Low-surface-area hard carbon anode for Na-ion batteries via graphene oxide as a dehydration agent
Abstract
Na-ion batteries are emerging as one of the most promising energy storage technologies, particularly for grid-level applications. Among anode candidate materials, hard carbon is very attractive due to its high capacity and low cost. However, hard carbon anodes often suffer a low first-cycle Coulombic efficiency and fast capacity fading. In this study, we discover that doping graphene oxide into sucrose, the precursor for hard carbon, can effectively reduce the specific surface area of hard carbon to as low as 5.4 m²/g. We further reveal that such doping can effectively prevent foaming during caramelization of sucrose and extend the pyrolysis burn-off of sucrose caramel over a wider temperature range. Thus, the obtained low-surface-area hard carbon greatly improves the first-cycle Coulombic efficiency from 74% to 83% and delivers a very stable cyclic life with 95% of capacity retention after 200 cycles.
- Authors:
-
- Oregon State Univ., Corvallis, OR (United States)
- Sharp Laboratories, Inc., Camas, WA (United States)
- Publication Date:
- Research Org.:
- Oregon State Univ., Corvallis, OR (United States)
- Sponsoring Org.:
- USDOE Advanced Research Projects Agency - Energy (ARPA-E)
- OSTI Identifier:
- 1224082
- Grant/Contract Number:
- AR0000297
- Resource Type:
- Accepted Manuscript
- Journal Name:
- ACS Applied Materials and Interfaces
- Additional Journal Information:
- Journal Volume: 7; Journal Issue: 4; Journal ID: ISSN 1944-8244
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE; hard carbon; Na-ion batteries; anode; low surface area; high first-cycle Coulombic efficiency
Citation Formats
Luo, Wei, Bommier, Clement, Jian, Zelang, Li, Xin, Carter, Rich, Vail, Sean, Lu, Yuhao, Lee, Jong -Jan, and Ji, Xiulei. Low-surface-area hard carbon anode for Na-ion batteries via graphene oxide as a dehydration agent. United States: N. p., 2015.
Web. doi:10.1021/am507679x.
Luo, Wei, Bommier, Clement, Jian, Zelang, Li, Xin, Carter, Rich, Vail, Sean, Lu, Yuhao, Lee, Jong -Jan, & Ji, Xiulei. Low-surface-area hard carbon anode for Na-ion batteries via graphene oxide as a dehydration agent. United States. https://doi.org/10.1021/am507679x
Luo, Wei, Bommier, Clement, Jian, Zelang, Li, Xin, Carter, Rich, Vail, Sean, Lu, Yuhao, Lee, Jong -Jan, and Ji, Xiulei. Wed .
"Low-surface-area hard carbon anode for Na-ion batteries via graphene oxide as a dehydration agent". United States. https://doi.org/10.1021/am507679x. https://www.osti.gov/servlets/purl/1224082.
@article{osti_1224082,
title = {Low-surface-area hard carbon anode for Na-ion batteries via graphene oxide as a dehydration agent},
author = {Luo, Wei and Bommier, Clement and Jian, Zelang and Li, Xin and Carter, Rich and Vail, Sean and Lu, Yuhao and Lee, Jong -Jan and Ji, Xiulei},
abstractNote = {Na-ion batteries are emerging as one of the most promising energy storage technologies, particularly for grid-level applications. Among anode candidate materials, hard carbon is very attractive due to its high capacity and low cost. However, hard carbon anodes often suffer a low first-cycle Coulombic efficiency and fast capacity fading. In this study, we discover that doping graphene oxide into sucrose, the precursor for hard carbon, can effectively reduce the specific surface area of hard carbon to as low as 5.4 m²/g. We further reveal that such doping can effectively prevent foaming during caramelization of sucrose and extend the pyrolysis burn-off of sucrose caramel over a wider temperature range. Thus, the obtained low-surface-area hard carbon greatly improves the first-cycle Coulombic efficiency from 74% to 83% and delivers a very stable cyclic life with 95% of capacity retention after 200 cycles.},
doi = {10.1021/am507679x},
journal = {ACS Applied Materials and Interfaces},
number = 4,
volume = 7,
place = {United States},
year = {Wed Feb 04 00:00:00 EST 2015},
month = {Wed Feb 04 00:00:00 EST 2015}
}
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