Using Radiogenic Noble Gas Nuclides to Identify and Characterize Rock Fracturing

Journal Article · 23 January 2025 · Earth and Space Science

DOI: https://doi.org/10.1029/2024ea003838 · OSTI ID:2505087

Gardner, W. Payton  ^[1]; Bauer, Stephen J.  ^[2]; Kibikas, William Martin  ^[2]; Siluk, Brynna Morgan  ^[3]; Broome, Scott Thomas ^[2]; Strickland, Chris ^[4]; Johnson, Christine  ^[4]; Vermeul, Vince ^[4]

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1. Univ. of Montana, Missoula, MT (United States)
2. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
3. Univ. of New Mexico, Albuquerque, NM (United States)
4. Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Fracture-released radiogenic noble gas nuclides are used to identify locations and constrain the volume of new fracture creation during subsurface detonations. Real-time, in situ noble gases and reactive gases were monitored using a field-deployed mass spectrometer and automated sampling system in a multilevel borehole array. Released gases were measured after two different detonations having distinct energy, pressure, and gas volume characteristics. Explosive-derived gases (N₂O, CO₂) and excess radiogenic ⁴He and ⁴⁰Ar above atmospheric background are used to identify locations of gas transport and new fracture creation after each detonation. Fracture-released radiogenic ⁴He is used to constrain the volume of newly created fractures with a model of helium release from fracturing. Explosive by-product gas was observed in multiple locations both near and distal to the shot locations for both detonations. Radiogenic ⁴He and ⁴⁰Ar release from rock damage was observed in locations near the detonation after the second, more powerful detonation. Observed ⁴He response is consistent with a model of diffusive release from newly created fractures. Volume of new fractures estimated from the ⁴He release ranges from 1 to 5 m² with apertures ranging from 0.1 to 1 m. Our results provide evidence that radiogenic noble gases released during fracture creation can be identified at the field scale in real time and used to identify timing and location of fracture creation during deformation events. This technique could be useful in subsurface science and engineering problems where the location and amount of newly created rock fracturing is of interest including fault rupture, mine safety, subsurface detonation monitoring and reservoir stimulation.

• Research Organization: Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States)
• Sponsoring Organization: USDOE; USDOE National Nuclear Security Administration (NNSA), Office of Defense Nuclear Nonproliferation; USDOE Office of Nuclear Energy (NE); USDOE Office of Science (SC)
• Grant/Contract Number: NA0003525; NE0008786; SC0021088
• OSTI ID: 2505087
• Report Number(s): SAND--2025-05640J
• Journal Information: Earth and Space Science, Journal Name: Earth and Space Science Journal Issue: 1 Vol. 12; ISSN 2333-5084
• Publisher: American Geophysical Union (AGU) - WileyCopyright Statement
• Country of Publication: United States
• Language: English