DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Soft x-ray free-electron laser induced damage to inorganic scintillators

Abstract

An irreversible response of inorganic scintillators to intense soft x-ray laser radiation was investigated at the FLASH (Free-electron LASer in Hamburg) facility. Three ionic crystals, namely, Ce:YAG (cerium-doped yttrium aluminum garnet), PbWO4 (lead tungstate), and ZnO (zinc oxide), were exposed to single 4.6 nm ultra-short laser pulses of variable pulse energy (up to 12 μJ) under normal incidence conditions with tight focus. Damaged areas produced with various levels of pulse fluences, were analyzed on the surface of irradiated samples using differential interference contrast (DIC) and atomic force microscopy (AFM). The effective beam area of 22.2 ± 2.2 μm2 was determined by means of the ablation imprints method with the use of poly(methyl methacrylate) - PMMA. Applied to the three inorganic materials, this procedure gave almost the same values of an effective area. The single-shot damage threshold fluence was determined for each of these inorganic materials. The Ce:YAG sample seems to be the most radiation resistant under the given irradiation conditions, its damage threshold was determined to be as high as 660.8 ± 71.2 mJ/cm2. Contrary to that, the PbWO4 sample exhibited the lowest radiation resistance with a threshold fluence of 62.6 ± 11.9 mJ/cm2. The threshold for ZnO was foundmore » to be 167.8 ± 30.8 mJ/cm2. Both interaction and material characteristics responsible for the damage threshold difference are discussed in the article.« less

Authors:
 [1];  [2];  [2];  [2];  [2];  [2];  [3];  [4];  [5];  [5];  [6];  [5];  [5];  [7];  [8];  [8];  [8];  [9];  [10];  [11] more »;  [11];  [12];  [12];  [13];  [14];  [15];  [16];  [17];  [2] « less
  1. Academy of Sciences of the Czech Republic (ASCR), Prague (Czech Republic). Inst. of Physics; Charles Univ. (Czech Republic)
  2. Academy of Sciences of the Czech Republic (ASCR), Prague (Czech Republic). Inst. of Physics
  3. Charles Univ. (Czech Republic)
  4. Paul Scherrer Inst. (PSI), Villigen (Switzerland); European XFEL CmbH, Hamburg (Germany)
  5. European XFEL CmbH, Hamburg (Germany)
  6. European XFEL CmbH, Hamburg (Germany); Center for Free-Electron Laser Science, Hamburg (Germany)
  7. Univ. Bordeaux (France)
  8. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
  9. Center for Free-Electron Laser Science, Hamburg (Germany); Univ. of Hamburg (Germany)
  10. Center for Free-Electron Laser Science, Hamburg (Germany); FOM Inst. DIFFER (The Netherlands)
  11. Polish Academy of Sciences (PAS), Warsaw (Poland)
  12. SLAC National Accelerator Lab., Menlo Park, CA (United States)
  13. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Inst. de minéralogie, Paris (France)
  14. Technische Univ. Wien (Germany)
  15. RIKEN, Hyogo (Japan)
  16. Slovak Academy of Sciences (Slovak Republic)
  17. P. J. Šafárik Univ. (Slovak Republic)
Publication Date:
Research Org.:
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1223351
Grant/Contract Number:  
P108/11/1312
Resource Type:
Accepted Manuscript
Journal Name:
Optical Materials Express
Additional Journal Information:
Journal Volume: 5; Journal Issue: 2; Journal ID: ISSN 2159-3930
Publisher:
Optical Society of America (OSA)
Country of Publication:
United States
Language:
English
Subject:
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY; 36 MATERIALS SCIENCE

Citation Formats

Burian, Tomáš, Hájková, Věra, Chalupský, Jaromír, Vyšín, Luděk, Boháček, Pavel, Přeček, Martin, Wild, Jan, Özkan, Cigdem, Coppola, Nicola, Farahani, Shafagh Dastjani, Schulz, Joachim, Sinn, Harald, Tschentscher, Thomas, Gaudin, Jérôme, Bajt, Saša, Tiedtke, Kai, Toleikis, Sven, Chapman, Henry N., Loch, Rolf A., Jurek, Marek, Sobierajski, Ryszard, Krzywinski, Jacek, Moeller, Stefan, Harmand, Marion, Galasso, Germano, Nagasono, Mitsuru, Saskl, Karel, Sovák, Pavol, and Juha, Libor. Soft x-ray free-electron laser induced damage to inorganic scintillators. United States: N. p., 2015. Web. doi:10.1364/OME.5.000254.
Burian, Tomáš, Hájková, Věra, Chalupský, Jaromír, Vyšín, Luděk, Boháček, Pavel, Přeček, Martin, Wild, Jan, Özkan, Cigdem, Coppola, Nicola, Farahani, Shafagh Dastjani, Schulz, Joachim, Sinn, Harald, Tschentscher, Thomas, Gaudin, Jérôme, Bajt, Saša, Tiedtke, Kai, Toleikis, Sven, Chapman, Henry N., Loch, Rolf A., Jurek, Marek, Sobierajski, Ryszard, Krzywinski, Jacek, Moeller, Stefan, Harmand, Marion, Galasso, Germano, Nagasono, Mitsuru, Saskl, Karel, Sovák, Pavol, & Juha, Libor. Soft x-ray free-electron laser induced damage to inorganic scintillators. United States. https://doi.org/10.1364/OME.5.000254
Burian, Tomáš, Hájková, Věra, Chalupský, Jaromír, Vyšín, Luděk, Boháček, Pavel, Přeček, Martin, Wild, Jan, Özkan, Cigdem, Coppola, Nicola, Farahani, Shafagh Dastjani, Schulz, Joachim, Sinn, Harald, Tschentscher, Thomas, Gaudin, Jérôme, Bajt, Saša, Tiedtke, Kai, Toleikis, Sven, Chapman, Henry N., Loch, Rolf A., Jurek, Marek, Sobierajski, Ryszard, Krzywinski, Jacek, Moeller, Stefan, Harmand, Marion, Galasso, Germano, Nagasono, Mitsuru, Saskl, Karel, Sovák, Pavol, and Juha, Libor. Wed . "Soft x-ray free-electron laser induced damage to inorganic scintillators". United States. https://doi.org/10.1364/OME.5.000254. https://www.osti.gov/servlets/purl/1223351.
@article{osti_1223351,
title = {Soft x-ray free-electron laser induced damage to inorganic scintillators},
author = {Burian, Tomáš and Hájková, Věra and Chalupský, Jaromír and Vyšín, Luděk and Boháček, Pavel and Přeček, Martin and Wild, Jan and Özkan, Cigdem and Coppola, Nicola and Farahani, Shafagh Dastjani and Schulz, Joachim and Sinn, Harald and Tschentscher, Thomas and Gaudin, Jérôme and Bajt, Saša and Tiedtke, Kai and Toleikis, Sven and Chapman, Henry N. and Loch, Rolf A. and Jurek, Marek and Sobierajski, Ryszard and Krzywinski, Jacek and Moeller, Stefan and Harmand, Marion and Galasso, Germano and Nagasono, Mitsuru and Saskl, Karel and Sovák, Pavol and Juha, Libor},
abstractNote = {An irreversible response of inorganic scintillators to intense soft x-ray laser radiation was investigated at the FLASH (Free-electron LASer in Hamburg) facility. Three ionic crystals, namely, Ce:YAG (cerium-doped yttrium aluminum garnet), PbWO4 (lead tungstate), and ZnO (zinc oxide), were exposed to single 4.6 nm ultra-short laser pulses of variable pulse energy (up to 12 μJ) under normal incidence conditions with tight focus. Damaged areas produced with various levels of pulse fluences, were analyzed on the surface of irradiated samples using differential interference contrast (DIC) and atomic force microscopy (AFM). The effective beam area of 22.2 ± 2.2 μm2 was determined by means of the ablation imprints method with the use of poly(methyl methacrylate) - PMMA. Applied to the three inorganic materials, this procedure gave almost the same values of an effective area. The single-shot damage threshold fluence was determined for each of these inorganic materials. The Ce:YAG sample seems to be the most radiation resistant under the given irradiation conditions, its damage threshold was determined to be as high as 660.8 ± 71.2 mJ/cm2. Contrary to that, the PbWO4 sample exhibited the lowest radiation resistance with a threshold fluence of 62.6 ± 11.9 mJ/cm2. The threshold for ZnO was found to be 167.8 ± 30.8 mJ/cm2. Both interaction and material characteristics responsible for the damage threshold difference are discussed in the article.},
doi = {10.1364/OME.5.000254},
journal = {Optical Materials Express},
number = 2,
volume = 5,
place = {United States},
year = {Wed Jan 07 00:00:00 EST 2015},
month = {Wed Jan 07 00:00:00 EST 2015}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 11 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

The soft x-ray free-electron laser FLASH at DESY: beamlines, diagnostics and end-stations
journal, February 2009


Measurement of gigawatt radiation pulses from a vacuum and extreme ultraviolet free-electron laser
journal, October 2003

  • Richter, M.; Gottwald, A.; Kroth, U.
  • Applied Physics Letters, Vol. 83, Issue 14
  • DOI: 10.1063/1.1614417

A compact X-ray free-electron laser emitting in the sub-ångström region
journal, June 2012


Radiation resistance of heavy scintillators to low-energy gamma-rays
journal, October 2004


First operation of a free-electron laser generating GW power radiation at 32 nm wavelength
journal, November 2005


First lasing and operation of an ångstrom-wavelength free-electron laser
journal, August 2010


Highly coherent and stable pulses from the FERMI seeded free-electron laser in the extreme ultraviolet
journal, September 2012


Analytic bond-order potential for atomistic simulations of zinc oxide
journal, June 2006


Conductors, semiconductors, and insulators irradiated with short-wavelength free-electron laser
journal, February 2007

  • Krzywinski, J.; Sobierajski, R.; Jurek, M.
  • Journal of Applied Physics, Vol. 101, Issue 4
  • DOI: 10.1063/1.2434989

Effective energy gap of semiconductors under irradiation with an ultrashort VUV laser pulse
journal, November 2009


Near edge x-ray absorption fine structure spectroscopy with x-ray free-electron lasers
text, January 2009

  • Bernstein, D. P.; Acremann, Y.; Scherz, A.
  • Deutsches Elektronen-Synchrotron, DESY, Hamburg
  • DOI: 10.3204/phppubdb-15410

Czochralski growth of YAG:Ce in a reducing protective atmosphere
journal, April 1981


Radiation induced formation of color centers in PbWO4 single crystals
journal, December 1997

  • Nikl, M.; Nitsch, K.; Baccaro, S.
  • Journal of Applied Physics, Vol. 82, Issue 11
  • DOI: 10.1063/1.366441

Efficiency and radiation hardness of phosphors in a proton beam
journal, May 1991

  • Holland, L. R.; Jenkins, G. M.; Fisher, J. H.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 56-57
  • DOI: 10.1016/0168-583x(91)95141-y

Response Time-Shortened Zinc Oxide Scintillator for Accurate Single-Shot Synchronization of Extreme Ultraviolet Free-Electron Laser and Short-Pulse Laser
journal, May 2011

  • Shimizu, Toshihiko; Yamanoi, Kohei; Sakai, Kohei
  • Applied Physics Express, Vol. 4, Issue 6
  • DOI: 10.1143/apex.4.062701

Influence of excitation density on luminescence decay in Y3Al5O12:Ce and BaF2 crystals excited by free electron laser radiation in VUV
journal, January 2005

  • Kirm, M.; Andrejczuk, A.; Krzywinski, J.
  • physica status solidi (c), Vol. 2, Issue 1
  • DOI: 10.1002/pssc.200460255

Radiation damage processes in complex-oxide scintillators
conference, May 2007

  • Nikl, Martin; Mihokova, Eva; Laguta, Valentin
  • International Congress on Optics and Optoelectronics, SPIE Proceedings
  • DOI: 10.1117/12.724737

Lead tungstate scintillation material
journal, September 2002

  • Annenkov, A. A.; Korzhik, M. V.; Lecoq, P.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 490, Issue 1-2
  • DOI: 10.1016/s0168-9002(02)00916-6

Radiation damage in scintillating crystals
journal, August 1998

  • Zhu, Ren-yuan
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 413, Issue 2-3
  • DOI: 10.1016/s0168-9002(98)00498-7

Scintillation detectors for x-rays
journal, February 2006


Near edge x-ray absorption fine structure spectroscopy with x-ray free-electron lasers
journal, September 2009

  • Bernstein, D. P.; Acremann, Y.; Scherz, A.
  • Applied Physics Letters, Vol. 95, Issue 13
  • DOI: 10.1063/1.3236540

Spot size characterization of focused non-Gaussian X-ray laser beams
journal, January 2010

  • Chalupský, J.; Krzywinski, J.; Juha, L.
  • Optics Express, Vol. 18, Issue 26
  • DOI: 10.1364/OE.18.027836

Fluence scan: an unexplored property of a laser beam
journal, January 2013

  • Chalupský, Jaromír; Burian, Tomáš; Hájková, Věra
  • Optics Express, Vol. 21, Issue 22
  • DOI: 10.1364/OE.21.026363

Characteristics of focused soft X-ray free-electron laser beam determined by ablation of organic molecular solids
journal, January 2007


Works referencing / citing this record:

Saturation of a Ce:Y$_{3}$Al$_{5}$O$_{12}$ scintillator response to ultra-short pulses of extreme ultraviolet soft X-ray and X-ray laser radiation
text, January 2017

  • Krzywinski, J.; Andrejczuk, A.; Bionta, R. M.
  • Deutsches Elektronen-Synchrotron, DESY, Hamburg
  • DOI: 10.3204/pubdb-2018-00266