Nature of polariton transport in a Fabry-Perot cavity
[1];
[2];
- University of Pennsylvania, Philadelphia, PA (United States)
- University of Pennsylvania, Philadelphia, PA (United States); Department of Chemistry and Biochemistry, Notre Dame, IN (United States)
- Arizona State University, Tempe, AZ (United States); Arizona State University, Mesa, AZ (United States)
- University of Pennsylvania, Philadelphia, PA (United States); Tel Aviv University (Israel)
Fabry-Perot microcavities can strongly enhance interactions between light and molecules, leading to the formation of hybrid light-matter states known as polaritons. Polaritons possess much smaller effective masses and much larger group velocities when the molecules are resonant with cavity modes that have finite (nonzero) in-plane wave vectors, giving rise to the possibilities of long-range and ultrafast ballistic transport. In this paper, we present the results of numerical simulations of the ultrafast ballistic transport phenomenon in real space and time during and after initialization with a short, spatially localized pulse. Here, we address this problem with two approaches: the standard transfer-matrix method (TMM) for planar structures and a second simulation based on the numerical solution of the Maxwell-Bloch equations that can be used for general configurations (complex metasurfaces, for instance) and excitation modes. The agreement between the TMM and the full numerical calculation with the Maxwell-Bloch equations when applied to multilayer planar configurations provides proof of the validity of both approaches for the present analyses. Overall, we find that the transport of the molecular excitons inside the cavity synchronize with the evolution of the enhanced electromagnetic field inside the cavity. Moreover, the synchronized transport rate is in good agreement with the group velocities predicted from a calculated dispersion relation across a wide range of frequencies. Finally, we relate the group velocity to the Hopfield coefficient obtained from quantum modeling and suggest that the dependence of light-matter coupling on the in-plane wave vector can be an important but overlooked factor for understanding the transport behavior of polaritons. These simulations provide an intuitive tool for understanding the collective motion of light and excitons and helps us to better understand how experimental observations of polaritons should be interpreted.
- Research Organization:
- University of Pennsylvania, Philadelphia, PA (United States)
- Sponsoring Organization:
- Air Force Office of Scientific Research (AFOSR); U.S. National Science Foundation (NSF); USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES)
- Grant/Contract Number:
- SC0019397
- OSTI ID:
- 2510484
- Journal Information:
- Physical Review A, Journal Name: Physical Review A Journal Issue: 3 Vol. 109; ISSN 2469-9926
- Publisher:
- American Physical Society (APS)Copyright Statement
- Country of Publication:
- United States
- Language:
- English
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