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Title: Techno-economic analysis and network design for CO2 conversion to jet fuels in the United States

Journal Article · · Renewable and Sustainable Energy Reviews
ORCiD logo [1]; ORCiD logo [1];  [2]; ORCiD logo [3]; ORCiD logo [4];  [5]
  1. Univ. of Tennessee, Knoxville, TN (United States)
  2. Zhejiang University, Hangzhou (China); Institute of Zhejiang University-Quzhou (China)
  3. Louisiana Tech Univ., Ruston, LA (United States)
  4. Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)
  5. Horace Mann School, Bronx, NY (United States)

The conversion of carbon dioxide (CO2) into jet fuel holds significant potential for reducing CO2 emissions, providing an alternative to carbon-based resources, and offering a renewable means of energy storage. The objective of this study is to conduct a techno-economic analysis and optimize the supply chain network for converting CO2 to jet fuel in the United States, aiming to minimize total costs while assessing the environmental and economic feasibility of two CO2 conversion pathways. This first pathway is based on Fischer-Tropsch synthesis (FTS), and the other one is based on the valorization and upgrading of light methanol (MeOH). Incorporating spatial and techno-economic data, a mixed-integer linear programming model was developed to select source plants and conversion pathways, locations of conversion refinery sites, and the amount of captured CO2 across the United States. The optimal results indicate that the FTS pathway is adopted at all selected refineries when the hydrogen price is 1000 dollars/t and the operating cost, mainly electricity used in conversion, is reduced to 5 % of its current level. Under this scenario, the total annual profit is 8 billion dollars, and the net carbon emissions are -88,783,284 tons. The sensitivity analyses reveal that the prices of electricity and hydrogen significantly contribute to total production costs. The CO2 recycle percentage of the FTS pathway influences the choice of applied pathways at refineries. Additionally, a higher conversion rate holds a substantial promise for reducing the total production cost and can make the MeOH pathway a viable choice.

Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Energy Efficiency and Renewable Energy (EERE)
Grant/Contract Number:
AC05-00OR22725
OSTI ID:
2483942
Journal Information:
Renewable and Sustainable Energy Reviews, Journal Name: Renewable and Sustainable Energy Reviews Vol. 210; ISSN 1364-0321
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

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