lee, Yongbin ^[2]; Bud’ko, S. L. ^[1]; Canfield, P. C. ^[1]; Kaminski, Adam ^[1]

Ames Lab., Ames, IA (United States); Iowa State Univ., Ames, IA (United States)
Ames Lab., Ames, IA (United States)

Publication Date:: Mon Apr 04 00:00:00 EDT 2016

Research Org.:: Ames Laboratory (AMES), Ames, IA (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1253756

Report Number(s):: IS-J-8943
Journal ID: ISSN 1745-2473; nphys3712

Grant/Contract Number:: AC02-07CH11358

Resource Type:: Accepted Manuscript

Journal Name:: Nature Physics

Additional Journal Information:: Journal Volume: 88; Journal Issue: 1-2; Journal ID: ISSN 1745-2473

Publisher:: Nature Publishing Group (NPG)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; electronic properties and materials; topological insulators

Citation Formats


                    Wu, Yun, Wang, Lin -Lin, Mun, Eundeok, Johnson, D. D., Mou, Daixiang, Huang, Lunan, Lee, Yongbin, Bud’ko, S. L., Canfield, P. C., and Kaminski, Adam. Dirac node arcs in PtSn4.  United States: N. p., 2016. 
Web.  doi:10.1038/nphys3712.

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                    Wu, Yun, Wang, Lin -Lin, Mun, Eundeok, Johnson, D. D., Mou, Daixiang, Huang, Lunan, Lee, Yongbin, Bud’ko, S. L., Canfield, P. C., & Kaminski, Adam. Dirac node arcs in PtSn4.  United States.  https://doi.org/10.1038/nphys3712

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                    Wu, Yun, Wang, Lin -Lin, Mun, Eundeok, Johnson, D. D., Mou, Daixiang, Huang, Lunan, Lee, Yongbin, Bud’ko, S. L., Canfield, P. C., and Kaminski, Adam. Mon .  
"Dirac node arcs in PtSn4".  United States.  https://doi.org/10.1038/nphys3712.  https://www.osti.gov/servlets/purl/1253756.

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@article{osti_1253756,

  title        = {Dirac node arcs in PtSn4},

  author       = {Wu, Yun and Wang, Lin -Lin and Mun, Eundeok and Johnson, D. D. and Mou, Daixiang and Huang, Lunan and Lee, Yongbin and Bud’ko, S. L. and Canfield, P. C. and Kaminski, Adam},

  abstractNote = {In topological quantum materials1,2,3 the conduction and valence bands are connected at points or along lines in the momentum space. A number of studies have demonstrated that several materials are indeed Dirac/Weyl semimetals4,5,6,7,8. However, there is still no experimental confirmation of materials with line nodes, in which the Dirac nodes form closed loops in the momentum space2,3. Here we report the discovery of a novel topological structure—Dirac node arcs—in the ultrahigh magnetoresistive material PtSn4 using laser-based angle-resolved photoemission spectroscopy data and density functional theory calculations. Unlike the closed loops of line nodes, the Dirac node arc structure arises owing to the surface states and resembles the Dirac dispersion in graphene that is extended along a short line in the momentum space. Here, we propose that this reported Dirac node arc structure is a novel topological state that provides an exciting platform for studying the exotic properties of Dirac fermions.},

  doi          = {10.1038/nphys3712},

  journal      = {Nature Physics},

  number       = 1-2,

  volume       = 88,

  place        = {United States},

  year         = {Mon Apr 04 00:00:00 EDT 2016},

  month        = {Mon Apr 04 00:00:00 EDT 2016}

}

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Frontiers of Physics, Vol. 14, Issue 3
DOI: 10.1007/s11467-019-0890-7

A magnetic topological semimetal Sr1−yMn1−zSb2 (y, z < 0.1)
journal, July 2017

Liu, J. Y.; Hu, J.; Zhang, Q.
Nature Materials, Vol. 16, Issue 9
DOI: 10.1038/nmat4953

Strong Intrinsic Spin Hall Effect in the TaAs Family of Weyl Semimetals
journal, September 2016

Sun, Yan; Zhang, Yang; Felser, Claudia
Physical Review Letters, Vol. 117, Issue 14
DOI: 10.1103/PhysRevLett.117.146403

Thermoelectric quantum oscillations in ZrSiS.
journalarticle, January 2017

Matusiak, Marcin; Kaczorowski, Dariusz
Springer Science and Business Media LLC
DOI: 10.17863/cam.43518

Spectroscopic evidence for type II Weyl semimetal state in MoTe2
text, January 2016

Huang, Lunan; McCormick, Timothy M.; Ochi, Masayuki
arXiv
DOI: 10.48550/arxiv.1603.06482

Compensated semimetal LaSb with unsaturated magnetoresistance
text, January 2016

Zeng, L. -K.; Lou, R.; Wu, D. -S.
arXiv
DOI: 10.48550/arxiv.1604.08142

Tunable point nodes from line node semimetals via application of light
text, January 2016

Narayan, Awadhesh
arXiv
DOI: 10.48550/arxiv.1607.02503

Thermoelectric quantum oscillations in ZrSiS
text, January 2017

Matusiak, Marcin; Cooper, J. R.; Kaczorowski, Dariusz
arXiv
DOI: 10.48550/arxiv.1701.02137

Antiferromagnetic Topological Nodal Line Semimetals
text, January 2017

Wang, Jing
arXiv
DOI: 10.48550/arxiv.1704.05608

Flat optical conductivity in ZrSiS due to two-dimensional Dirac bands
text, January 2017

Schilling, M. B.; Schoop, L. M.; Lotsch, B. V.
arXiv
DOI: 10.48550/arxiv.1707.09620

Surface and 3D quantum Hall effects from engineering of exceptional points in nodal-line semimetals
text, January 2017

Molina, Rafael A.; Gonzalez, Jose
arXiv
DOI: 10.48550/arxiv.1710.01960

Distinct multiple fermionic states in a single topological metal
text, January 2017

Hosen, M. Mofazzel; Dimitri, Klauss; Nandy, Ashis K.
arXiv
DOI: 10.48550/arxiv.1711.07390

Observation of Gapless Dirac Surface States in ZrGeTe
text, January 2017

Hosen, M. Mofazzel; Dimitri, Klauss; Aperis, Alex
arXiv
DOI: 10.48550/arxiv.1711.08011

Rules for Phase Shifts of Quantum Oscillations in Topological Nodal-line Semimetals
text, January 2018

Li, Cequn; Wang, C. M.; Wan, Bo
arXiv
DOI: 10.48550/arxiv.1801.05709

Extreme magnetoresistance in the topologically trivial lanthanum monopnictide LaAs
text, January 2018

Yang, H. -Y.; Nummy, T.; Li, H.
arXiv
DOI: 10.48550/arxiv.1803.10866

Fragility of Fermi arcs in Dirac semimetals
text, January 2019

Wu, Yun; Jo, Na Hyun; Wang, Lin-Lin
arXiv
DOI: 10.48550/arxiv.1904.03138

Nearly massless Dirac fermions hosted by Sb square net in BaMnSb2
journal, July 2016

Liu, Jinyu; Hu, Jin; Cao, Huibo
Scientific Reports, Vol. 6, Issue 1
DOI: 10.1038/srep30525

Three-Dimensional Anisotropic Magnetoresistance in the Dirac Node-Line Material ZrSiSe
preprint, January 2017

Pan, Haiyang; Tong, Bingbing; Yu, Jihai
arXiv
DOI: 10.48550/arxiv.1708.02779

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Title: Dirac node arcs in PtSn4

Abstract

Citation Formats

Colloquium: Topological insulators journal, November 2010

Topological nodal semimetals journal, December 2011

Dimensional crossover in topological matter: Evolution of the multiple Dirac point in the layered system to the flat band on the surface journal, March 2011

Discovery of a Three-Dimensional Topological Dirac Semimetal, Na3Bi journal, January 2014

Observation of a three-dimensional topological Dirac semimetal phase in high-mobility Cd3As2 journal, May 2014

Discovery of a Weyl fermion semimetal and topological Fermi arcs journal, July 2015

Discovery of a Weyl fermion state with Fermi arcs in niobium arsenide journal, August 2015

Experimental discovery of a topological Weyl semimetal state in TaP journal, November 2015

Dirac Semimetal in Three Dimensions journal, April 2012

Dirac semimetal and topological phase transitions in A 3 Bi ( A = Na , K, Rb) journal, May 2012

Three-dimensional Dirac semimetal and quantum transport in Cd 3 As 2 journal, September 2013

A stable three-dimensional topological Dirac semimetal Cd3As2 journal, May 2014

Elektron und Gravitation. I journal, May 1929

A Weyl Fermion semimetal with surface Fermi arcs in the transition metal monopnictide TaAs class journal, June 2015

Topological node-line semimetal in three-dimensional graphene networks journal, July 2015

Topological Node-Line Semimetal and Dirac Semimetal State in Antiperovskite Cu 3 PdN journal, July 2015

Dirac Line Nodes in Inversion-Symmetric Crystals journal, July 2015

Topological nodal line semimetals with and without spin-orbital coupling journal, August 2015

Drumhead surface states and topological nodal-line fermions in TlTaSe 2 journal, March 2016

A new form of Ca 3 P 2 with a ring of Dirac nodes journal, August 2015

Line-Node Dirac Semimetal and Topological Insulating Phase in Noncentrosymmetric Pnictides CaAg X ( X = P, As) journal, January 2016

Topological nodal-line fermions in spin-orbit metal PbTaSe2 journal, February 2016

Ultrahigh mobility and giant magnetoresistance in the Dirac semimetal Cd3As2 journal, November 2014

Extremely large magnetoresistance and ultrahigh mobility in the topological Weyl semimetal candidate NbP journal, June 2015

Large, non-saturating magnetoresistance in WTe2 journal, September 2014

Magnetic field effects on transport properties of PtSn 4 journal, January 2012

Temperature-Induced Lifshitz Transition in WTe 2 journal, October 2015

Growth of single crystals from metallic fluxes journal, June 1992

Use of frit-disc crucibles for routine and exploratory solution growth of single crystalline samples journal, December 2015

Tunable vacuum ultraviolet laser based spectrometer for angle resolved photoemission spectroscopy journal, March 2014

Inhomogeneous Electron Gas journal, November 1964

Self-Consistent Equations Including Exchange and Correlation Effects journal, November 1965

Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set journal, October 1996

Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set journal, July 1996

Generalized Gradient Approximation Made Simple journal, October 1996

Projector augmented-wave method journal, December 1994

Special points for Brillouin-zone integrations journal, June 1976

Structure refinements and some properties of the transition metal stannides Os3Sn7, Ir5Sn7, Ni0.402(4)Pd0.598Sn4, α-PdSn2 and PtSn4 journal, September 2000

Inhomogeneous Electron Gas journal, March 1973

High-resolution X-ray luminescence extension imaging journal, February 2021

Electronic structure of AlFeN films exhibiting crystallographic orientation change from c- to a-axis with Fe concentrations and annealing effect journal, February 2020

Elektron und gravitation. I journal, November 1986

Dimensional crossover in topological matter: Evolution of the multiple Dirac point in the layered system to the flat band on the surface text, January 2010

Discovery of a Three-dimensional Topological Dirac Semimetal, Na3Bi text, January 2013

Ultrahigh mobility and giant magnetoresistance in the Dirac semimetal Cd$_3$As$_2$ text, January 2014

Discovery of a Weyl Fermion Semimetal and Topological Fermi Arcs text, January 2015

Extremely large magnetoresistance and ultrahigh mobility in the topological Weyl semimetal NbP text, January 2015

Dirac Line Nodes in Inversion Symmetric Crystals text, January 2015

Experimental discovery of a topological Weyl semimetal state in TaP text, January 2015

Dirac Nodal Arc Semimetal PtSn 4 : An Ideal Platform for Understanding Surface Properties and Catalysis for Hydrogen Evolution journal, August 2019

Transport evidence of 3D topological nodal-line semimetal phase in ZrSiS journal, July 2017

Topological quantum catalyst: Dirac nodal line states and a potential electrocatalyst of hydrogen evolution in the TiSi family journal, December 2017

Thermoelectric quantum oscillations in ZrSiS journal, May 2017

Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2 journal, July 2016

Unconventional mass enhancement around the Dirac nodal loop in ZrSiS journal, November 2017

Experimental realization of two-dimensional Dirac nodal line fermions in monolayer Cu2Si journal, October 2017

Distinct multiple fermionic states in a single topological metal journal, August 2018

Observation of Dirac-like energy band and ring-torus Fermi surface associated with the nodal line in topological insulator CaAgAs journal, January 2018

Visualizing electronic structures of quantum materials by angle-resolved photoemission spectroscopy journal, August 2018

Nearly massless Dirac fermions hosted by Sb square net in BaMnSb2 journal, July 2016

Coexistence of open and closed type nodal line topological semimetals in two dimensional B 2 C journal, January 2018

Discovery of a novel spin-polarized nodal ring in a two-dimensional HK lattice journal, January 2018

Extremely large magnetoresistance in the nonmagnetic semimetal YBi journal, January 2018

Strong anisotropic nodal lines in the TiBe family journal, January 2019

Efficient hydrogen evolution reaction with platinum stannide PtSn 4 via surface oxidation journal, January 2020

Out-of-plane transport in ZrSiS and ZrSiSe microstructures journal, October 2019

First-principles study of structural, mechanical, lattice dynamical and thermal properties of nodal-line semimetals ZrXY (X=Si,Ge; Y=S,Se) journal, October 2016

Topological nature of the node-arc semimetal PtSn 4 probed by de Haas-van Alphen quantum oscillations journal, March 2018

Emergence of topological phases by stacking of two-dimensional lattices with nonsymmorphic symmetry journal, December 2018

New materials physics journal, November 2019

Surface termination dependent quasiparticle scattering interference and magneto-transport study on ZrSiS journal, October 2018

New type of hybrid nodal line semimetal in Be 2 Si journal, March 2019

Straight nodal lines and waterslide surface states observed in acoustic metacrystals journal, July 2019

Quantum oscillations and nontrivial topological state in a compensated semimetal TaP 2 journal, September 2019

Dual topological insulator and insulator-semimetal transition in mirror-symmetric honeycomb materials journal, November 2019

Impurity-induced resonant states in topological nodal-line semimetals journal, November 2019

Plateaus of quantized conductance with high steps in topological nodal-line semimetals journal, January 2020

Title: Dirac node arcs in PtSn₄

Colloquium: Topological insulators
journal, November 2010

Topological nodal semimetals
journal, December 2011

Dimensional crossover in topological matter: Evolution of the multiple Dirac point in the layered system to the flat band on the surface
journal, March 2011

Discovery of a Three-Dimensional Topological Dirac Semimetal, Na3Bi
journal, January 2014

Observation of a three-dimensional topological Dirac semimetal phase in high-mobility Cd3As2
journal, May 2014

Discovery of a Weyl fermion semimetal and topological Fermi arcs
journal, July 2015

Discovery of a Weyl fermion state with Fermi arcs in niobium arsenide
journal, August 2015

Experimental discovery of a topological Weyl semimetal state in TaP
journal, November 2015

Dirac Semimetal in Three Dimensions
journal, April 2012

Dirac semimetal and topological phase transitions in $A_{3}$ Bi ( $A = Na$ , K, Rb)
journal, May 2012

Three-dimensional Dirac semimetal and quantum transport in Cd $_{3}$ As $_{2}$
journal, September 2013

A stable three-dimensional topological Dirac semimetal Cd3As2
journal, May 2014

Elektron und Gravitation. I
journal, May 1929

A Weyl Fermion semimetal with surface Fermi arcs in the transition metal monopnictide TaAs class
journal, June 2015

Topological node-line semimetal in three-dimensional graphene networks
journal, July 2015

Topological Node-Line Semimetal and Dirac Semimetal State in Antiperovskite ${Cu}_{3} PdN$
journal, July 2015

Dirac Line Nodes in Inversion-Symmetric Crystals
journal, July 2015

Topological nodal line semimetals with and without spin-orbital coupling
journal, August 2015

Drumhead surface states and topological nodal-line fermions in ${TlTaSe}_{2}$
journal, March 2016

A new form of Ca ₃ P ₂ with a ring of Dirac nodes
journal, August 2015

Line-Node Dirac Semimetal and Topological Insulating Phase in Noncentrosymmetric Pnictides CaAg X ( X = P, As)
journal, January 2016

Topological nodal-line fermions in spin-orbit metal PbTaSe2
journal, February 2016

Ultrahigh mobility and giant magnetoresistance in the Dirac semimetal Cd3As2
journal, November 2014

Extremely large magnetoresistance and ultrahigh mobility in the topological Weyl semimetal candidate NbP
journal, June 2015

Large, non-saturating magnetoresistance in WTe2
journal, September 2014

Magnetic field effects on transport properties of PtSn $_{4}$
journal, January 2012

Temperature-Induced Lifshitz Transition in ${WTe}_{2}$
journal, October 2015

Growth of single crystals from metallic fluxes
journal, June 1992

Use of frit-disc crucibles for routine and exploratory solution growth of single crystalline samples
journal, December 2015

Tunable vacuum ultraviolet laser based spectrometer for angle resolved photoemission spectroscopy
journal, March 2014

Inhomogeneous Electron Gas
journal, November 1964

Self-Consistent Equations Including Exchange and Correlation Effects
journal, November 1965

Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
journal, October 1996

Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set
journal, July 1996

Generalized Gradient Approximation Made Simple
journal, October 1996

Projector augmented-wave method
journal, December 1994

Special points for Brillouin-zone integrations
journal, June 1976

Structure refinements and some properties of the transition metal stannides Os3Sn7, Ir5Sn7, Ni0.402(4)Pd0.598Sn4, α-PdSn2 and PtSn4
journal, September 2000

Inhomogeneous Electron Gas
journal, March 1973

High-resolution X-ray luminescence extension imaging
journal, February 2021

Electronic structure of AlFeN films exhibiting crystallographic orientation change from c- to a-axis with Fe concentrations and annealing effect
journal, February 2020

Elektron und gravitation. I
journal, November 1986

Dimensional crossover in topological matter: Evolution of the multiple Dirac point in the layered system to the flat band on the surface
text, January 2010

Discovery of a Three-dimensional Topological Dirac Semimetal, Na3Bi
text, January 2013

Ultrahigh mobility and giant magnetoresistance in the Dirac semimetal Cd$_3$As$_2$
text, January 2014

Discovery of a Weyl Fermion Semimetal and Topological Fermi Arcs
text, January 2015

Extremely large magnetoresistance and ultrahigh mobility in the topological Weyl semimetal NbP
text, January 2015

Dirac Line Nodes in Inversion Symmetric Crystals
text, January 2015

Experimental discovery of a topological Weyl semimetal state in TaP
text, January 2015

Dirac Nodal Arc Semimetal PtSn ₄ : An Ideal Platform for Understanding Surface Properties and Catalysis for Hydrogen Evolution
journal, August 2019

Transport evidence of 3D topological nodal-line semimetal phase in ZrSiS
journal, July 2017

Topological quantum catalyst: Dirac nodal line states and a potential electrocatalyst of hydrogen evolution in the TiSi family
journal, December 2017

Thermoelectric quantum oscillations in ZrSiS
journal, May 2017

Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2
journal, July 2016

Unconventional mass enhancement around the Dirac nodal loop in ZrSiS
journal, November 2017

Experimental realization of two-dimensional Dirac nodal line fermions in monolayer Cu2Si
journal, October 2017

Distinct multiple fermionic states in a single topological metal
journal, August 2018

Observation of Dirac-like energy band and ring-torus Fermi surface associated with the nodal line in topological insulator CaAgAs
journal, January 2018

Visualizing electronic structures of quantum materials by angle-resolved photoemission spectroscopy
journal, August 2018

Nearly massless Dirac fermions hosted by Sb square net in BaMnSb2
journal, July 2016

Coexistence of open and closed type nodal line topological semimetals in two dimensional B ₂ C
journal, January 2018

Discovery of a novel spin-polarized nodal ring in a two-dimensional HK lattice
journal, January 2018

Extremely large magnetoresistance in the nonmagnetic semimetal YBi
journal, January 2018

Strong anisotropic nodal lines in the TiBe family
journal, January 2019

Efficient hydrogen evolution reaction with platinum stannide PtSn ₄ via surface oxidation
journal, January 2020

Out-of-plane transport in ZrSiS and ZrSiSe microstructures
journal, October 2019

First-principles study of structural, mechanical, lattice dynamical and thermal properties of nodal-line semimetals ZrXY (X=Si,Ge; Y=S,Se)
journal, October 2016

Topological nature of the node-arc semimetal PtSn ₄ probed by de Haas-van Alphen quantum oscillations
journal, March 2018

Emergence of topological phases by stacking of two-dimensional lattices with nonsymmorphic symmetry
journal, December 2018

New materials physics
journal, November 2019

Surface termination dependent quasiparticle scattering interference and magneto-transport study on ZrSiS
journal, October 2018

New type of hybrid nodal line semimetal in Be ₂ Si
journal, March 2019

Straight nodal lines and waterslide surface states observed in acoustic metacrystals
journal, July 2019

Quantum oscillations and nontrivial topological state in a compensated semimetal ${TaP}_{2}$
journal, September 2019

Dual topological insulator and insulator-semimetal transition in mirror-symmetric honeycomb materials
journal, November 2019

Impurity-induced resonant states in topological nodal-line semimetals
journal, November 2019

Plateaus of quantized conductance with high steps in topological nodal-line semimetals
journal, January 2020

Tunable point nodes from line-node semimetals via application of light
journal, July 2016

Photovoltaic anomalous Hall effect in line-node semimetals
journal, October 2016