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Title: Sources and composition of submicron organic mass in marine aerosol particles

Abstract

Recent studies have proposed a variety of interpretations of the sources and composition of atmospheric marine aerosol particles (aMA) based on a range of physical and chemical measurements collected during open-ocean research cruises. To investigate the processes that affect marine organic particles, this study uses the characteristic functional group composition (from Fourier transform infrared (FTIR) spectroscopy) of aMAP from five ocean regions to show that: (i) The organic functional group composition of aMAP that can be identified as atmospheric primary marine (ocean-derived) aerosol (aPMA) is 65±12% hydroxyl, 21±9% alkane, 6±6% amine, and 7±8% carboxylic acid functional groups. Contributions from photochemical reactions add carboxylic acid groups (15%-25%), shipping effluent in seawater and ship emissions add additional alkane groups (up to 70%), and coastal emissions mix in alkane and carboxylic acid groups from coastal pollution sources. (ii) The organic composition of aPMA is nearly identical to model generated primary marine aerosol particles (gPMA) from bubbled seawater (55% hydroxyl, 32% alkane, and 13% amine functional groups), indicating that its overall functional group composition is the direct consequence of the organic constituents of the seawater source. (iii) While the seawater organic functional group composition was nearly invariant across all three ocean regions studied, themore » gPMA alkane group fraction increased with chlorophyll-a concentrations (r = 0.79). gPMA from productive seawater had a larger fraction of alkane functional groups (35%) compared to gPMA from non-productive seawater (16%), likely due to the presence of surfactants in productive seawater that stabilize the bubble film and lead to preferential drainage of the more soluble (lower alkane group fraction) organic components. gPMA has a hydroxyl group absorption peak location characteristic of monosaccharides and disaccharides, where the seawater OM hydroxyl group peak location is closer to that of polysaccharides. This may result from the larger saccharides preferentially remaining in the seawater during gPMA and aPMA production« less

Authors:
 [1];  [1];  [2];  [3];  [4];  [4]
+ Show Author Affiliations
  1. Univ. of California, San Diego, CA (United States). Scripps Inst. of Oceanography.
  2. Pacific Northwest National Lab. (PNNL), Richland, WA (United States). Atmospheric Science and Global Change Div. (ASGC).
  3. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  4. National Oceanic and Atmospheric Administration (NOAA), Seattle, WA (United States). Pacific Marine Environmental Lab. (PMEL).
Publication Date:
Research Org.:
Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Biological and Environmental Research (BER)
Contributing Org.:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
OSTI Identifier:
1167616
Report Number(s):
PNNL/SA-101597
Journal ID: ISSN 2169-897X; KP1703020
Grant/Contract Number:  
AGS-1013423; OCE-1129580; AGS-1360645
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Geophysical Research: Atmospheres
Additional Journal Information:
Journal Volume: 119; Journal Issue: 22; Journal ID: ISSN 2169-897X
Publisher:
American Geophysical Union
Country of Publication:
United States
Language:
English
Subject:
58 GEOSCIENCES; 54 ENVIRONMENTAL SCIENCES; submicron organic mass; atmospheric marine aerosol particles (aMA); FTIR spectroscopy

Citation Formats

Frossard, Amanda A., Russell, Lynn M., Burrows, Susannah M., Elliott, Scott M., Bates, Timothy S., and Quinn, Patricia K. Sources and composition of submicron organic mass in marine aerosol particles. United States: N. p., 2014. Web. doi:10.1002/2014JD021913.
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Frossard, Amanda A., Russell, Lynn M., Burrows, Susannah M., Elliott, Scott M., Bates, Timothy S., & Quinn, Patricia K. Sources and composition of submicron organic mass in marine aerosol particles. United States. https://doi.org/10.1002/2014JD021913
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Frossard, Amanda A., Russell, Lynn M., Burrows, Susannah M., Elliott, Scott M., Bates, Timothy S., and Quinn, Patricia K. Thu . "Sources and composition of submicron organic mass in marine aerosol particles". United States. https://doi.org/10.1002/2014JD021913. https://www.osti.gov/servlets/purl/1167616.
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@article{osti_1167616,
title = {Sources and composition of submicron organic mass in marine aerosol particles},
author = {Frossard, Amanda A. and Russell, Lynn M. and Burrows, Susannah M. and Elliott, Scott M. and Bates, Timothy S. and Quinn, Patricia K.},
abstractNote = {Recent studies have proposed a variety of interpretations of the sources and composition of atmospheric marine aerosol particles (aMA) based on a range of physical and chemical measurements collected during open-ocean research cruises. To investigate the processes that affect marine organic particles, this study uses the characteristic functional group composition (from Fourier transform infrared (FTIR) spectroscopy) of aMAP from five ocean regions to show that: (i) The organic functional group composition of aMAP that can be identified as atmospheric primary marine (ocean-derived) aerosol (aPMA) is 65±12% hydroxyl, 21±9% alkane, 6±6% amine, and 7±8% carboxylic acid functional groups. Contributions from photochemical reactions add carboxylic acid groups (15%-25%), shipping effluent in seawater and ship emissions add additional alkane groups (up to 70%), and coastal emissions mix in alkane and carboxylic acid groups from coastal pollution sources. (ii) The organic composition of aPMA is nearly identical to model generated primary marine aerosol particles (gPMA) from bubbled seawater (55% hydroxyl, 32% alkane, and 13% amine functional groups), indicating that its overall functional group composition is the direct consequence of the organic constituents of the seawater source. (iii) While the seawater organic functional group composition was nearly invariant across all three ocean regions studied, the gPMA alkane group fraction increased with chlorophyll-a concentrations (r = 0.79). gPMA from productive seawater had a larger fraction of alkane functional groups (35%) compared to gPMA from non-productive seawater (16%), likely due to the presence of surfactants in productive seawater that stabilize the bubble film and lead to preferential drainage of the more soluble (lower alkane group fraction) organic components. gPMA has a hydroxyl group absorption peak location characteristic of monosaccharides and disaccharides, where the seawater OM hydroxyl group peak location is closer to that of polysaccharides. This may result from the larger saccharides preferentially remaining in the seawater during gPMA and aPMA production},
doi = {10.1002/2014JD021913},
journal = {Journal of Geophysical Research: Atmospheres},
number = 22,
volume = 119,
place = {United States},
year = {Thu Nov 27 00:00:00 EST 2014},
month = {Thu Nov 27 00:00:00 EST 2014}
}
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Figures / Tables:

Table 1 Table 1: Definitions of marine aerosol and relevant seawater terminology.
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  • Environmental Monitoring and Assessment, Vol. 193, Issue 1
  • DOI: 10.1007/s10661-020-08783-4

The production, concentration, and vertical distribution of the sea-salt aerosol
journal, January 1980

  • Blanchard, D. C.; Woodcock, A. H.
  • Deep Sea Research Part B. Oceanographic Literature Review, Vol. 27, Issue 12, p. 881
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Infrared Spectra of Carbohydrates
book, January 1957

Chemical Oceanography and the Marine Carbon Cycle
journal, January 2009

  • Amon, Rainer
  • Journal of the American Chemical Society, Vol. 131, Issue 6
  • DOI: 10.1021/ja900090t

Hierarchical Grouping to Optimize an Objective Function
journal, March 1963

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    Evidence for marine biogenic influence on summertime Arctic aerosol: SUMMERTIME ARCTIC AEROSOL COMPOSITION
    journal, June 2017

    • Willis, Megan D.; Köllner, Franziska; Burkart, Julia
    • Geophysical Research Letters, Vol. 44, Issue 12
    • DOI: 10.1002/2017gl073359

    Large Increases in Primary Trimethylaminium and Secondary Dimethylaminium in Atmospheric Particles Associated With Cyclonic Eddies in the Northwest Pacific Ocean
    journal, November 2018

    • Hu, Qingjing; Qu, Keming; Gao, Huiwang
    • Journal of Geophysical Research: Atmospheres, Vol. 123, Issue 21
    • DOI: 10.1029/2018jd028836

    Substantial Seasonal Contribution of Observed Biogenic Sulfate Particles to Cloud Condensation Nuclei
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    Chemical transfer of dissolved organic matter from surface seawater to sea spray water-soluble organic aerosol in the marine atmosphere
    journal, October 2018

    Factors driving the seasonal and hourly variability of sea-spray aerosol number in the North Atlantic
    journal, September 2019

    • Saliba, Georges; Chen, Chia-Li; Lewis, Savannah
    • Proceedings of the National Academy of Sciences, Vol. 116, Issue 41
    • DOI: 10.1073/pnas.1907574116

    Natural aerosols explain seasonal and spatial patterns of Southern Ocean cloud albedo
    journal, July 2015

    • McCoy, Daniel T.; Burrows, Susannah M.; Wood, Robert
    • Science Advances, Vol. 1, Issue 6
    • DOI: 10.1126/sciadv.1500157

    Evaluating Uncertainties in Marine Biogeochemical Models: Benchmarking Aerosol Precursors
    journal, May 2018

    • Ogunro, Oluwaseun; Elliott, Scott; Wingenter, Oliver
    • Atmosphere, Vol. 9, Issue 5
    • DOI: 10.3390/atmos9050184

    A physically based framework for modeling the organic fractionation of sea spray aerosol from bubble film Langmuir equilibria
    journal, January 2014

    • Burrows, S. M.; Ogunro, O.; Frossard, A. A.
    • Atmospheric Chemistry and Physics, Vol. 14, Issue 24
    • DOI: 10.5194/acp-14-13601-2014

    The impacts of regional shipping emissions on the chemical characteristics of coastal submicron aerosols near Houston, TX
    journal, January 2018

    • Schulze, Benjamin C.; Wallace, Henry W.; Bui, Alexander T.
    • Atmospheric Chemistry and Physics, Vol. 18, Issue 19
    • DOI: 10.5194/acp-18-14217-2018

    High summertime aerosol organic functional group concentrations from marine and seabird sources at Ross Island, Antarctica, during AWARE
    journal, January 2018

    • Liu, Jun; Dedrick, Jeramy; Russell, Lynn M.
    • Atmospheric Chemistry and Physics, Vol. 18, Issue 12
    • DOI: 10.5194/acp-18-8571-2018

    Classification of aerosol population type and cloud condensation nuclei properties in a coastal California littoral environment using an unsupervised cluster model
    journal, January 2019

    • Atwood, Samuel A.; Kreidenweis, Sonia M.; DeMott, Paul J.
    • Atmospheric Chemistry and Physics, Vol. 19, Issue 10
    • DOI: 10.5194/acp-19-6931-2019

    An open platform for Aerosol InfraRed Spectroscopy analysis – AIRSpec
    journal, January 2019

    • Reggente, Matteo; Höhn, Rudolf; Takahama, Satoshi
    • Atmospheric Measurement Techniques, Vol. 12, Issue 4
    • DOI: 10.5194/amt-12-2313-2019

    An automated baseline correction protocol for infrared spectra of atmospheric aerosols collected on polytetrafluoroethylene (Teflon) filters
    journal, January 2016

    • Kuzmiakova, Adele; Dillner, Ann M.; Takahama, Satoshi
    • Atmospheric Measurement Techniques, Vol. 9, Issue 6
    • DOI: 10.5194/amt-9-2615-2016

    The Ocean's Vital Skin: Toward an Integrated Understanding of the Sea Surface Microlayer
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    Size-resolved aerosol and cloud condensation nuclei (CCN) properties in the remote marine South China Sea – Part 1: Observations and source classification
    journal, January 2017

    • Atwood, Samuel A.; Reid, Jeffrey S.; Kreidenweis, Sonia M.
    • Atmospheric Chemistry and Physics, Vol. 17, Issue 2
    • DOI: 10.5194/acp-17-1105-2017

    An open platform for Aerosol InfraRed Spectroscopy analysis – AIRSpec
    posted_content, December 2018

    • Reggente, Matteo; Höhn, Rudolf; Takahama, Satoshi
    • Atmospheric Measurement Techniques
    • DOI: 10.5194/amt-2018-332

    The potential role of methanesulfonic acid (MSA) in aerosol formation and growth and the associated radiative forcings
    journal, January 2019

    • Hodshire, Anna L.; Campuzano-Jost, Pedro; Kodros, John K.
    • Atmospheric Chemistry and Physics, Vol. 19, Issue 5
    • DOI: 10.5194/acp-19-3137-2019

    An Automated Baseline Correction Protocol for Infrared Spectra of Atmospheric Aerosols Collected on Polytetrafluoroethylene (Teflon) Filters
    posted_content, January 2016

    • Kuzmiakova, Adele; Dillner, Ann M.; Takahama, Satoshi
    • Atmospheric Measurement Techniques
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    The impacts of regional shipping emissions on the chemical characteristics of coastal submicron aerosols near Houston, TX
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    • Schulze, Benjamin C.; Wallace, Henry W.; Bui, Alexander T.
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    XRF and FTIR data from Pismo Beach Air Quality Study from May 2019 - May 2021
    dataset, January 2022

    • Lewis, Savannah L.; Russell, Lynn M.; McKinsey, John A.
    • UC San Diego Library Digital Collections
    • DOI: 10.6075/j04f1qww
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