Exploring Quantum Materials with Resonant Inelastic X-Ray Scattering

Mitrano, M.; Johnston, S.; Kim, Young-June; Dean, M. P. M.

doi:10.1103/physrevx.14.040501

Title: Exploring Quantum Materials with Resonant Inelastic X-Ray Scattering

Journal Article · 13 December 2024 · Physical Review. X

DOI: https://doi.org/10.1103/physrevx.14.040501 · OSTI ID:2481399

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Harvard Univ., Cambridge, MA (United States)
Univ. of Tennessee, Knoxville, TN (United States)
Univ. of Toronto, ON (Canada)
Brookhaven National Laboratory (BNL), Upton, NY (United States)

Understanding quantum materials—solids in which interactions among constituent electrons yield a great variety of novel emergent quantum phenomena—is a forefront challenge in modern condensed matter physics. This goal has driven the invention and refinement of several experimental methods, which can spectroscopically determine the elementary excitations and correlation functions that determine material properties. Here we focus on the future experimental and theoretical trends of resonant inelastic x-ray scattering (RIXS), which is a remarkably versatile and rapidly growing technique for probing different charge, lattice, spin, and orbital excitations in quantum materials. We provide a forward-looking introduction to RIXS and outline how this technique is poised to deepen our insight into the nature of quantum materials and of their emergent electronic phenomena.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012704

OSTI ID:: 2481399

Report Number(s):: BNL--226450-2024-JAAM

Journal Information:: Physical Review. X, Journal Name: Physical Review. X Journal Issue: 4 Vol. 14; ISSN 2160-3308

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Correlation functions measured by indirect resonant inelastic X-ray scattering Brink, J. van den; Veenendaal, M. van Europhysics Letters (EPL), Vol. 73, Issue 1 https://doi.org/10.1209/epl/i2005-10366-9	journal	January 2006
Beyond the single-site approximation modeling of electron-phonon coupling effects on resonant inelastic X-ray scattering spectra Bieniasz, Krzysztof; Johnston, Steven; Berciu, Mona SciPost Physics, Vol. 11, Issue 3 https://doi.org/10.21468/SciPostPhys.11.3.062	journal	January 2021
Measurement of the dynamic charge response of materials using low-energy, momentum-resolved electron energy-loss spectroscopy (M-EELS) Vig, Sean; Kogar, Anshul; Mitrano, Matteo SciPost Physics, Vol. 3, Issue 4 https://doi.org/10.21468/SciPostPhys.3.4.026	journal	January 2017
X-Ray Performance of Critical-angle Transmission Grating Prototypes for the Arcus Mission Heilmann, Ralf K.; Bruccoleri, Alexander R.; Burwitz, Vadim The Astrophysical Journal, Vol. 934, Issue 2 https://doi.org/10.3847/1538-4357/ac7a3a	journal	August 2022
Hunting Majorana Fermions in Kitaev Magnets Motome, Yukitoshi; Nasu, Joji Journal of the Physical Society of Japan, Vol. 89, Issue 1 https://doi.org/10.7566/JPSJ.89.012002	journal	January 2020

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