Interfacial development of electrophoretically deposited graphene oxide films on Al alloys

Jin, Sumin; Dickerson, James H.; Pham, Viet Hung; Brochu, Mathieu

doi:10.1149/2.0121511jes

Title: Interfacial development of electrophoretically deposited graphene oxide films on Al alloys

Abstract

Adhesion between film and substrate is critical for electronic device and coating applications. Interfacial development between electrophoretically deposited graphene oxide films on Al 1100 and Al 5052 alloys were investigated using FT-IR and XPS depth profiling techniques. Obtained results suggest metal ion permeation from the substrates into deposited graphene oxide films. The interface between the films and the substrates were primarily composed of Al-O-C bonds from oxygenated defects on graphene oxide plane rather than expected Al-C formation. Films heat treated at 150 °C had change in microstructure and peak shifts in XPS spectra suggesting change in chemical structure of bonds between the films and the substrates.

Authors:

Jin, Sumin ^[1]; Dickerson, James H. ^[2]; Pham, Viet Hung ^[3]; Brochu, Mathieu ^[1]

McGill Univ., Montreal, QC (Canada)
Brookhaven National Lab. (BNL), Upton, NY (United States); Brown Univ., Providence, RI (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States)

Publication Date:: Tue Jul 28 00:00:00 EDT 2015

Research Org.:: Brookhaven National Lab. (BNL), Upton, NY (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1235849

Report Number(s):: BNL-108606-2015-JA
Journal ID: ISSN 0013-4651; KC0403020

Grant/Contract Number:: SC00112704

Resource Type:: Accepted Manuscript

Journal Name:: Journal of the Electrochemical Society

Additional Journal Information:: Journal Volume: 162; Journal Issue: 11; Journal ID: ISSN 0013-4651

Publisher:: The Electrochemical Society

Country of Publication:: United States

Language:: English

Subject:: 77 NANOSCIENCE AND NANOTECHNOLOGY; electrophoretic deposition; graphene oxide; aluminum alloys; Center for Functional Nanomaterials; Al 1100; Al 5052; X ray photoelectron spectroscopy (XPS); interfaces

Citation Formats


                    Jin, Sumin, Dickerson, James H., Pham, Viet Hung, and Brochu, Mathieu. Interfacial development of electrophoretically deposited graphene oxide films on Al alloys.  United States: N. p., 2015. 
Web.  doi:10.1149/2.0121511jes.

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                    Jin, Sumin, Dickerson, James H., Pham, Viet Hung, & Brochu, Mathieu. Interfacial development of electrophoretically deposited graphene oxide films on Al alloys.  United States.  https://doi.org/10.1149/2.0121511jes

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                    Jin, Sumin, Dickerson, James H., Pham, Viet Hung, and Brochu, Mathieu. Tue .  
"Interfacial development of electrophoretically deposited graphene oxide films on Al alloys".  United States.  https://doi.org/10.1149/2.0121511jes.  https://www.osti.gov/servlets/purl/1235849.

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@article{osti_1235849,

  title        = {Interfacial development of electrophoretically deposited graphene oxide films on Al alloys},

  author       = {Jin, Sumin and Dickerson, James H. and Pham, Viet Hung and Brochu, Mathieu},

  abstractNote = {Adhesion between film and substrate is critical for electronic device and coating applications. Interfacial development between electrophoretically deposited graphene oxide films on Al 1100 and Al 5052 alloys were investigated using FT-IR and XPS depth profiling techniques. Obtained results suggest metal ion permeation from the substrates into deposited graphene oxide films. The interface between the films and the substrates were primarily composed of Al-O-C bonds from oxygenated defects on graphene oxide plane rather than expected Al-C formation. Films heat treated at 150 °C had change in microstructure and peak shifts in XPS spectra suggesting change in chemical structure of bonds between the films and the substrates.},

  doi          = {10.1149/2.0121511jes},

  journal      = {Journal of the Electrochemical Society},

  number       = 11,

  volume       = 162,

  place        = {United States},

  year         = {Tue Jul 28 00:00:00 EDT 2015},

  month        = {Tue Jul 28 00:00:00 EDT 2015}

}

Copy to clipboard

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Works referencing / citing this record:

Graphene Oxide Coatings Deposited on Steel Substrate Using Electrophoretic Deposition and Electrochemical Evaluation of Coatings in Saline Media
journal, September 2018

Rehman, Zaeem Ur; Raza, Mohsin Ali; Ghauri, Faizan Ali
Key Engineering Materials, Vol. 778
DOI: 10.4028/www.scientific.net/kem.778.111

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Similar Records

Title: Interfacial development of electrophoretically deposited graphene oxide films on Al alloys

Abstract

Citation Formats

Applications of Graphene Electrophoretic Deposition. A Review journal, November 2012

Electrophoretic deposition of high quality transparent conductive graphene films on insulating glass substrates journal, March 2012

Transferable Graphene Oxide Films with Tunable Microstructures journal, November 2010

Thin Film Fabrication and Simultaneous Anodic Reduction of Deposited Graphene Oxide Platelets by Electrophoretic Deposition journal, March 2010

Electrophoretic deposition of graphene nanosheets on nickel foams for electrochemical capacitors journal, May 2010

Quantitative evaluation of electrophoretic deposition kinetics of graphene oxide journal, February 2014

Formation of a deposit by electrophoresis journal, January 1940

Metal Permeation into Multi-layered Graphene Oxide journal, January 2014

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Microstructural and hardness behavior of graphene-nanoplatelets/aluminum composites synthesized by mechanical alloying journal, December 2014

Reinforcement with graphene nanosheets in aluminum matrix composites journal, April 2012

Investigating aluminum alloy reinforced by graphene nanoflakes journal, August 2014

Reduced graphene oxide coated thin aluminum film as an optoacoustic transmitter for high pressure and high frequency ultrasound generation journal, December 2012

Electroplating formation of Al–C covalent bonds on multiwalled carbon nanotubes journal, February 2011

Fast and simple fabrication of a large transparent chemically-converted graphene film by spray-coating journal, June 2010

Fabrication of hexagonally ordered nanopores in anodic alumina: An alternative pretreatment journal, February 2011

Structure of Graphite Oxide Revisited ‖ journal, June 1998

The adsorption and decomposition of carboxylic acids on Al (111) journal, January 1986

Chemical analysis of graphene oxide films after heat and chemical treatments by X-ray photoelectron and Micro-Raman spectroscopy journal, January 2009

Oxygen plasma modification of pitch-based isotropic carbon fibres journal, January 2003

Reduction of graphene oxide by electron beam generated plasmas produced in methane/argon mixtures journal, October 2010

Low temperature plasma-mediated synthesis of graphene nanosheets for supercapacitor electrodes journal, January 2012

Passive layers developed on different tempers of AA7075 aluminium alloy after molybdenum implantation: XPS study of molybdenum implantation on AA7075 aluminium alloy journal, February 2012

Chemical bonding and reaction at metal/polymer interfaces journal, May 1985

Interaction of aliphatic acids and alcohols with aluminum surfaces journal, July 1992

Graphene Oxide Coatings Deposited on Steel Substrate Using Electrophoretic Deposition and Electrochemical Evaluation of Coatings in Saline Media journal, September 2018

Applications of Graphene Electrophoretic Deposition. A Review
journal, November 2012

Electrophoretic deposition of high quality transparent conductive graphene films on insulating glass substrates
journal, March 2012

Transferable Graphene Oxide Films with Tunable Microstructures
journal, November 2010

Thin Film Fabrication and Simultaneous Anodic Reduction of Deposited Graphene Oxide Platelets by Electrophoretic Deposition
journal, March 2010

Electrophoretic deposition of graphene nanosheets on nickel foams for electrochemical capacitors
journal, May 2010

Quantitative evaluation of electrophoretic deposition kinetics of graphene oxide
journal, February 2014

Formation of a deposit by electrophoresis
journal, January 1940

Metal Permeation into Multi-layered Graphene Oxide
journal, January 2014

Graphene–aluminum nanocomposites
journal, October 2011

Microstructural and hardness behavior of graphene-nanoplatelets/aluminum composites synthesized by mechanical alloying
journal, December 2014

Reinforcement with graphene nanosheets in aluminum matrix composites
journal, April 2012

Investigating aluminum alloy reinforced by graphene nanoflakes
journal, August 2014

Reduced graphene oxide coated thin aluminum film as an optoacoustic transmitter for high pressure and high frequency ultrasound generation
journal, December 2012

Electroplating formation of Al–C covalent bonds on multiwalled carbon nanotubes
journal, February 2011

Fast and simple fabrication of a large transparent chemically-converted graphene film by spray-coating
journal, June 2010

Fabrication of hexagonally ordered nanopores in anodic alumina: An alternative pretreatment
journal, February 2011

Structure of Graphite Oxide Revisited ^‖
journal, June 1998

The adsorption and decomposition of carboxylic acids on Al (111)
journal, January 1986

Chemical analysis of graphene oxide films after heat and chemical treatments by X-ray photoelectron and Micro-Raman spectroscopy
journal, January 2009

Oxygen plasma modification of pitch-based isotropic carbon fibres
journal, January 2003

Reduction of graphene oxide by electron beam generated plasmas produced in methane/argon mixtures
journal, October 2010

Low temperature plasma-mediated synthesis of graphene nanosheets for supercapacitor electrodes
journal, January 2012

Passive layers developed on different tempers of AA7075 aluminium alloy after molybdenum implantation: XPS study of molybdenum implantation on AA7075 aluminium alloy
journal, February 2012

Chemical bonding and reaction at metal/polymer interfaces
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journal, July 1992

Graphene Oxide Coatings Deposited on Steel Substrate Using Electrophoretic Deposition and Electrochemical Evaluation of Coatings in Saline Media
journal, September 2018