DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Quasi-differential neutron induced neutron emissions from 235U, and 239Pu

Journal Article · · Annals of Nuclear Energy
 [1];  [1];  [1];  [2];  [2]
  1. Rensselaer Polytechnic Inst., Troy, NY (United States)
  2. Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Uncertainty in nuclear reaction cross sections, angular distributions, and other nuclear data directly impact how well simulations of nuclear systems represent physical observations. Here, to determine how well the nuclear data in ENDF/B-VIII.0, JEFF-3.3, and JENDL-4.0 evaluations describe the physical behaviour of 235U, and 239Pu when subjected to a neutron flux, the neutron emission spectrum was measured for carbon, 93.0% 235U, and 93.9% 239Pu samples, and compared against detailed MCNP6 simulations. The measurements were performed at the Los Alamos Neutron Science Center using a quasi-differential method previously developed at Rensselaer Polytechnic Institute. The measurement spanned 0.82–20 MeV and 30–150 degrees. The measurements show there are a significant number of discrepancies between library predictions of the neutron yield and physical observation. A few of the main discrepancies found are described in this paper. Based on these results a new evaluation utilizing these results for carbon, 235U, and 239Pu is recommended.

Research Organization:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE; USDOE National Nuclear Security Administration (NNSA), Office of Defense Programs (DP); USNRC
Grant/Contract Number:
89233218CNA000001
OSTI ID:
2477789
Report Number(s):
LA-UR--20-30430
Journal Information:
Annals of Nuclear Energy, Journal Name: Annals of Nuclear Energy Vol. 165; ISSN 0306-4549
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

References (15)

A versatile pulse shape discriminator for charged particle separation and its application to fast neutron time-of-flight spectroscopy journal November 1978
A fission ionization detector for neutron flux measurements at a spallation source
  • Wender, S. A.; Balestrini, S.; Brown, A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 336, Issue 1-2 https://doi.org/10.1016/0168-9002(93)91102-S
journal November 1993
Quasi-differential neutron scattering from 238U from 0.5 to 20 MeV journal November 2014
Quasi-differential elastic and inelastic neutron scattering from iron in the MeV energy range journal December 2017
Physics of Neutron Interactions with 238U: New Developments and Challenges journal April 2014
ENDF/B-VIII.0: The 8 th Major Release of the Nuclear Reaction Data Library with CIELO-project Cross Sections, New Standards and Thermal Scattering Data journal February 2018
CIELO Collaboration Summary Results: International Evaluations of Neutron Reactions on Uranium, Plutonium, Iron, Oxygen and Hydrogen journal February 2018
A system for differential neutron scattering experiments in the energy range from 0.5 to 20MeV
  • Saglime, F. J.; Danon, Y.; Block, R. C.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 620, Issue 2-3 https://doi.org/10.1016/j.nima.2010.04.051
journal August 2010
Critical review of CIELO evaluations of n + 235 U, 238 U using differential experiments journal January 2018
The JEFF evaluated nuclear data project conference May 2008
JENDL-4.0: A New Library for Nuclear Science and Engineering journal January 2011
Vibrational properties of Pu and Ga in a Pu-Ga alloy from neutron-resonance Doppler spectroscopy journal November 1998
Prompt-fission-neutron spectra in the Pu 239 ( n , f ) reaction journal April 2020
Quasi-Differential Neutron Scattering in Zirconium from 0.5 to 20 MeV journal June 2013
SCINFUL: A Monte Carlo based computer program to determine a scintillator full energy response to neutron detection for E/sub n/ between 0. 1 and 80 MeV: Program development and comparisons of program predictions with experimental data report April 1988