Interstitial and substitutional doping of Mn 2+ in 2D PEA 2 PbBr 4 and BA 2 PbBr 4 perovskites

Kuruppu, Udara M.; Magdaleno, Alvaro J.; Kshirsagar, Anuraj S.; Donnadieu, Bruno; Prins, Ferry; Gangishetty, Mahesh K.

doi:10.1039/D4CC04074K

Title: Interstitial and substitutional doping of Mn ²⁺ in 2D PEA ₂ PbBr ₄ and BA ₂ PbBr ₄ perovskites

Journal Article · 11 December 2024 · ChemComm

DOI: https://doi.org/10.1039/D4CC04074K · OSTI ID:2481000

^[1]; Magdaleno, Alvaro J. ^[2];

^[1]; Donnadieu, Bruno ^[1];

^[2];

^[3]

Department of Chemistry, Mississippi State University, Mississippi State, Mississippi 39762, USA
Condensed Matter Physics Center (IFIMAC), Autonomous University of Madrid, 28049, Madrid, Spain, Department of Condensed Matter Physics, Autonomous University of Madrid, 28049, Madrid, Spain
Department of Chemistry, Mississippi State University, Mississippi State, Mississippi 39762, USA, Department of Physics and Astronomy, Mississippi State University, Mississippi State, Mississippi 39762, USA

Mn ²⁺ doping imposes intriguing optoelectronic properties on lead-halide perovskites; however, its impact on their crystal structure remains unclear.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: SC0024214

OSTI ID:: 2481000

Journal Information:: ChemComm, Journal Name: ChemComm Journal Issue: 100 Vol. 60; ISSN CHCOFS; ISSN 1359-7345

Publisher:: Royal Society of Chemistry (RSC)Copyright Statement

Country of Publication:: United Kingdom

Language:: English

References (13)

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Efficient Exciton to Dopant Energy Transfer in Mn ²⁺ -Doped (C ₄ H ₉ NH ₃ ) ₂ PbBr ₄ Two-Dimensional (2D) Layered Perovskites Biswas, Anupam; Bakthavatsalam, Rangarajan; Kundu, Janardan Chemistry of Materials, Vol. 29, Issue 18 https://doi.org/10.1021/acs.chemmater.7b02429	journal	September 2017
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Tuning the Structural Rigidity of Two-Dimensional Ruddlesden–Popper Perovskites through the Organic Cation Fridriksson, Magnus B.; van der Meer, Nadia; de Haas, Jiska The Journal of Physical Chemistry C, Vol. 124, Issue 51 https://doi.org/10.1021/acs.jpcc.0c08893	journal	December 2020
Mn Doping in Centimeter-Sized Layered 2D Butylammonium Lead Bromide (BA ₂ PbBr ₄ ) Single Crystals and Their Optical Properties Sheikh, Tariq; Nag, Angshuman The Journal of Physical Chemistry C, Vol. 123, Issue 14 https://doi.org/10.1021/acs.jpcc.9b01550	journal	March 2019
Electrons, Excitons, and Phonons in Two-Dimensional Hybrid Perovskites: Connecting Structural, Optical, and Electronic Properties Straus, Daniel B.; Kagan, Cherie R. The Journal of Physical Chemistry Letters, Vol. 9, Issue 6 https://doi.org/10.1021/acs.jpclett.8b00201	journal	February 2018
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Exciton diffusion in two-dimensional metal-halide perovskites Seitz, Michael; Magdaleno, Alvaro J.; Alcázar-Cano, Nerea Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-15882-w	journal	April 2020

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Title: Interstitial and substitutional doping of Mn ²⁺ in 2D PEA ₂ PbBr ₄ and BA ₂ PbBr ₄ perovskites