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Title: Robust multiresonant nonlocal metasurfaces by rational design

Journal Article · · Nanophotonics (Online)

Dielectric metasurfaces supporting optical resonances have become a promising platform for quantum and nonlinear optics. However, resonant metasurfaces remain limited in their capacity to independently control the behavior of many distinct resonances despite efforts in computational optimization and inverse design. In this work, we overcome longstanding limitations by introducing a generalized rational design paradigm based on symmetry. Specifically, we use symmetry-broken metasurfaces with periodic “quadromer” lattices comprised of four nanostructures per unit cell to enable extensive control of multiple optical resonances. The rationally designed metasurfaces are readily fabricable, and we experimentally demonstrate metasurfaces that support up to four high Q-factor resonances with deliberately chosen free-space polarizations, spectral separations, and mode profiles. Our design paradigm may unlock new applications for multiresonant metasurfaces in quantum and nonlinear optics, optical sensing, and augmented reality displays.

Research Organization:
Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)
Grant/Contract Number:
NA0003525
OSTI ID:
2510942
Report Number(s):
SAND--2025-04202J
Journal Information:
Nanophotonics (Online), Journal Name: Nanophotonics (Online) Journal Issue: 4 Vol. 14; ISSN 2192-8614
Publisher:
de GruyterCopyright Statement
Country of Publication:
United States
Language:
English

References (40)

Enhanced Infrared Vision by Nonlinear Up‐Conversion in Nonlocal Metasurfaces journal June 2024
Diffractive Nonlocal Metasurfaces journal July 2022
Legume: A free implementation of the guided-mode expansion method for photonic crystal slabs journal November 2024
Frequency Conversion in a Time-Variant Dielectric Metasurface journal September 2020
Polarization Engineering of Entangled Photons from a Lithium Niobate Nonlinear Metasurface journal August 2023
Topology Optimization Enables High-Q Metasurface for Color Selectivity journal July 2024
Optomechanical Enhancement of Doubly Resonant 2D Optical Nonlinearity journal February 2016
Light-Emitting Metasurfaces: Simultaneous Control of Spontaneous Emission and Far-Field Radiation journal October 2018
Generative Model for the Inverse Design of Metasurfaces journal September 2018
Inverse Design of Photonic Crystals through Automatic Differentiation journal June 2020
Zone-Folded Quasi-bound State Metasurfaces with Customized, Symmetry-Protected Energy-Momentum Relations journal May 2023
Roadmap for Optical Metasurfaces journal February 2024
Broken Symmetry Dielectric Resonators for High Quality Factor Fano Metasurfaces journal November 2016
Enhanced Second-Harmonic Generation Using Broken Symmetry III–V Semiconductor Fano Metasurfaces journal January 2018
Observation of trapped light within the radiation continuum journal July 2013
Multifunctional resonant wavefront-shaping meta-optics based on multilayer and multi-perturbation nonlocal metasurfaces journal August 2022
Unlocking the out-of-plane dimension for photonic bound states in the continuum to achieve maximum optical chirality journal October 2023
Resolving molecule-specific information in dynamic lipid membrane processes with multi-resonant infrared metasurfaces journal June 2018
Realizing symmetry-guaranteed pairs of bound states in the continuum in metasurfaces journal December 2022
Brillouin zone folding driven bound states in the continuum journal May 2023
Non-local metasurfaces for spectrally decoupled wavefront manipulation and eye tracking journal September 2021
Continuous spectral and coupling-strength encoding with dual-gradient metasurfaces journal August 2024
Passive bias-free non-reciprocal metasurfaces based on thermally nonlinear quasi-bound states in the continuum journal November 2023
Sum-frequency generation in doubly resonant GaP photonic crystal nanocavities journal July 2010
Near-field imaging of optical resonances in silicon metasurfaces using photoelectron microscopy journal June 2024
Roadmap on photonic metasurfaces journal June 2024
Selection rules for quasibound states in the continuum journal July 2020
Symmetry, degeneracy, and uncoupled modes in two-dimensional photonic lattices journal September 1995
Experimental Observation of Optical Bound States in the Continuum journal October 2011
Asymmetric Metasurfaces with High- Q Resonances Governed by Bound States in the Continuum journal November 2018
Multifunctional Nonlocal Metasurfaces journal July 2020
Parity-Time Symmetric Nonlocal Metasurfaces: All-Angle Negative Refraction and Volumetric Imaging journal October 2016
Angle-multiplexed all-dielectric metasurfaces for broadband molecular fingerprint retrieval journal May 2019
Imaging-based molecular barcoding with pixelated dielectric metasurfaces journal June 2018
Resonant metasurfaces for generating complex quantum states journal August 2022
Dimerized high contrast gratings journal June 2018
Designing nanophotonic structures using conditional deep convolutional generative adversarial networks journal June 2019
Active nonlocal metasurfaces journal September 2020
Si metasurface supporting multiple quasi-BICs for degenerate four-wave mixing journal June 2024
Inverse design of nonlinear metasurfaces for sum frequency generation journal June 2024