High-temperature 205Tl decay clarifies 205Pb dating in early Solar System

Leckenby, Guy; Sidhu, Ragandeep Singh; Chen, Rui Jiu; Mancino, Riccardo; Szányi, Balázs; Bai, Mei; Battino, Umberto; Blaum, Klaus; Brandau, Carsten; Cristallo, Sergio; Dickel, Timo; Dillmann, Iris; Dmytriiev, Dmytro; Faestermann, Thomas; Forstner, Oliver; Franczak, Bernhard; Geissel, Hans; Gernhäuser, Roman; Glorius, Jan; Griffin, Chris; Gumberidze, Alexandre; Haettner, Emma; Hillenbrand, Pierre-Michel; Karakas, Amanda; Kaur, Tejpreet; Korten, Wolfram; Kozhuharov, Christophor; Kuzminchuk, Natalia; Langanke, Karlheinz; Litvinov, Sergey; Litvinov, Yuri A.; Lugaro, Maria; Martínez-Pinedo, Gabriel; Menz, Esther; Meyer, Bradley; Morgenroth, Tino; Neff, Thomas; Nociforo, Chiara; Petridis, Nikolaos; Pignatari, Marco; Popp, Ulrich; Purushothaman, Sivaji; Reifarth, René; Sanjari, Shahab; Scheidenberger, Christoph; Spillmann, Uwe; Steck, Markus; Stöhlker, Thomas; Tanaka, Yoshiki K.; Trassinelli, Martino; Trotsenko, Sergiy; Varga, László; Vescovi, Diego; Wang, Meng; Weick, Helmut; Yagüe Lopéz, Andrés; Yamaguchi, Takayuki; Zhang, Yuhu; Zhao, Jianwei

doi:10.1038/s41586-024-08130-4

Title: High-temperature ²⁰⁵Tl decay clarifies ²⁰⁵Pb dating in early Solar System

Journal Article · 12 November 2024 · Nature (London)

DOI: https://doi.org/10.1038/s41586-024-08130-4 · OSTI ID:2478636

;

; Mancino, Riccardo; Szányi, Balázs; Bai, Mei; Battino, Umberto;

; Brandau, Carsten; Cristallo, Sergio;

;

; Dmytriiev, Dmytro;

;

; Franczak, Bernhard; Geissel, Hans;

; Glorius, Jan; Griffin, Chris more »

Radioactive nuclei with lifetimes on the order of millions of years can reveal the formation history of the Sun and active nucleosynthesis occurring at the time and place of its birth. Among such nuclei whose decay signatures are found in the oldest meteorites, ²⁰⁵Pb is a powerful example, as it is produced exclusively by slow neutron captures (the s process), with most being synthesized in asymptotic giant branch (AGB) stars. However, making accurate abundance predictions for ²⁰⁵Pb has so far been impossible because the weak decay rates of ²⁰⁵Pb and ²⁰⁵Tl are very uncertain at stellar temperatures. To constrain these decay rates, we measured for the first time the bound-state β^- decay of fully ionized ²⁰⁵Tl⁸¹⁺, an exotic decay mode that only occurs in highly charged ions. The measured half-life is 4.7 times longer than the previous theoretical estimate and our 10% experimental uncertainty has eliminated the main nuclear-physics limitation. With new, experimentally backed decay rates, we used AGB stellar models to calculate ²⁰⁵Pb yields. Propagating those yields with basic galactic chemical evolution (GCE) and comparing with the ²⁰⁵Pb/²⁰⁴Pb ratio from meteorites, we determined the isolation time of solar material inside its parent molecular cloud. We find positive isolation times that are consistent with the other s-process short-lived radioactive nuclei found in the early Solar System. Our results reaffirm the site of the Sun’s birth as a long-lived, giant molecular cloud and support the use of the ²⁰⁵Pb–²⁰⁵Tl decay system as a chronometer in the early Solar System.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE Laboratory Directed Research and Development (LDRD) Program

Contributing Organization:: The n_TOF collaboration

Grant/Contract Number:: 89233218CNA000001

OSTI ID:: 2478636

Report Number(s):: LA-UR--24-23164

Journal Information:: Nature (London), Journal Name: Nature (London) Journal Issue: 8038 Vol. 635; ISSN 0028-0836

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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¹²⁹ I and ²⁴⁷ Cm in meteorites constrain the last astrophysical source of solar r-process elements Côté, Benoit; Eichler, Marius; Yagüe López, Andrés Science, Vol. 371, Issue 6532 https://doi.org/10.1126/science.aba1111	journal	February 2021
The resonances in the $$^{22}$$Ne+$$\alpha $$ fusion reactions Wiescher, M.; deBoer, R. J.; Görres, J. The European Physical Journal A, Vol. 59, Issue 1 https://doi.org/10.1140/epja/s10050-023-00917-9	journal	January 2023
A Perspective from Extinct Radionuclides on a Young Stellar Object: The Sun and Its Accretion Disk Dauphas, Nicolas; Chaussidon, Marc Annual Review of Earth and Planetary Sciences, Vol. 39, Issue 1 https://doi.org/10.1146/annurev-earth-040610-133428	journal	May 2011
Short-Lived Nuclides in the Early Solar System: Abundances, Origins, and Applications Davis, Andrew M. Annual Review of Nuclear and Particle Science, Vol. 72, Issue 1 https://doi.org/10.1146/annurev-nucl-010722-074615	journal	September 2022
ThesProcess and Beyond Lugaro, Maria; Pignatari, Marco; Reifarth, René Annual Review of Nuclear and Particle Science, Vol. 73, Issue 1 https://doi.org/10.1146/annurev-nucl-102422-080857	journal	September 2023
The Chemical Composition of the Sun Asplund, Martin; Grevesse, Nicolas; Sauval, A. Jacques Annual Review of Astronomy and Astrophysics, Vol. 47, Issue 1 https://doi.org/10.1146/annurev.astro.46.060407.145222	journal	September 2009
Assessing Search and Unsupervised Clustering Algorithms in Nested Sampling Maillard, Lune; Finocchi, Fabio; Trassinelli, Martino Entropy, Vol. 25, Issue 2 https://doi.org/10.3390/e25020347	journal	February 2023
Stellar Yields from Metal-Rich Asymptotic Giant Branch Models Karakas, Amanda I.; Lugaro, Maria The Astrophysical Journal, Vol. 825, Issue 1 https://doi.org/10.3847/0004-637X/825/1/26	journal	June 2016
Application of a Theory and Simulation-Based Convective Boundary Mixing Model for agb star Evolution and Nucleosynthesis Battino, U.; Pignatari, M.; Ritter, C. The Astrophysical Journal, Vol. 827, Issue 1 https://doi.org/10.3847/0004-637X/827/1/30	journal	August 2016
On the Origin of Early Solar System Radioactivities: Problems with the Asymptotic Giant Branch and Massive Star Scenarios Vescovi, D.; Busso, M.; Palmerini, S. The Astrophysical Journal, Vol. 863, Issue 2 https://doi.org/10.3847/1538-4357/aad191	journal	August 2018
Galactic Chemical Evolution of Radioactive Isotopes Côté, Benoit; Lugaro, Maria; Reifarth, Rene The Astrophysical Journal, Vol. 878, Issue 2 https://doi.org/10.3847/1538-4357/ab21d1	journal	June 2019
Stochastic Chemical Evolution of Radioactive Isotopes with a Monte Carlo Approach Côté, Benoit; Yagüe, Andrés; Világos, Blanka The Astrophysical Journal, Vol. 887, Issue 2 https://doi.org/10.3847/1538-4357/ab5a88	journal	December 2019
Monte Carlo Investigation of the Ratios of Short-lived Radioactive Isotopes in the Interstellar Medium Yagüe López, Andrés; Côté, Benoit; Lugaro, Maria The Astrophysical Journal, Vol. 915, Issue 2 https://doi.org/10.3847/1538-4357/ac02bf	journal	July 2021
Galactic Chemical Evolution of Radioactive Isotopes with an s-process Contribution Trueman, Thomas C. L.; Côté, Benoit; Yagüe López, Andrés The Astrophysical Journal, Vol. 924, Issue 1 https://doi.org/10.3847/1538-4357/ac31b0	journal	January 2022
Theoretical Estimate of the Half-life for the Radioactive ¹³⁴Cs and ¹³⁵Cs in Astrophysical Scenarios Taioli, Simone; Vescovi, Diego; Busso, Maurizio The Astrophysical Journal, Vol. 933, Issue 2 https://doi.org/10.3847/1538-4357/ac74b3	journal	July 2022
Inhomogeneous Enrichment of Radioactive Nuclei in the Galaxy: Deposition of Live ⁵³Mn, ⁶⁰Fe, ¹⁸²Hf, and ²⁴⁴Pu into Deep-sea Archives. Surfing the Wave? Wehmeyer, Benjamin; López, Andrés Yagüe; Côté, Benoit The Astrophysical Journal, Vol. 944, Issue 2 https://doi.org/10.3847/1538-4357/acafec	journal	February 2023
Magnetic-buoyancy-induced Mixing in AGB Stars: Presolar SiC Grains Vescovi, Diego; Cristallo, Sergio; Busso, Maurizio The Astrophysical Journal, Vol. 897, Issue 2 https://doi.org/10.3847/2041-8213/ab9fa1	journal	July 2020
The Stellar β-decay Rate of ¹³⁴ Cs and Its Impact on the Barium Nucleosynthesis in the s-process Li, Kuo-Ang; Qi, Chong; Lugaro, Maria The Astrophysical Journal Letters, Vol. 919, Issue 2 https://doi.org/10.3847/2041-8213/ac260f	journal	September 2021

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