DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: ‘Hard’ crystalline lattice in the Weyl semimetal NbAs

Abstract

Here, we report the effect of hydrostatic pressure on the magnetotransport properties of the Weyl semimetal NbAs. Subtle changes can be seen in the ρxx(T) profiles with pressure up to 2.31 GPa. The Fermi surfaces undergo an anisotropic evolution under pressure: the extremal areas slightly increase in the kx-ky plane, but decrease in the kz-ky(kx) plane. The topological features of the two pockets observed at atmospheric pressure, however, remain unchanged at 2.31 GPa. No superconductivity can be seen down to 0.3 K for all the pressures measured. By fitting the temperature dependence of specific heat to the Debye model, we obtain a small Sommerfeld coefficient γ0=0.09(1) mJ (mol•K2)-1 and a large Debye temperature, θD=450(9) K, confirming a 'hard' crystalline lattice that is stable under pressure. We also studied the Kadowaki–Woods ratio of this low-carrier-density massless system, RKW=3.2 x 104 μΩ cm mol2 K2 J-2. After we account for the small carrier density in NbAs, this RKW indicates a suppressed transport scattering rate relative to other metals.

Authors:
 [1];  [2];  [1];  [1];  [1]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  2. Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
Publication Date:
Research Org.:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1249050
Report Number(s):
LA-UR-15-28700
Journal ID: ISSN 0953-8984
Grant/Contract Number:  
AC52-06NA25396
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Physics. Condensed Matter
Additional Journal Information:
Journal Volume: 28; Journal Issue: 5; Journal ID: ISSN 0953-8984
Publisher:
IOP Publishing
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 36 MATERIALS SCIENCE

Citation Formats

Luo, Yongkang, Ghimire, N. J., Bauer, E. D., Thompson, J. D., and Ronning, F. ‘Hard’ crystalline lattice in the Weyl semimetal NbAs. United States: N. p., 2016. Web. doi:10.1088/0953-8984/28/5/055502.
Luo, Yongkang, Ghimire, N. J., Bauer, E. D., Thompson, J. D., & Ronning, F. ‘Hard’ crystalline lattice in the Weyl semimetal NbAs. United States. https://doi.org/10.1088/0953-8984/28/5/055502
Luo, Yongkang, Ghimire, N. J., Bauer, E. D., Thompson, J. D., and Ronning, F. Thu . "‘Hard’ crystalline lattice in the Weyl semimetal NbAs". United States. https://doi.org/10.1088/0953-8984/28/5/055502. https://www.osti.gov/servlets/purl/1249050.
@article{osti_1249050,
title = {‘Hard’ crystalline lattice in the Weyl semimetal NbAs},
author = {Luo, Yongkang and Ghimire, N. J. and Bauer, E. D. and Thompson, J. D. and Ronning, F.},
abstractNote = {Here, we report the effect of hydrostatic pressure on the magnetotransport properties of the Weyl semimetal NbAs. Subtle changes can be seen in the ρxx(T) profiles with pressure up to 2.31 GPa. The Fermi surfaces undergo an anisotropic evolution under pressure: the extremal areas slightly increase in the kx-ky plane, but decrease in the kz-ky(kx) plane. The topological features of the two pockets observed at atmospheric pressure, however, remain unchanged at 2.31 GPa. No superconductivity can be seen down to 0.3 K for all the pressures measured. By fitting the temperature dependence of specific heat to the Debye model, we obtain a small Sommerfeld coefficient γ0=0.09(1) mJ (mol•K2)-1 and a large Debye temperature, θD=450(9) K, confirming a 'hard' crystalline lattice that is stable under pressure. We also studied the Kadowaki–Woods ratio of this low-carrier-density massless system, RKW=3.2 x 104 μΩ cm mol2 K2 J-2. After we account for the small carrier density in NbAs, this RKW indicates a suppressed transport scattering rate relative to other metals.},
doi = {10.1088/0953-8984/28/5/055502},
journal = {Journal of Physics. Condensed Matter},
number = 5,
volume = 28,
place = {United States},
year = {Thu Jan 14 00:00:00 EST 2016},
month = {Thu Jan 14 00:00:00 EST 2016}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 22 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Elektron und Gravitation. I
journal, May 1929


Weyl electrons kiss
journal, May 2011


Recent developments in transport phenomena in Weyl semimetals
journal, November 2013


Chiral anomaly, charge density waves, and axion strings from Weyl semimetals
journal, April 2013


Weyl Semimetal Phase in Noncentrosymmetric Transition-Metal Monophosphides
journal, March 2015


Discovery of a Weyl fermion semimetal and topological Fermi arcs
journal, July 2015


Experimental Discovery of Weyl Semimetal TaAs
journal, July 2015


Observation of Weyl nodes in TaAs
journal, August 2015

  • Lv, B. Q.; Xu, N.; Weng, H. M.
  • Nature Physics, Vol. 11, Issue 9
  • DOI: 10.1038/nphys3426

Discovery of a Weyl fermion state with Fermi arcs in niobium arsenide
journal, August 2015

  • Xu, Su-Yang; Alidoust, Nasser; Belopolski, Ilya
  • Nature Physics, Vol. 11, Issue 9
  • DOI: 10.1038/nphys3437

Friedel oscillations due to Fermi arcs in Weyl semimetals
journal, November 2012


Helical Fermi arcs and surface states in time-reversal invariant Weyl semimetals
journal, June 2013


Quantum oscillations from surface Fermi arcs in Weyl and Dirac semimetals
journal, October 2014

  • Potter, Andrew C.; Kimchi, Itamar; Vishwanath, Ashvin
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms6161

Observation of the Chiral-Anomaly-Induced Negative Magnetoresistance in 3D Weyl Semimetal TaAs
journal, August 2015


Extremely large magnetoresistance and ultrahigh mobility in the topological Weyl semimetal candidate NbP
journal, June 2015

  • Shekhar, Chandra; Nayak, Ajaya K.; Sun, Yan
  • Nature Physics, Vol. 11, Issue 8
  • DOI: 10.1038/nphys3372

Chiral anomaly and classical negative magnetoresistance of Weyl metals
journal, September 2013


The Kondo lattice and weak antiferromagnetism
journal, July 1977


Three-dimensional Dirac semimetal and quantum transport in Cd 3 As 2
journal, September 2013


Observation of superconductivity induced by a point contact on 3D Dirac semimetal Cd3As2 crystals
journal, November 2015

  • Wang, He; Wang, Huichao; Liu, Haiwen
  • Nature Materials, Vol. 15, Issue 1
  • DOI: 10.1038/nmat4456

Magnetic Oscillations in Metals
book, October 2011


Detection of Berry's Phase in a Bulk Rashba Semiconductor
journal, December 2013


Pressure-Induced Electronic Transition in Black Phosphorus
journal, October 2015


Anisotropic Fermi Surface and Quantum Limit Transport in High Mobility Three-Dimensional Dirac Semimetal Cd 3 As 2
journal, September 2015


Quantal Phase Factors Accompanying Adiabatic Changes
journal, March 1984

  • Berry, M. V.
  • Proceedings of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 392, Issue 1802
  • DOI: 10.1098/rspa.1984.0023

Berry’s phase for energy bands in solids
journal, June 1989


Hall effect in the extremely large magnetoresistance semimetal WTe 2
journal, November 2015

  • Luo, Yongkang; Li, H.; Dai, Y. M.
  • Applied Physics Letters, Vol. 107, Issue 18
  • DOI: 10.1063/1.4935240

Universal relationship of the resistivity and specific heat in heavy-Fermion compounds
journal, May 1986


A unified explanation of the Kadowaki–Woods ratio in strongly correlated metals
journal, April 2009

  • Jacko, A. C.; Fjærestad, J. O.; Powell, B. J.
  • Nature Physics, Vol. 5, Issue 6
  • DOI: 10.1038/nphys1249

Scalable T2 resistivity in a small single-component Fermi surface
journal, August 2015


Elektron und gravitation. I
journal, November 1986


Electron-Electron Scattering in Transition Metals.
journal, September 1968


Recent developments in transport phenomena in Weyl semimetals
text, January 2013


Weyl semimetal phase in non-centrosymmetric transition metal monophosphides
text, January 2015


Discovery of a Weyl Fermion Semimetal and Topological Fermi Arcs
text, January 2015


Experimental discovery of Weyl semimetal TaAs
text, January 2015


Observation of Weyl nodes in TaAs
text, January 2015


Scalable T^2 resistivity in a small single-component Fermi surface
text, January 2015


Hall effect in the extremely large magnetoresistance semimetal WTe$_2$
text, January 2015


Works referencing / citing this record:

Crystal growth of Dirac semimetal ZrSiS with high magnetoresistance and mobility
journal, January 2017

  • Sankar, Raman; Peramaiyan, G.; Muthuselvam, I. Panneer
  • Scientific Reports, Vol. 7, Issue 1
  • DOI: 10.1038/srep40603

Directly photoexcited Dirac and Weyl fermions in ZrSiS and NbAs
journal, November 2018

  • Weber, Chris P.; Schoop, Leslie M.; Parkin, Stuart S. P.
  • Applied Physics Letters, Vol. 113, Issue 22
  • DOI: 10.1063/1.5055207

Orbital effect and weak localization in the longitudinal magnetoresistance of Weyl semimetals NbP, NbAs, TaP, and TaAs
journal, March 2020


Inducing superconductivity in Weyl semimetal microstructures by selective ion sputtering
journal, May 2017

  • Bachmann, Maja D.; Nair, Nityan; Flicker, Felix
  • Science Advances, Vol. 3, Issue 5
  • DOI: 10.1126/sciadv.1602983

Coexistence of Weyl Physics and Planar Defects in Semimetals TaP and TaAs
text, January 2016


Inducing superconductivity in Weyl semi-metal microstructures by selective ion sputtering
text, January 2017


Crystal growth of Dirac semimetal ZrSiS with high magnetoresistance and mobility
journal, January 2017

  • Sankar, Raman; Peramaiyan, G.; Muthuselvam, I. Panneer
  • Scientific Reports, Vol. 7, Issue 1
  • DOI: 10.1038/srep40603