Birefringent Color Filter by Layered Metal‐Organic Chalcogenides: In‐Plane Anisotropy and Odd/Even Effect

Ye, Zichao; Zhao, Jie; Kang, Kisung; McCormack, Scott J.; Shao, Yu‐Tsun; Efremov, Mikhail Y.; Schleife, André; Kriven, Waltraud M.; Zuo, Jian‐Min; Allen, Leslie H.

doi:10.1002/adom.202402159

Title: Birefringent Color Filter by Layered Metal‐Organic Chalcogenides: In‐Plane Anisotropy and Odd/Even Effect

Journal Article · 24 December 2024 · Advanced Optical Materials

DOI: https://doi.org/10.1002/adom.202402159 · OSTI ID:2483925

Ye, Zichao ^[1]; Zhao, Jie ^[1];

^[1]; McCormack, Scott J. ^[2]; Shao, Yu‐Tsun ^[3]; Efremov, Mikhail Y. ^[4];

^[1]; Kriven, Waltraud M. ^[1]; Zuo, Jian‐Min ^[1];

^[1]

Univ. of Illinois at Urbana-Champaign, IL (United States)
Univ. of Illinois at Urbana-Champaign, IL (United States); Univ. of California, Davis, CA (United States)
Univ. of Illinois at Urbana-Champaign, IL (United States); Univ. of Southern California, Los Angeles, CA (United States)
Univ. of Wisconsin, Madison, WI (United States)

Anisotropic 2D materials are gaining interest recently as building blocks for angular‐dependent optical/electrical devices. However, the fundamental understanding of their structure‐property‐relationship is limited, which hinders further modulation of their unique characteristics via structure tailoring. Here the in‐plane structural anisotropy and the tunable optical/electrical properties of a series of radiation‐sensitive (X‐ray, e‐beam) metal‐organic chalcogenide (MOC) single crystals are comprehensively revealed with ligands of variable length/parity. Their monoclinic crystallography is determined at atomic resolution by a simple method that couples X‐ray/electron diffraction with first‐principles calculations. The in‐plane inorganic backbone of the MOCs exhibits a strong lattice anisotropy with odd/even alternations, which originates from that of the out‐of‐plane organic motifs via organic/inorganic accommodation. Such structural anisotropy is implied mechanically by the preferred orientation of crystal cleavage. It triggers a maximum ≈8 × distinction of in‐plane electrical conductivity of the semiconducting MOCs, plus a distinct birefringence (maximum Δn ≈ 0.03) with a dispersive orientation of dielectric axes, which rotate up to 25.7° from UV to visible‐light regime, inspiring an emerging pathway for color filtering via single crystal rotation. Such in‐plane optical characteristics also exhibit odd/even alternation and can be flexibly tuned by the designable out‐of‐plane ligands.

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Research Organization:: Univ. of Illinois at Urbana-Champaign, IL (United States)

Sponsoring Organization:: USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)

Grant/Contract Number:: AC02-06CH11357; AC02-98CH10886; SC0024064

OSTI ID:: 2483925

Journal Information:: Advanced Optical Materials, Journal Name: Advanced Optical Materials Journal Issue: 9 Vol. 13; ISSN 2195-1071

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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birefringence
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Title: Birefringent Color Filter by Layered Metal‐Organic Chalcogenides: In‐Plane Anisotropy and Odd/Even Effect

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