Opportunities for gas-phase science at short-wavelength free-electron lasers with undulator-based polarization control

Ilchen, Markus; Allaria, Enrico; Rebernik Ribič, Primož; Nuhn, Heinz-Dieter; Lutman, Alberto; Schneidmiller, Evgeny; Tischer, Markus; Yurkov, Mikail; Calvi, Marco; Prat, Eduard; Reiche, Sven; Schmidt, Thomas; Geloni, Gianluca Aldo; Karabekyan, Suren; Yan, Jiawei; Serkez, Svitozar; Gao, Zhangfeng; Deng, Bangjie; Feng, Chao; Deng, Haixiao; Helml, Wolfram; Funke, Lars; Larsson, Mats; Zhaunerchyk, Vitali; Meyer, Michael; Mazza, Tommaso; Jahnke, Till; Dörner, Reinhard; Calegari, Francesca; Smirnova, Olga; Vozzi, Caterina; De Ninno, Giovanni; Wätzel, Jonas; Berakdar, Jamal; Bari, Sadia; Schwob, Lucas; Rouxel, Jérémy R.; Mukamel, Shaul; Bartschat, Klaus; Hamilton, Kathryn; Argenti, Luca; Douguet, Nicolas; Novikovskiy, Nikolay M.; Demekhin, Philipp V.; Walter, Peter

doi:10.1103/PhysRevResearch.7.011001

Title: Opportunities for gas-phase science at short-wavelength free-electron lasers with undulator-based polarization control

Journal Article · 27 January 2025 · Physical Review Research

DOI: https://doi.org/10.1103/PhysRevResearch.7.011001 · OSTI ID:2507110

Ilchen, Markus; Allaria, Enrico; Rebernik Ribič, Primož; Nuhn, Heinz-Dieter; Lutman, Alberto; Schneidmiller, Evgeny; Tischer, Markus; Yurkov, Mikail; Calvi, Marco; Prat, Eduard; Reiche, Sven; Schmidt, Thomas; Geloni, Gianluca Aldo; Karabekyan, Suren; Yan, Jiawei; Serkez, Svitozar; Gao, Zhangfeng; Deng, Bangjie; Feng, Chao; Deng, Haixiao more »

Free-electron lasers (FELs) are the world's most brilliant light sources with rapidly evolving technological capabilities in terms of ultrabright and ultrashort pulses over a large range of photon energies. Their revolutionary and innovative developments have opened new fields of science regarding nonlinear light-matter interaction, the investigation of ultrafast processes from specific observer sites, and approaches to imaging matter with atomic resolution. A core aspect of FEL science is the study of isolated and prototypical systems in the gas phase with the possibility of addressing well-defined electronic transitions or particular atomic sites in molecules. Notably for polarization-controlled short-wavelength FELs, the gas phase offers new avenues for investigations of nonlinear and ultrafast phenomena in spin-orientated systems, for decoding the function of the chiral building blocks of life as well as steering reactions and particle emission dynamics in otherwise inaccessible ways. This roadmap comprises descriptions of technological capabilities of facilities worldwide, innovative diagnostics and instrumentation, as well as recent scientific highlights, novel methodology, and mathematical modeling. The experimental and theoretical landscape of using polarization controllable FELs for dichroic light-matter interaction in the gas phase will be discussed and comprehensively outlined to stimulate and strengthen global collaborative efforts of all disciplines. Published by the American Physical Society 2025

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Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-06CH11357; AC02-76SF00515; SC0020311

OSTI ID:: 2507110

Journal Information:: Physical Review Research, Journal Name: Physical Review Research Journal Issue: 1 Vol. 7; ISSN 2643-1564; ISSN PPRHAI

Publisher:: American Physical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Wavefront metrology measurements at SACLA by means of X-ray grating interferometry Kayser, Yves; Rutishauser, Simon; Katayama, Tetsuo Optics Express, Vol. 22, Issue 8 https://doi.org/10.1364/OE.22.009004	journal	January 2014
Characterizing isolated attosecond pulses with angular streaking Li, Siqi; Guo, Zhaoheng; Coffee, Ryan N. Optics Express, Vol. 26, Issue 4 https://doi.org/10.1364/OE.26.004531	journal	January 2018
Ultrafast optical rotation in chiral molecules with ultrashort and tightly focused beams Ayuso, David; Ordonez, Andres F.; Ivanov, Misha Optica, Vol. 8, Issue 10 https://doi.org/10.1364/OPTICA.423618	journal	September 2021
Status of the SXFEL Facility Zhao, Zhentang; Wang, Dong; Gu, Qiang Applied Sciences, Vol. 7, Issue 6, p. 607 https://doi.org/10.3390/app7060607	journal	June 2017
Ab Initio Simulation of Attosecond Transient Absorption Spectroscopy in Two-Dimensional Materials Sato, Shunsuke; Hübener, Hannes; De Giovannini, Umberto Applied Sciences, Vol. 8, Issue 10 https://doi.org/10.3390/app8101777	journal	September 2018
Continuum Electronic States: The Tiresia Code Decleva, Piero; Stener, Mauro; Toffoli, Daniele Molecules, Vol. 27, Issue 6 https://doi.org/10.3390/molecules27062026	journal	March 2022

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