Cavity-enhanced high-order harmonic generation for high-performance time-resolved photoemission experiments

Allison, Thomas K.; Kunin, Alice; Schönhense, Gerd

doi:10.1063/5.0244045

Title: Cavity-enhanced high-order harmonic generation for high-performance time-resolved photoemission experiments

Journal Article · 22 January 2025 · APL Photonics

DOI: https://doi.org/10.1063/5.0244045 · OSTI ID:2505086

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Recent breakthroughs in high repetition-rate extreme ultraviolet (XUV) light sources and photoelectron analyzers have led to dramatic advances in the performance of time-resolved photoemission experiments. In this perspective article, we discuss the application of cavity-enhanced high-order harmonic generation, with repetition rates exceeding 10 MHz, to photoemission experiments using advanced endstations incorporating time-of-flight photoelectron analyzers. We discuss recent results, perspective on future areas for further technological improvement, and the wide array of science enabled by ultrafast XUV photoemission experiments, now in a qualitatively new regime.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: NONE; SC0022004

OSTI ID:: 2505086

Journal Information:: APL Photonics, Journal Name: APL Photonics Journal Issue: 1 Vol. 10; ISSN 2378-0967

Publisher:: American Institute of PhysicsCopyright Statement

Country of Publication:: United States

Language:: English

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Enhancement cavities for few-cycle pulses Lilienfein, N.; Hofer, C.; Holzberger, S. Optics Letters, Vol. 42, Issue 2 https://doi.org/10.1364/ol.42.000271	journal	January 2017
Extreme ultraviolet light source at a megahertz repetition rate based on high-harmonic generation inside a mode-locked thin-disk laser oscillator Labaye, F.; Gaponenko, M.; Wittwer, V. J. Optics Letters, Vol. 42, Issue 24 https://doi.org/10.1364/ol.42.005170	journal	January 2017
High-power frequency comb at 2 μm wavelength emitted by a Tm-doped fiber laser system Gaida, C.; Heuermann, T.; Gebhardt, M. Optics Letters, Vol. 43, Issue 21 https://doi.org/10.1364/ol.43.005178	journal	January 2018
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High-harmonic generation at 250 MHz with photon energies exceeding 100 eV Carstens, H.; Högner, M.; Saule, T. Optica, Vol. 3, Issue 4 https://doi.org/10.1364/optica.3.000366	journal	January 2016
Molecular fingerprinting with bright, broadband infrared frequency combs Timmers, Henry; Kowligy, Abijith; Lind, Alex Optica, Vol. 5, Issue 6 https://doi.org/10.1364/optica.5.000727	journal	January 2018
Low-repetition-rate optical frequency comb Canella, Francesco; Weitenberg, Johannes; Thariq, Muhammad Optica, Vol. 11, Issue 1 https://doi.org/10.1364/optica.506353	journal	January 2024
Real-time observation of electronic, vibrational, and rotational dynamics in nitric oxide with attosecond soft x-ray pulses at 400 eV Saito, Nariyuki; Sannohe, Hiroki; Ishii, Nobuhisa Optica, Vol. 6, Issue 12 https://doi.org/10.1364/optica.6.001542	journal	January 2019
Realizing Attosecond Core-Level X-ray Spectroscopy for the Investigation of Condensed Matter Systems Summers, Adam M.; Severino, Stefano; Reduzzi, Maurizio Ultrafast Science, Vol. 3 https://doi.org/10.34133/ultrafastscience.0004	journal	January 2023

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