Giant switchable photovoltaic effect in organometal trihalide perovskite devices
Abstract
Organolead trihalide perovskite (OTP) materials are emerging as naturally abundant materials for low-cost, solution-processed and highly efficient solar cells. Here, we show that, in OTP-based photovoltaic devices with vertical and lateral cell configurations, the photocurrent direction can be switched repeatedly by applying a small electric field of <1 V μm–1. The switchable photocurrent, generally observed in devices based on ferroelectric materials, reached 20.1 mA cm–2 under one sun illumination in OTP devices with a vertical architecture, which is four orders of magnitude larger than that measured in other ferroelectric photovoltaic devices. This field-switchable photovoltaic effect can be explained by the formation of reversible p–i–n structures induced by ion drift in the perovskite layer. Furthermore, the demonstration of switchable OTP photovoltaics and electric-field-manipulated doping paves the way for innovative solar cell designs and for the exploitation of OTP materials in electrically and optically readable memristors and circuits.
- Authors:
-
- Univ. of Nebraska, Lincoln, NE (United States)
- Publication Date:
- Research Org.:
- Univ. of Nebraska, Lincoln, NE (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1238052
- Grant/Contract Number:
- EE0006709
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Materials
- Additional Journal Information:
- Journal Volume: 14; Journal Issue: 2; Journal ID: ISSN 1476-1122
- Publisher:
- Springer Nature - Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; 36 MATERIALS SCIENCE; solar cells
Citation Formats
Xiao, Zhengguo, Yuan, Yongbo, Shao, Yuchuan, Wang, Qi, Dong, Qingfeng, Bi, Cheng, Sharma, Pankaj, Gruverman, Alexei, and Huang, Jinsong. Giant switchable photovoltaic effect in organometal trihalide perovskite devices. United States: N. p., 2014.
Web. doi:10.1038/nmat4150.
Xiao, Zhengguo, Yuan, Yongbo, Shao, Yuchuan, Wang, Qi, Dong, Qingfeng, Bi, Cheng, Sharma, Pankaj, Gruverman, Alexei, & Huang, Jinsong. Giant switchable photovoltaic effect in organometal trihalide perovskite devices. United States. https://doi.org/10.1038/nmat4150
Xiao, Zhengguo, Yuan, Yongbo, Shao, Yuchuan, Wang, Qi, Dong, Qingfeng, Bi, Cheng, Sharma, Pankaj, Gruverman, Alexei, and Huang, Jinsong. Mon .
"Giant switchable photovoltaic effect in organometal trihalide perovskite devices". United States. https://doi.org/10.1038/nmat4150. https://www.osti.gov/servlets/purl/1238052.
@article{osti_1238052,
title = {Giant switchable photovoltaic effect in organometal trihalide perovskite devices},
author = {Xiao, Zhengguo and Yuan, Yongbo and Shao, Yuchuan and Wang, Qi and Dong, Qingfeng and Bi, Cheng and Sharma, Pankaj and Gruverman, Alexei and Huang, Jinsong},
abstractNote = {Organolead trihalide perovskite (OTP) materials are emerging as naturally abundant materials for low-cost, solution-processed and highly efficient solar cells. Here, we show that, in OTP-based photovoltaic devices with vertical and lateral cell configurations, the photocurrent direction can be switched repeatedly by applying a small electric field of <1 V μm–1. The switchable photocurrent, generally observed in devices based on ferroelectric materials, reached 20.1 mA cm–2 under one sun illumination in OTP devices with a vertical architecture, which is four orders of magnitude larger than that measured in other ferroelectric photovoltaic devices. This field-switchable photovoltaic effect can be explained by the formation of reversible p–i–n structures induced by ion drift in the perovskite layer. Furthermore, the demonstration of switchable OTP photovoltaics and electric-field-manipulated doping paves the way for innovative solar cell designs and for the exploitation of OTP materials in electrically and optically readable memristors and circuits.},
doi = {10.1038/nmat4150},
journal = {Nature Materials},
number = 2,
volume = 14,
place = {United States},
year = {Mon Dec 08 00:00:00 EST 2014},
month = {Mon Dec 08 00:00:00 EST 2014}
}
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